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    Multipiezo effect in a two-dimensional Janus altermagnetic Fe2MoS2Se2 monolayer

    Rui Yang1, Bo Zhao2, Huan Yang1, Xue Jiang3,*, Jijun Zhao3, and Yujun Zheng1,†

    • *Contact author: jiangx@scnu.edu.cn
    • †Contact author: yzheng@sdu.edu.cn

    Phys. Rev. B 114, 154425 – Published 24 September, 2026

    DOI: https://doi.org/10.1103/45hv-7fqp

    Abstract

    Two-dimensional (2D) altermagnets (AMs), characterized by distinctive spin splitting and robustness against external fields, have emerged as promising candidates for spintronic device applications. Exploring multipiezo effects in 2D AMs through precise and energy-efficient modulation strategies has become crucial for realizing their multifunctional applications. In this work, we demonstrate that the Fe2MoS2Se2 monolayer is a 2D AM with a pronounced spin splitting of 0.45 eV for valence bands. The Fe2MoS2Se2 monolayer exhibits valley degeneracy at the X/X′ valleys, which is protected by [C2∥C4z] and [C2∥Mxy] symmetries. Uniaxial strain as an energy-efficient modulation strategy breaks the balance of these symmetries. This imbalance induces piezomagnetic and piezovalley effects in Fe2MoS2Se2 monolayer, accompanied by the emergence of an anomalous valley Hall effect. Furthermore, Fe2MoS2Se2 monolayer possesses a Janus structure, which enables significant in-plane and out-of-plane piezoelectric effects under uniaxial strain. The multipiezo effects make the Janus Fe2MoS2Se2 monolayer a promising platform for the development of multifunctional spintronic devices.

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