Electronic structure and resonant circular dichroism of from soft x-ray angle-resolved photoemission
Phys. Rev. B 114, 185122 – Published 18 September, 2026
DOI: https://doi.org/10.1103/59pf-43kx
Abstract
Coupling between spin, orbital, charge, and lattice degrees of freedom in transition-metal oxides produces a variety of electronic and magnetic phenomena of importance for future technologies. Here, we explore the electronic band structure of a (111)-oriented thin film through soft x-ray angle-resolved photoemission spectroscopy (ARPES). The measurements agree with the electronic band structure calculated with density functional theory using the Hubbard correction. Furthermore, we probe the circular dichroism in ARPES and observe a pronounced momentum-resolved magnetic circular dichroism (MCD) in resonant photoemission from the Mn edge. The momentum distribution of the resonant MCD reproduces that of the Fermi surface, establishing resonant circular dichroism ARPES as a momentum-resolved probe of itinerant Bloch states, with implications for unconventional magnets such as altermagnets and -wave magnets.