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Strain transfer in ferroelectric-ferrimagnetic magnetoelectric composite

Sujoy Saha1, Ram Prakash Singh1, Ying Liu2,3, Atal Bihari Swain4, Amritesh Kumar5, V. Subramanian4, A. Arockiarajan5, G. Srinivasan2, and Rajeev Ranjan1,*

  • 1Department of Materials Engineering, Indian Institute of Science, Bangalore-560012, India
  • 2Department of Physics, Oakland University, Rochester, Michigan 48309-4479, USA
  • 3Department of Materials Science and Engineering, Hubei University, Wuhan 430062, China
  • 4Department of Physics, Indian Institute of Technology Madras, Chennai-600036, India
  • 5Department of Applied Mechanics, Indian Institute of Technology Madras, Chennai-600036, India

  • *rajeev@iisc.ac.in

Phys. Rev. B 103, L140106 – Published 22 April, 2021

DOI: https://doi.org/10.1103/PhysRevB.103.L140106

Abstract

We show that electrically poled ferroelectric matrix considerably enhances the localized magnetostrictive deformations in a ferroelectric-ferrimagnetic composite. Magnetostrain measurements performed on Dy-free and Dy-modified BiFeO3−PbTiO3 (BF-PT) ferroelectric ceramics revealed no measurable macroscopic strain in poled and unpoled Dy-free nonferromagnetic specimens. Dy-modified BF-PT, on the other hand, exhibit ferrimagnetic dysprosium-iron garnet (DyIG) as precipitates and exhibit a macroscopic strain of −4 ppm in the poled state. Despite the small (6%) volume fraction of DyIG, the macroscopic strain in Dy-modified BF-PT is almost 50% of the strain of pure DyIG. Our results suggest that the amplification of the localized magnetostrictive deformation in the ferrimagnetic islands by the neighboring ferroelectric regions is caused by the magnetostrictive stress-induced motion of ferroelectric-ferroelastic domains of the poled ferroelectric matrix.

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