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    Electronic structure and resonant circular dichroism of La0.7Sr0.3MnO3 from soft x-ray angle-resolved photoemission

    Øyvind Finnseth1, Damian Brzozowski1, Anders Christian Mathisen2, Stefanie Suzanne Brinkman2, Xin Liang Tan2, Fabian Göhler2, Benjamin A. D. Williamson1, Kristoffer Eggestad1, Meng-Jie Huang3 et al.

    Jens Buck4,3, Moritz Hoesch5, Kai Rossnagel6,3, Sverre M. Selbach1, Hendrik Bentmann2, and Ingrid Hallsteinsen1,*

    • *Contact author: ingrid.g.hallsteinsen@ntnu.no

    Phys. Rev. B 114, 185122 – Published 18 September, 2026

    DOI: https://doi.org/10.1103/59pf-43kx

    Abstract

    Coupling between spin, orbital, charge, and lattice degrees of freedom in transition-metal oxides produces a variety of electronic and magnetic phenomena of importance for future technologies. Here, we explore the electronic band structure of a (111)-oriented La0.7Sr0.3MnO3 thin film through soft x-ray angle-resolved photoemission spectroscopy (ARPES). The measurements agree with the electronic band structure calculated with density functional theory using the Hubbard U correction. Furthermore, we probe the circular dichroism in ARPES and observe a pronounced momentum-resolved magnetic circular dichroism (MCD) in resonant photoemission from the Mn L edge. The momentum distribution of the resonant MCD reproduces that of the Fermi surface, establishing resonant circular dichroism ARPES as a momentum-resolved probe of itinerant Bloch states, with implications for unconventional magnets such as altermagnets and p-wave magnets.

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