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Quantum geometry probed by chiral excitonic optical response of Chern insulators

Wen-Xuan Qiu1 and Fengcheng Wu1,2,*

  • 1School of Physics and Technology, Wuhan University, Wuhan 430072, China
  • 2Wuhan Institute of Quantum Technology, Wuhan 430206, China

  • *Contact author: wufcheng@whu.edu.cn

Phys. Rev. B 111, L121104 – Published 17 March, 2025

DOI: https://doi.org/10.1103/PhysRevB.111.L121104

Abstract

We theoretically derive the sum rule for the negative first moment of the absorptive optical conductivity with excitonic effects and establish its connection to the quantum weight K and Chern number C of the ground state. Applying this framework, we investigate the excitonic optical response of the Chern insulator at a hole filling factor ν=1 in twisted bilayer MoTe2. A single chiral exciton state, which selectively absorbs circularly polarized light of a specific handedness, dominates the optical sum rule. The chiral exciton state comprises two types of interlayer electron-hole transitions, which cancel out the total out-of-plane dipole moment. The absorption spectrum shows nearly perfect magnetic circular dichroism, which can be attributed to the nearly saturated bound K≥|C| of the Chern insulator under study. Our work illustrates the potential of using excitonic optical responses to probe quantum geometry encoded by K and C of Chern insulators in moiré superlattices.

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