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Fingerprinting triangular-lattice antiferromagnet by excitation gaps

K. E. Avers1,2,3, P. A. Maksimov4, P. F. S. Rosa1, S. M. Thomas1, J. D. Thompson1, W. P. Halperin2, R. Movshovich1, and A. L. Chernyshev5

  • 1Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA
  • 2Department of Physics and Astronomy, Northwestern University, Evanston, Illinois 60208, USA
  • 3Center for Applied Physics and Superconducting Technologies, Northwestern University, Evanston, Illinois 60208, USA
  • 4Bogolyubov Laboratory of Theoretical Physics, Joint Institute for Nuclear Research, Dubna, Moscow Region 141980, Russia
  • 5Department of Physics and Astronomy, University of California, Irvine, California 92697, USA

Phys. Rev. B 103, L180406 – Published 21 May, 2021

DOI: https://doi.org/10.1103/PhysRevB.103.L180406

Abstract

CeCd3As3 is a rare-earth triangular-lattice antiferromagnet with large interlayer separation. Our field-dependent heat capacity measurements at dilution fridge temperatures allow us to trace the field evolution of the spin-excitation gaps throughout the antiferromagnetic and paramagnetic regions. The distinct gap evolution places strong constraints on the microscopic pseudospin model, which, in return, yields a close quantitative description of the gap behavior. This analysis provides crucial insights into the nature of the magnetic state of CeCd3As3, with a certainty regarding its stripe order and low-energy model parameters that sets a compelling paradigm for exploring and understanding the rapidly growing family of the rare-earth-based triangular-lattice systems.

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