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Optically tunable spin Hall effect in periodically driven monolayer transition metal dichalcogenides

Naoya Arakawa1,* and Kenji Yonemitsu1,2

  • 1The Institute of Science and Engineering, Chuo University, Bunkyo, Tokyo 112-8551, Japan
  • 2Department of Physics, Chuo University, Bunkyo, Tokyo 112-8551, Japan

  • *Contact author: arakawa@phys.chuo-u.ac.jp

Phys. Rev. B 111, L121110 – Published 21 March, 2025

DOI: https://doi.org/10.1103/PhysRevB.111.L121110

Abstract

We show that the driving field of circularly polarized light (CPL) can be used to enhance and reverse the spin current generated in the spin Hall effect for some transition metal dichalcogenides. This is demonstrated by analyzing the time-averaged spin Hall conductivities in the nonequilibrium steady states of monolayers WS2, MoS2, MoTe2, and WTe2 driven by CPL with the Floquet linear-response theory. We argue that the enhancement and reversals of the spin current come from a combination of the non-Rashba effect of broken inversion symmetry and the nonperturbative effect of CPL beyond the dynamical localization. This work allows optical control of the magnitude and direction of the pure spin current.

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