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Frustration-enhanced persistent currents in correlated trimer nanorings

Tie-Feng Fang1,*, Wei-Tao Lu1, Ai-Min Guo2, and Qing-Feng Sun3,4,†

  • 1School of Physical Science and Technology, Nantong University, Nantong 226019, China
  • 2Hunan Key Laboratory for Super-microstructure and Ultrafast Process, School of Physics and Electronics, Central South University, Changsha 410083, China
  • 3International Center for Quantum Materials, School of Physics, Peking University, Beijing 100871, China
  • 4Hefei National Laboratory, Hefei 230088, China

  • *Contact author: fangtiefeng@lzu.edu.cn
  • †Contact author: sunqf@pku.edu.cn

Phys. Rev. B 111, L081117 – Published 26 February, 2025

DOI: https://doi.org/10.1103/PhysRevB.111.L081117

Abstract

We investigate the persistent current in a correlated trimer nanoring comprising three magnetic atoms, which sits on a metallic host and encloses a magnetic flux. In the molecular-orbital regime, charge fluctuations can reverse the aromaticity of the trimer molecule by driving quantum phase transitions between many-body states. It is shown that in frustrated trimers the superexchange-induced current as a function of interatom hopping is enhanced by the competition of conflicting magnetic orders, with an asymmetric peak at the quantum criticality separating the ferromagnetic and antiferromagnetic Kondo regimes. Interestingly, the critical current undergoes an anomalous rise with temperature before decaying, signaling the suppression of the Kondo bound state at finite temperature. Our results demonstrate that the coherent current response to external flux indeed conveys important information on the states of strongly correlated systems.

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