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Twisted magnetocaloric effect by spin-glass driven large exchange bias

Manisha Bansal1,*, Wasim Akram1,*, Samir Kumar Giri2, and Tuhin Maity1,3,†

  • *These authors contributed equally to this work.
  • †Contact author: tuhin@iisertvm.ac.in

Phys. Rev. B 111, L140418 – Published 30 April, 2025

DOI: https://doi.org/10.1103/PhysRevB.111.L140418

Abstract

We observe a twisted magnetocaloric effect (MCE) in a ferrimagnetic SmCaCoMnO6-antiferromagnetic Sm0.1Ca0.9MnO3 composite due to large exchange bias (EB) coupling (maximum EB ∼9.45 kOe at 2 K with a bias field of ∼10 kOe). The isothermal magnetization curves cross each other at high fields, and the crossover field increases with decreasing temperature. This leads to distinct moving peaks at the low temperature (≤15 K) in the nonmonotonic entropy change vs temperature curves, referred to as twisted MCE. The EB is also observed at low temperatures (≤15 K), due to the spin glass formation at the interface of SmCaCoMnO6 and Sm0.1Ca0.9MnO3. Similar materials systems without EB do not show the twisted MCE. Our proposed analytical model correlates the twisted MCE with the interacting anisotropies of spin glass and EB coupling at the interface. The coupled MCE and EB opens up new possibilities of simultaneous spintronic device applications and magnetocaloric refrigeration, leading to self-cooled electronics.

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