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    Quantitative isolation of spin Hall magnetoresistance at antiferromagnetic insulator interfaces

    Yufan Wang1, Yi Huang1, Jiarui Niu1, Shuai Zhang1, Mengdi Yin1,4, Hongna Gu1, Zeyi Zhu1, Haotian Duan1, Xiao Xiao1 et al.

    Lina Chen2,3, Yongbing Xu4, and Ronghua Liu1,4,*

    • *Contact author: rhliu@nju.edu.cn

    Phys. Rev. Applied 26, 044001 – Published 1 October, 2026

    DOI: https://doi.org/10.1103/l9cl-c39r

    Abstract

    We investigated the competing mechanisms of spin Hall magnetoresistance (SMR) and ordinary magnetoresistance (OMR) in van der Waals A-type antiferromagnet CrPS4/Pt heterostructures. By engineering the Pt thickness, we demonstrate a clear crossover from an SMR-dominated regime in thin (5 nm) Pt bilayers to an OMR-dominated regime in thick (30 nm) ones, providing a reliable protocol for isolating the elusive SMR signal from the OMR signal. Strikingly, a robust SMR persists at room temperature, far exceeding the bulk Néel temperature (TN≈38  K), which we attribute to a magnetic proximity-induced interfacial state. A field-dependent phase shift in the SMR angular response across TN reveals that this interfacial magnetism is distinct from the bulk antiferromagnetic order. Complementary anomalous Hall effect measurements independently confirm the existence of this interfacial magnetization. Our work not only establishes CrPS4 as a promising room-temperature spintronic material but also establishes thickness-dependent magnetotransport as a powerful tool for probing interfacial magnetic phenomena in antiferromagnetic heterojunctions.

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