- Letter
Unveiling the hybridization process in a quantum critical ferromagnet by ultrafast optical spectroscopy
Phys. Rev. B 103, L180409 – Published 25 May, 2021
DOI: https://doi.org/10.1103/PhysRevB.103.L180409
Abstract
We report the ultrafast optical pump-probe spectroscopy measurements on the recently discovered quantum critical ferromagnet . Our experimental results reveal the two-stage development of the hybridization between localized moments and conduction electrons with lowering temperature, as evidenced by (1) the presence of hybridization fluctuation for temperatures from () to (), and (2) the emergence of collective hybridization below the coherence temperature, , marked by the opening of an indirect gap of . We also observe three coherent phonon modes being softened anomalously below , reflecting directly their coupling with the emergent coherent heavy electrons. Our findings establish the universal nature of fluctuation and coherence during the hybridization process in heavy fermion systems.