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    Néel-vector-dependent magneto-optical and spin Hall responses in altermagnetic CrSb

    Zongying Wang1 and Weiyi Pan2,*

    • *Contact author: weiyi.pan@physik.uni-regensburg.de

    Phys. Rev. B 114, 204421 – Published 20 October, 2026

    DOI: https://doi.org/10.1103/148w-67vq

    Abstract

    Altermagnets enable spin-split bands and anomalous transport phenomena with vanishing net magnetization, yet the symmetry-governed dependence of their optical and spin transport responses on the Néel-vector orientation remains largely unexplored. Using first-principles calculations and systematic magnetic point group analysis, we establish the complete response tensor forms dictated by the magnetic point group for the typical altermagnet CrSb, revealing a fundamental dichotomy: first-order Kerr/Faraday effects, governed by the antisymmetric optical conductivity, are odd functions of the Néel vector, while second-order Voigt/Schäfer-Hubert effects, determined by diagonal dielectric anisotropies, are even functions. Quantitatively, the Kerr rotation angle reaches up to ∼0.55mrad, the Faraday rotation up to ∼6.9×105mrad/cm, and the Voigt rotation up to ∼106mrad/cm, with their angular dependencies following distinct symmetry patterns. For the spin Hall effect, the time-reversal-odd (T-odd) and time-reversal-even (T-even) contributions to the spin Hall conductivity coexist and are of comparable magnitude (∼102ℏeScm). In the ground-state Néel configuration along the c axis, the T-even spin Hall conductivity reaches 265ℏeScm, while the T-odd component is 85ℏeScm, corresponding to charge-to-spin conversion efficiencies of 1.63% and 0.52%, respectively. Notably, reorienting the Néel vector not only modulates the transverse spin Hall components but also activates longitudinal spin-current–charge-current configurations (e.g., σxxSz and σyySz for N||12a+b), which are strictly forbidden in the conventional spin Hall effect. These results establish a comprehensive, symmetry-governed framework for the Néel-vector dependence of magneto-optical and spin-transport responses in CrSb, offering a multidimensional response spectrum for probing the Néel vector direction.

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