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Light-induced transitions of valley Chern numbers and flat bands in a nontwisted moiré graphene–hexagonal boron nitride superlattice

Saud Alabdulal1, Miftah Hadi Syahputra Anfa2, Hocine Bahlouli2,3, and Michael Vogl2,4

Phys. Rev. B 112, 195411 – Published 5 November, 2025

DOI: https://doi.org/10.1103/4zcv-2c1n

Abstract

Motivated by the rich topology and interesting quasiband structure of twisted moiré materials subjected to light, we study a nontwisted moiré material under the influence of light. Our work is in part motivated by a desire to find an easier-to-synthesize platform that can help experimentally elucidate the interesting physics of moiré materials coupled to light. Similar to twisted moiré materials, we uncover rich topology and interesting band flattening effects, which we summarize in relevant plots such as a topological phase diagram. Our work demonstrates that much of the interesting phenomenology of twisted moiré materials under the influence of electromagnetic waves seems to be generically present even in more experimentally accessible untwisted moiré platforms, which remain highly tunable by light.

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References (60)

  1. M. Hentschel, R. Kienberger, Ch. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, Attosecond metrology, Nature (London) 414, 509 (2001).
  2. S. X. Hu and L. A. Collins, Attosecond pump probe: Exploring ultrafast electron motion inside an atom, Phys. Rev. Lett. 96, 073004 (2006).
  3. D. S. Rana, I. Kawayama, K. Mavani, K. Takahashi, H. Murakami, and M. Tonouchi, Understanding the nature of ultrafast polarization dynamics of ferroelectric memory in the multiferroic BiFeO3, Adv. Mater. 21, 2881 (2009).
  4. Y. M. Sheu, S. A. Trugman, L. Yan, Q. X. Jia, A. J. Taylor, and R. P. Prasankumar, Using ultrashort optical pulses to couple ferroelectric and ferromagnetic order in an oxide heterostructure, Nat. Commun. 5, 5832 (2014).
  5. Y. Zhang, J. Dai, X. Zhong, D, Zhang, G. Zhong, and J. Li, Probing ultrafast dynamics of ferroelectrics by time-resolved pump-probe spectroscopy, Adv. Sci. 8, 2102488 (2021).
  6. F. Chen, Y. Zhu, S. Liu, Y. Qi, H. Y. Hwang, N. C. Brandt, J. Lu, F. Quirin, H. Enquist, P. Zalden, T. Hu, J. Goodfellow, M.-J. Sher, M. C. Hoffmann, D. Zhu, H. Lemke, J. Glownia, M. Chollet, A. R. Damodaran, J. Park, and et al., Ultrafast terahertz-field-driven ionic response in ferroelectric BaTiO3, Phy. Rev. B 94, 180104(R) (2016).
  7. D. Stich, F. Späth, H. Kraus, A. Sperlich, V. Dyakonov, and T. Hertel, Triplet–triplet exciton dynamics in single-walled carbon nanotubes, Nat. Photon. 8, 139 (2014).
  8. Y. Bai, J.-H. Olivier, G. Bullard, C. Liu, and M. J. Therien, Dynamics of charged excitons in electronically and morphologically homogeneous single-walled carbon nanotubes, Proc. Natl. Acad. Sci. USA 115, 674 (2018).
  9. K. Birkmeier, T. Hertel, and A. Hartschuh, Probing the ultrafast dynamics of excitons in single semiconducting carbon nanotubes, Nat. Commun. 13, 6290 (2022).
  10. M. F. Jager, C. Ott, P. M. Kraus, C. J. Kaplan, W. Pouse, R. E. Marvel, R. F. Haglund, D. M. Neumark, and S. R. Leone, Tracking the insulator-to-metal phase transition in VO2 with few-femtosecond extreme uv transient absorption spectroscopy, Proc. Natl. Acad. Sci. USA 114, 9558 (2017).
  11. M. R. Bionta, E. Haddad, A. Leblanc, V. Gruson, P. Lassonde, H. Ibrahim, J. Chaillou, N. Émond, M. R. Otto, Á. Jiménez-Galán, R. E. F. Silva, M. Ivanov, B. J. Siwick, M. Chaker, and F. Légaré, Tracking ultrafast solid-state dynamics using high harmonic spectroscopy, Phys. Rev. Res. 3, 023250 (2021).
  12. M. Deb, E. Popova, H.-Y. Jaffrès, N. Keller, and M. Bargheer, Controlling high-frequency spin-wave dynamics using double-pulse laser excitation, Phys. Rev. Appl. 18, 044001 (2022).
  13. C. E. Graves, A. H. Reid, T. Wang, B. Wu, S. de Jong, K. Vahaplar, I. Radu, D. P. Bernstein, M. Messerschmidt, L. Müller, R. Coffee et al., Nanoscale spin reversal by non-local angular momentum transfer following ultrafast laser excitation in ferrimagnetic GdFeCo, Nat. Mater. 12, 293 (2013).
