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Physical properties of (Mn1−xCox)Si at x≃0.060–0.100: Quantum criticality

A. E. Petrova, S. Yu. Gavrilkin, and G. V. Rybalchenko

Dirk Menzel

I. P. Zibrov

S. M. Stishov*

  • P. N. Lebedev Physical Institute, Leninsky pr., 53, 119991 Moscow, Russia

  • Institut für Physik der Kondensierten Materie, Technische Universität Braunschweig, D-38106 Braunschweig, Germany

  • Institute for High Pressure Physics of RAS, 108840 Troitsk, Russia

  • P. N. Lebedev Physical Institute, Leninsky pr., 53, 119991 Moscow, Russia

  • *stishovsm@lebedev.ru

Phys. Rev. B 103, L180401 – Published 3 May, 2021

DOI: https://doi.org/10.1103/PhysRevB.103.L180401

Abstract

We have grown and characterized three samples of Co-doped MnSi and studied their physical properties (magnetization and magnetic susceptibility, heat capacity, and electrical resistance). All three samples show non-Fermi liquid physical properties. From literature data and current results it follows that impurities (Co and Fe) eliminate the first-order phase transition peaks and spread the fluctuation maxima in such a way that the low-temperature part effectively reaches the zero temperature, where the fluctuations inevitably become quantum. The behavior of low-temperature parts of the heat capacity of the samples suggests that a gradual transition from classical to quantum fluctuations can be described by a simple power function of temperature with the exponent less than one. The dρ/dT data generally support this suggestion. The values of the heat capacity exponents immediately lead to the diverging ratio Cp/T and hence to the diverging effective electron mass. We found that at a large concentration of the dopant there are no distinct phase transition points. What we observe is probably a region of the helical fluctuations spreading over a significant range of concentrations and temperatures, which become quantum close to 0 K.

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