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    Partially polarized order in the orthogonal Ising Shastry-Sutherland magnet BaNd2PdS5

    Ying Fu1,2, Qiye Liu3, Han Ge2, Nan Zhao4,5,2, Tiantian Li2, Fangli Li2, Huanpeng Bu2, Jiayue Yuan2, Junyu Li2 et al.

    Jun-Feng Dai6, Jieming Sheng7, and Liusuo Wu2,1,8,*

    • *Contact author: wuls@sustech.edu.cn

    Phys. Rev. B 114, 154410 – Published 10 September, 2026

    DOI: https://doi.org/10.1103/3hb8-jqw3

    Abstract

    We report a comprehensive study of single-crystal BaNd2PdS5, a Shastry-Sutherland lattice (SSL) antiferromagnet. Thermodynamic and magnetization measurements identify an AFM transition at TN≈3.6K. The Nd3+ local-crystal-field environment imposes a rigid, mutually orthogonal Ising anisotropy, effectively splitting the SSL into two perpendicular magnetic sublattices. This orthogonal spin texture is demonstrated by a pronounced in-plane anisotropy: the saturation magnetization and the critical fields for suppressing AFM order along [100] and [110] directions differ by a factor of about 2, in close agreement with a minimal two-sublattice model. The low-temperature phase diagram for B∥[110] reveals a field-induced quantum critical point near 2.2 T and a sublattice-selective partially polarized ordered state, in which the field-coupled sublattice is polarized while the orthogonal sublattice remains antiferromagnetically ordered. Together, these results establish BaNd2PdS5 as a platform to explore how lattice and site symmetries constrain collective magnetism in frustrated insulators and to guide engineering of sublattice-selective quantum criticality.

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