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  • Letter

Quantum phase transition of a two-dimensional quadrupolar system

G. E. Astrakharchik1, I. L. Kurbakov2, D. V. Sychev3, A. K. Fedorov4,5, and Yu. E. Lozovik2,6,7

  • 1Departament de Física, Campus Nord B4-B5, Universitat Politècnica de Catalunya, E-08034 Barcelona, Spain
  • 2Institute of Spectroscopy, Russian Academy of Sciences, Troitsk, Moscow 142190, Russia
  • 3School of Electrical and Computer Engineering, Purdue University, West Lafayette, Indiana 47907, USA
  • 4Russian Quantum Center, Skolkovo, Moscow 143025, Russia
  • 5Moscow Institute of Physics and Technology, Dolgoprudny, Moscow Region 141700, Russia
  • 6Center for Basic Research, All-Russia Research Institute of Automatics, Moscow 127055, Russia
  • 7MIEM at National Research University HSE, Moscow 109028, Russia

Phys. Rev. B 103, L140101 – Published 1 April, 2021

DOI: https://doi.org/10.1103/PhysRevB.103.L140101

Abstract

Ensembles with long-range interactions between particles are promising for revealing strong quantum collective effects and many-body phenomena. Here we study the ground-state phase diagram of a two-dimensional Bose system with quadrupolar interactions using a diffusion Monte Carlo technique. We predict a quantum phase transition from a gas to a solid phase. The Lindemann ratio and the condensate fraction at the transition point are γ=0.269(4) and n0/n=0.031(4), correspondingly. We observe the strong rotonization of the collective excitation branch in the vicinity of the phase transition point. Our results can be probed using state-of-the-art experimental systems of various nature, such as quasi-two-dimensional systems of quadrupolar excitons in transition metal dichalcogenide trilayers, quadrupolar molecules, and excitons or Rydberg atoms with quadrupole moments induced by strong magnetic fields.

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