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Quantum Griffiths phase in the kagome Kondo lattice CeRh0.9Pd0.1Sn

Nan Tang1,*, Rajesh Tripathi2, Yasuyuki Shimura3, Toshiro Takabatake3, Devashibhai A. Adroja2,4, and Philipp Gegenwart1,†

  • 1Experimental Physics VI, Center for Electronic Correlations and Magnetism, University of Augsburg, 86159 Augsburg, Germany
  • 2ISIS Neutron and Muon Source, STFC, Rutherford Appleton Laboratory, Chilton, Oxon OX11 0QX, United Kingdom
  • 3Department of Quantum Matter, Graduate School of Advanced Science and Engineering, Hiroshima University, Higashi-Hiroshima 739-8530, Japan
  • 4Highly Correlated Matter Research Group, Physics Department, University of Johannesburg, Auckland Park 2006, South Africa

  • *Contact author: nan.tang@uni-a.de
  • †Contact author: philipp.gegenwart@uni-a.de

Phys. Rev. B 112, 155151 – Published 23 October, 2025

DOI: https://doi.org/10.1103/8lf7-j26n

Abstract

CeRhSn is a valence fluctuating heavy-fermion metal with a twisted Ce-kagome lattice, displaying zero-field quantum criticality, previously associated with geometrical frustration. The partial substitution of Rh by Pd in CeRh1−xPdxSn enlarges the unit-cell volume, suppresses valence fluctuations, decreases the Kondo temperature, and stabilizes a possible long-range antiferromagnetic (AFM) ordered ground state with TN=0.8 K at x=0.5. Previous thermodynamic and spectroscopic measurements for x=0.1 suggested a quantum critical spin liquid. We report low-temperature dilatometry and magnetization measurements on CeRh0.9Pd0.1Sn and compare with published low-T specific heat data. The absence of a Grüneisen parameter divergence excludes a conventional quantum criticality scenario. Instead, the weak power-law divergences signal non-Fermi-liquid (NFL) behavior, according to a disorder-driven quantum Griffiths phase scenario. At low temperatures, a negative thermal expansion is found in fields above approximately 0.5 T and the NFL scaling breaks down, probably due to the polarization of AFM correlations.

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