  14. C. D. Stanciu, F. Hansteen, A. V. Kimel, A. Kirilyuk, A. Tsukamoto, A. Itoh, and Th Rasing, All-optical magnetic recording with circularly polarized light, Phys. Rev. Lett. 99, 047601 (2007).
  15. M. Rini, R. Tobey, N. Dean, J. Itatani, Y. Tomioka, Y. Tokura, R. W. Schoenlein, and A. Cavalleri, Control of the electronic phase of a manganite by mode-selective vibrational excitation, Nature (London) 449, 72 (2007).
  16. S. A. Weidinger and M. Knap, Floquet prethermalization and regimes of heating in a periodically driven, interacting quantum system, Sci. Rep. 7, 45382 (2017).
  17. U. De Giovannini, and H. Hübener, Floquet analysis of excitations in materials, J. Phys. Mater. 3, 012001 (2019).
  18. T. Oka and S. Kitamura, Floquet engineering of quantum materials, Annu. Rev. Condens. Matter Phys. 10, 387 (2019).
  19. M. A. Sentef, M. Claassen, A. F. Kemper, B. Moritz, T. Oka, J. K. Freericks, and T. P. Devereaux, Theory of Floquet band formation and local pseudospin textures in pump-probe photoemission of graphene, Nat. Commun. 6, 7047 (2015).
  20. S. Ito, M. Schüler, M. Meierhofer, S. Schlauderer, J. Freudenstein, J. Reimann, D. Afanasiev, K. A. Kokh, O. E. Tereshchenko, J. Güdde et al., Build-up and dephasing of Floquet–Bloch bands on subcycle timescales, Nature (London) 616, 696 (2023).
  21. M. A. Sentef, J. Li, F. Künzel, and M. Eckstein, Quantum to classical crossover of Floquet engineering in correlated quantum systems, Phys. Rev. Res. 2, 033033 (2020).
  22. D. M. Kennes, M. Claassen, M. A. Sentef, and C. Karrasch, Light-induced d-wave superconductivity through Floquet-engineered Fermi surfaces in cuprates, Phys. Rev. B 100, 075115 (2019).
  23. C. J. Eckhardt, G. Passetti, M. Othman, C. Karrasch, F. Cavaliere, M. A. Sentef, and D. M. Kennes, Quantum Floquet engineering with an exactly solvable tight-binding chain in a cavity, Commun. Phys. 5, 122 (2022).
  24. G. E. Topp, C. J. Eckhardt, D. M. Kennes, M. A. Sentef, and P. Törmä, Light-matter coupling and quantum geometry in moiré materials, Phys. Rev. B 104, 064306 (2021).
  25. E. V. Boström, M. Claassen, J. McIver, G. Jotzu, A. Rubio, and M. Sentef, Light-induced topological magnons in two-dimensional van der Waals magnets, SciPost Phys. 9, 061 (2020).
  26. O. V. Kibis, I. V. Iorsh, and I. A. Shelykh, Floquet engineering of 2D materials, J. Phys.: Conf. Ser. 1461, 012064 (2020).
  27. X. Kong, W. Luo, L. Li, M. Yoon, T. Berlijn, and L. Liang, Floquet band engineering and topological phase transitions in 1t' transition metal dichalcogenides, 2D Mater. 9, 025005 (2022).
  28. M. S. Rudner, and N. H. Lindner, Band structure engineering and non-equilibrium dynamics in Floquet topological insulators, Nat. Rev. Phys. 2, 229 (2020).
  29. A. Castro, U. De Giovannini, S. A. Sato, H. Hübener, and A. Rubio, Floquet engineering the band structure of materials with optimal control theory, Phys. Rev. Res. 4, 033213 (2022).
  30. R. Fleury, A. B Khanikaev, and A. Alù, Floquet topological insulators for sound, Nat. Commun. 7, 11744 (2016).
  31. F. Zhan, J. Zeng, Z. Chen, X. Jin, J. Fan, T. Chen, and R. Wang, Floquet engineering of nonequilibrium valley-polarized quantum anomalous Hall effect with tunable Chern number, Nano Lett. 23, 2166 (2023).
  32. D. Shin, H. Hübener, U. De Giovannini, H. Jin, A. Rubio, and N. Park, Phonon-driven spin-Floquet magneto-valleytronics in MoS2, Nat. Commun. 9, 638 (2018).
  33. H. Cao, J.-T. Sun, and S. Meng, Floquet engineering of anomalous Hall effects in monolayer MoS2, npj Quantum Mater. 9, 90 (2024).
  34. A. G. Grushin, Á. Gómez-León, and T. Neupert, Floquet fractional Chern insulators, Phys. Rev. Lett. 112, 156801 (2014).
  35. Y. Ashida, A. İmamoğlu, J. Faist, D. Jaksch, A. Cavalleri, and E. Demler, Quantum electrodynamic control of matter: Cavity-enhanced ferroelectric phase transition, Phys. Rev. X 10, 041027 (2020).
  36. Y. Li, H. A. Fertig, and B. Seradjeh, Floquet-engineered topological flat bands in irradiated twisted bilayer graphene, Phys. Rev. Res. 2, 043275 (2020).
