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  • Letter

Strongly anisotropic spin dynamics in magnetic topological insulators

A. Alfonsov1,*, J. I. Facio1,*, K. Mehlawat1,2,*, A. G. Moghaddam1,3, R. Ray1, A. Zeugner4, M. Richter1,5, J. van den Brink1,2, A. Isaeva1,6 et al.

B. Büchner1,2 and V. Kataev1

  • 1Leibniz Institute for Solid State and Materials Research, IFW Dresden, D-01069 Dresden, Germany
  • 2Würzburg-Dresden Cluster of Excellence ct.qmat, TU Dresden, D-01062 Dresden, Germany
  • 3Department of Physics, Institute for Advanced Studies in Basic Sciences (IASBS), Zanjan 45137-66731, Iran
  • 4Faculty of Chemistry and Food Chemistry, TU Dresden, D-01062 Dresden, Germany
  • 5Dresden Center for Computational Materials Science (DCMS), TU Dresden, D-01062 Dresden, Germany
  • 6Van der Waals–Zeeman Institute, Institute of Physics, University of Amsterdam, 1098 XH Amsterdam, The Netherlands

  • *These authors contributed equally to this work.

Phys. Rev. B 103, L180403 – Published 19 May, 2021

DOI: https://doi.org/10.1103/PhysRevB.103.L180403

Abstract

The recent discovery of magnetic topological insulators has opened new avenues to explore exotic states of matter that can emerge from the interplay between topological electronic states and magnetic degrees of freedom, be it ordered or strongly fluctuating. Motivated by the effects that the dynamics of the magnetic moments can have on the topological surface states, we investigate the magnetic fluctuations across the (MnBi2Te4)(Bi2Te3)n family. Our paramagnetic electron spin resonance experiments reveal contrasting Mn spin dynamics in different compounds, which manifests in a strongly anisotropic Mn spin relaxation in MnBi2Te4 while being almost isotropic in MnBi4Te7. Our density-functional calculations explain these striking observations in terms of the sensitivity of the local electronic structure to the Mn spin orientation, and indicate that the anisotropy of the magnetic fluctuations can be controlled by the carrier density, which may directly affect the electronic topological surface states.

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