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    Characterization of unidirectional charge states in NbSe2 nanoribbonlike structures

    Lili Zhou1,2, Yu Zhang1,2,*, Liangguang Jia1, Yaoyao Chen1, Can Zhang1,2, Fudi Zhou1,2, Shuyi He1, Shuangquan Qu1, Jia-Bin Qiao3 et al.

    Xiaolong Xu1, Teng Zhang1, Huixia Yang1,†, Lijun Zhang4, and Yeliang Wang1,‡

    • 1School of Integrated Circuits and Electronics, MIIT Key Laboratory for Low-Dimensional Quantum Structure and Devices, Beijing Institute of Technology, Beijing 100081, China
    • 2School of Interdisciplinary Science, Beijing Institute of Technology, Beijing 100081, China
    • 3Centre for Quantum Physics, Key Laboratory of Advanced Optoelectronic Quantum Architecture and Measurement, School of Physics, Beijing Institute of Technology, Beijing 100081, China
    • 4State Key Laboratory of Integrated Optoelectronics, Key Laboratory of Automobile Materials of MOE, Key Laboratory of Material Simulation Methods & Software of MOE, and School of Materials Science and Engineering, Jilin University, Changchun, China

    • *Contact author: yzhang@bit.edu.cn
    • †Contact author: yanghuixia@bit.edu.cn
    • ‡Contact author: yeliang.wang@bit.edu.cn

    Phys. Rev. B 112, 035424 – Published 24 July, 2025

    DOI: https://doi.org/10.1103/2clm-692k

    Abstract

    Nanoribbons derived from two-dimensional (2D) materials can exhibit extraordinary electronic properties that are not present in their monolayer counterparts. Fabricating nanoribbons of 2D materials with intrinsic collective electronic states and uncovering the underlying quantum confinement effects are fundamental concepts in both physics and nanotechnology. Monolayer NbSe2 is a model system in this regard, as it has been proved to host a 3×3 charge-density-wave ground state. However, discrete NbSe2 nanoribbons have not been produced yet. Here, we successfully fabricate quantities of NbSe2 nanoribbonlike structures, where the atoms spontaneously reconstruct into a 7×1 stripe phase. Our spectroscopic measurements further reveal a unidirectional charge density modulation in NbSe2 nanoribbonlike structures, with the charge states exhibiting an out-of-phase accumulation on the two sides of −0.15 V. These findings establish NbSe2 nanoribbons as an intriguing platform for exploring one-dimensional-confined collective electronic states, offering a stepping stone toward nanoelectronic devices.

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