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    Mott glass and criticality in an S=12 bilayer Heisenberg model with interlayer bond dilution

    Kunpeng Li (李坤鹏), Han-Qing Wu (邬汉青), and Dao-Xin Yao (姚道新)*

    • *Contact author: yaodaox@mail.sysu.edu.cn

    Phys. Rev. B 112, 214407 – Published 3 December, 2025

    DOI: https://doi.org/10.1103/8wbp-xxz1

    Abstract

    We employ the stochastic series expansion quantum Monte Carlo method to investigate the S=1/2 antiferromagnetic Heisenberg model on a bilayer square lattice with diluted interlayer couplings. Both regular and random dilution patterns are considered. In systems with regular dilution, tuning the interlayer interaction drives a quantum phase transition from a Néel-ordered phase to a quantum disordered phase, consistent with the O(3) universality class. In contrast, random dilution gives rise to a two-step transition: from the Néel phase to an intermediate Mott glass (MG) phase, followed by a transition to the quantum disordered phase. Within the MG phase, the uniform magnetic susceptibility exhibits a stretched-exponential temperature dependence χu∼exp(−b/Tα), 0<α<1. At the Néel-to-glass transition, the quenched disorder modifies the critical exponents in a manner consistent with the Harris criterion. These findings provide new insights into disorder-driven quantum phase transitions and the emergence of glassy phases in diluted bilayer quantum magnets.

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