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  • Letter

Unveiling the hybridization process in a quantum critical ferromagnet by ultrafast optical spectroscopy

Y. H. Pei1, Y. J. Zhang2,3, Z. X. Wei1,4, Y. X. Chen2, K. Hu1, Yi-feng Yang5,6,7, H. Q. Yuan2,8,9,*, and J. Qi1,†

  • 1State Key Laboratory of Electronic Thin Films and Integrated Devices, University of Electronic Science and Technology of China, Chengdu 611731, China
  • 2Center for Correlated Matter and Department of Physics, Zhejiang University, Hangzhou 310058, China
  • 3Institute for Advanced Materials, Hubei Normal University, Huangshi 435002, China
  • 4Institute of Electronic and Information Engineering, University of Electronic Science and Technology of China, Dongguan 523808, China
  • 5Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Science, Beijing 100190, China
  • 6University of Chinese Academy of Sciences, Beijing 100049, China
  • 7Songshan Lake Materials Laboratory, Dongguan 523808, China
  • 8State Key Laboratory of Silicon Materials, Zhejiang University, Hangzhou 310058, China
  • 9Zhejiang Province Key Laboratory of Quantum Technology and Device, Department of Physics, Zhejiang University, Hangzhou 310058, China

  • *hqyuan@zju.edu.cn
  • †jbqi@uestc.edu.cn

Phys. Rev. B 103, L180409 – Published 25 May, 2021

DOI: https://doi.org/10.1103/PhysRevB.103.L180409

Abstract

We report the ultrafast optical pump-probe spectroscopy measurements on the recently discovered quantum critical ferromagnet CeRh6Ge4. Our experimental results reveal the two-stage development of the hybridization between localized f moments and conduction electrons with lowering temperature, as evidenced by (1) the presence of hybridization fluctuation for temperatures from ∼85K (T*) to ∼140K (T†), and (2) the emergence of collective hybridization below the coherence temperature, T*, marked by the opening of an indirect gap of 2Δ≈12meV. We also observe three coherent phonon modes being softened anomalously below T*, reflecting directly their coupling with the emergent coherent heavy electrons. Our findings establish the universal nature of fluctuation and coherence during the hybridization process in heavy fermion systems.

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