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Low-energy magneto-optics of Tb2Ti2O7 in a [111] magnetic field

Xinshu Zhang1, Yi Luo1, T. Halloran1, J. Gaudet1, Huiyuan Man1, S. M. Koohpayeh1,2, and N. P. Armitage1

  • 1Institute for Quantum Matter, Department of Physics and Astronomy, The Johns Hopkins University, Baltimore, Maryland 21218, USA
  • 2Department of Materials Science and Engineering, The Johns Hopkins University, Baltimore, Maryland 21218, USA

Phys. Rev. B 103, L140403 – Published 12 April, 2021

DOI: https://doi.org/10.1103/PhysRevB.103.L140403

Abstract

The pyrochlore magnet Tb2Ti2O7 shows a lack of magnetic order to low temperatures and is considered to be a quantum spin liquid candidate. We perform time-domain THz spectroscopy on high-quality Tb2Ti2O7 crystals and study the low-energy excitations as a function of [111] magnetic field with high energy resolution. The low-energy crystal-field excitations change their energies anomalously under magnetic field. Despite several sharp field-dependent changes, we show that the material's spectrum can be described not by phase transitions but by field-dependent hybridization between the low-energy crystal-field levels. We highlight the strong coupling between spin and lattice degrees of freedom in Tb2Ti2O7 as evidenced by the magnetic-field tunable crystal-field environment. Calculations based on single ion physics with field-induced symmetry reduction of the crystal-field environment can reproduce our data.

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