  37. G. E. Topp, G. Jotzu, J. W. McIver, L. Xian, A. Rubio, and M. A. Sentef, Topological Floquet engineering of twisted bilayer graphene, Phys. Rev. Res. 1, 023031 (2019).
  38. M. Vogl, M. Rodriguez-Vega, and G. A. Fiete, Effective Floquet Hamiltonians for periodically driven twisted bilayer graphene, Phys. Rev. B 101, 235411, (2020).
  39. M. Vogl, M. Rodriguez-Vega, B. Flebus, A. H. MacDonald, and G. A. Fiete, Floquet engineering of topological transitions in a twisted transition metal dichalcogenide homobilayer, Phys. Rev. B 103, 014310 (2021).
  40. A. Dubey, R. Kundu, and A. Kundu, Time-resolved ARPES and optical transport properties of irradiated twisted bilayer graphene in a steady state, Phys. Rev. B 111, 035431 (2025).
  41. M. Mitrano, A. Cantaluppi, D. Nicoletti, S. Kaiser, A. Perucchi, S. Lupi, P. Di Pietro, D. Pontiroli, M. Riccò, S. R. Clark, D. Jaksch, and A. Cavalleri, Possible light-induced superconductivity in K3C60 at high temperature, Nature (London) 530, 461 (2016).
  42. D. Fausti, R. I. Tobey, N. Dean, S. Kaiser, A. Dienst, M. C. Hoffmann, S. Pyon, T. Takayama, H. Takagi, and A. Cavalleri, Light-induced superconductivity in a stripe-ordered cuprate, Science 331, 189 (2011).
  43. M. Suda, R. Kato, and H. M. Yamamoto, Light-induced superconductivity using a photoactive electric double layer, Science 347, 743 (2015).
  44. S. Fava, G. De Vecchi, G. Jotzu, M. Buzzi, T. Gebert, Y. Liu, B. Keimer, and A. Cavalleri, Magnetic field expulsion in optically driven YBa2Cu3O6.48, Nature (London) 632, 75 (2024).
  45. T. F. Nova, A. S. Disa, M. Fechner, and A. Cavalleri, Metastable ferroelectricity in optically strained SrTiO3, Science 364, 1075 (2019).
  46. X. Li, T. Qiu, J. Zhang, E. Baldini, J. Lu, A. M. Rappe, and K. A. Nelson, Terahertz field–induced ferroelectricity in quantum paraelectric SrTiO3, Science 364, 1079 (2019).
  47. T. F. Nova, A. Cartella, A. Cantaluppi, M. Först, D. Bossini, R. V. Mikhaylovskiy, A. V. Kimel, R. Merlin, and A. Cavalleri, An effective magnetic field from optically driven phonons, Nat. Phys. 13, 132 (2017).
  48. J. W. McIver, B. Schulte, F.-U. Stein, T. Matsuyama, G. Jotzu, G. Meier, and A. Cavalleri, Light-induced anomalous Hall effect in graphene, Nat. Phys. 16, 38 (2020).
  49. M. H. S. Anfa, S. Elatresh, H. Bahlouli, and M. Vogl, Effective k-valley Hamiltonian for transition metal dichalcogenide bilayers under pressure and application to twisted bilayers with pressure-induced topological phase transitions, Phys. Rev. B 111, 245434 (2025).
  50. P. Moon and M. Koshino, Electronic properties of graphene/hexagonal-boron-nitride moiré superlattice, Phys. Rev. B 90, 155406 (2014).
  51. M. Koshino and T. Ando, Electronic Properties of Monolayer and Multilayer Graphene (Springer International Publishing, Cham, 2013), pp. 173–211.
  52. L. Liu, Y. P. Feng, and Z. X. Shen, Structural and electronic properties of h-BN, Phys. Rev. B 68, 104102 (2003).
  53. J. Sławińska, I. Zasada, and Z. Klusek, Energy gap tuning in graphene on hexagonal boron nitride bilayer system, Phys. Rev. B 81, 155433 (2010).
  54. F. Bloch, Über die quantenmechanik der elektronen in kristallgittern, Z. Phys. 52, 555 (1929).
  55. H. Sambe, Steady states and quasienergies of a quantum-mechanical system in an oscillating field, Phys. Rev. A 7, 2203 (1973).
  56. M. S. Rudner, N. H. Lindner, E. Berg, and M. Levin, Anomalous edge states and the bulk-edge correspondence for periodically driven two-dimensional systems, Phys. Rev. X 3, 031005 (2013).
  57. L. Wawer and M. Fleischhauer, Chern number and Berry curvature for Gaussian mixed states of fermions, Phys. Rev. B 104, 094104 (2021).
  58. T. Fukui, Y. Hatsugai, and H. Suzuki, Chern numbers in discretized brillouin zone: Efficient method of computing (spin) Hall conductances, J. Phys. Soc. Jpn. 74, 1674 (2005).
  59. D. J. Thouless, M. Kohmoto, M. P. Nightingale, and M. den Nijs, Quantized Hall conductance in a two-dimensional periodic potential, Phys. Rev. Lett. 49, 405 (1982).
  60. https://github.com/miftahhadi/driven_ghbn.

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