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  • Featured in Physics
  • Open Access

Determining the 3P0 Excited-State Tune-Out Wavelength of 174Yb in a Triple-Magic Lattice

Tim O. Höhn1,2, René A. Villela1,2, Er Zu1,2, Leonardo Bezzo1,2,*, Ronen M. Kroeze1,2, and Monika Aidelsburger1,2,3,†

  • *Current address: ICFO - Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology, 08860 Castelldefels (Barcelona), Spain.
  • †Contact author: Monika.Aidelsburger@physik.uni-muenchen.de

PRX Quantum 7, 010303 – Published 6 January, 2026

DOI: https://doi.org/10.1103/32q9-j82c

Abstract

Precise state-dependent control of optical potentials is of great importance for various applications utilizing cold neutral atoms. In particular, tune-out wavelengths for the clock state pair in alkaline-earth(-like) atoms provide maximally state-selective trap conditions that hold promise for the realization of novel approaches in quantum computation and simulation. While several ground-state tune-out wavelengths have been determined, similar experimental studies for metastable excited states are challenged by inelastic collisions and Raman losses, so far prohibiting precise measurements of excited-state tune-out conditions. In this work we report on the measurement of a tune-out wavelength for the metastable 3P0 clock state in 174Yb at 519.920(9) THz. In order to circumvent collisional losses, we isolate individual 3P0 atoms in a two-dimensional clock-magic-wavelength lattice at 759 nm. To minimize the limitation imposed by Raman scattering, we further implement resolved sideband cooling on the clock transition, which allows us to reduce the lattice depth and surpass lifetimes of 5 s. The precision of the tune-out measurement is further enhanced by fluorescence imaging in a triple-magic configuration, where we implement molasses cooling on the 3P1 intercombination line and identify a magic angle of 38.5(9)∘ in the clock-magic lattice.

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synopsis

A Color Ignored by Atoms

Published 6 January, 2026

At a newly identified wavelength, trapping light avoids disturbing a specific excited atomic state.

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References (69)

  1. J. W. Lis, A. Senoo, W. F. McGrew, F. Rönchen, A. Jenkins, and A. M. Kaufman, Midcircuit operations using the omg architecture in neutral atom arrays, Phys. Rev. X 13, 041035 (2023).
  2. S. Ma, G. Liu, P. Peng, B. Zhang, S. Jandura, J. Claes, A. P. Burgers, G. Pupillo, S. Puri, and J. D. Thompson, High-fidelity gates and mid-circuit erasure conversion in an atomic qubit, Nature 622, 279 (2023).
  3. W. Huie, L. Li, N. Chen, X. Hu, Z. Jia, WonKyuCalvin Sun, and J. P. Covey, Repetitive readout and real-time control of nuclear spin qubits in 171Yb atoms, PRX Quantum 4, 030337 (2023).
  4. B. W. Reichardt et al., Fault-tolerant quantum computation with a neutral atom processor, ArXiv:2411.11822.
  5. F. Scazza, C. Hofrichter, M. Höfer, P. C. De Groot, I. Bloch, and S. Fölling, Observation of two-orbital spin-exchange interactions with ultracold SU(N)-symmetric fermions, Nat. Phys. 10, 779 (2014).
  6. G. Pagano, M. Mancini, G. Cappellini, P. Lombardi, F. Schäfer, H. Hu, X.-J. Liu, J. Catani, C. Sias, M. Inguscio, and L. Fallani, A one-dimensional liquid of fermions with tunable spin, Nat. Phys. 10, 198 (2014).
  7. S. Taie, E. Ibarra-García-Padilla, N. Nishizawa, Y. Takasu, Y. Kuno, H.-T. Wei, R. T. Scalettar, K. R. Hazzard, and Y. Takahashi, Observation of antiferromagnetic correlations in an ultracold SU(N) Hubbard model, Nat. Phys. 18, 1356 (2022).
  8. G. Pasqualetti, O. Bettermann, N. Darkwah Oppong, E. Ibarra-García-Padilla, S. Dasgupta, R. T. Scalettar, K. R. A. Hazzard, I. Bloch, and S. Fölling, Equation of state and thermometry of the 2D SU(N) Fermi-Hubbard model, Phys. Rev. Lett. 132, 083401 (2024).
  9. J. Ye, H. J. Kimble, and H. Katori, Quantum state engineering and precision metrology using state-insensitive light traps, Science 320, 1734 (2008).
  10. A. D. Ludlow, M. M. Boyd, J. Ye, E. Peik, and P. O. Schmidt, Optical atomic clocks, Rev. Mod. Phys. 87, 637 (2015).
  11. A. Aeppli, K. Kim, W. Warfield, M. S. Safronova, and J. Ye, Clock with 8×10−19 systematic uncertainty, Phys. Rev. Lett. 133, 023401 (2024).
  12. M. A. Norcia, A. W. Young, W. J. Eckner, E. Oelker, J. Ye, and A. M. Kaufman, Seconds-scale coherence on an optical clock transition in a tweezer array, Science 366, 93 (2019).
  13. I. S. Madjarov, A. Cooper, A. L. Shaw, J. P. Covey, V. Schkolnik, T. H. Yoon, J. R. Williams, and M. Endres, An atomic-array optical clock with single-atom readout, Phys. Rev. X 9, 041052 (2019).
  14. A. Cao, W. J. Eckner, T. Lukin Yelin, A. W. Young, S. Jandura, L. Yan, K. Kim, G. Pupillo, J. Ye, N. Darkwah Oppong, and A. M. Kaufman, Multi-qubit gates and Schrödinger cat states in an optical clock, Nature 634, 315 (2024).
  15. S. Kolkowitz, S. Bromley, T. Bothwell, M. Wall, G. Marti, A. Koller, X. Zhang, A. Rey, and J. Ye, Spin–orbit-coupled fermions in an optical lattice clock, Nature 542, 66 (2017).
  16. M. Mancini, G. Pagano, G. Cappellini, L. Livi, M. Rider, J. Catani, C. Sias, P. Zoller, M. Inguscio, M. Dalmonte, and L. Fallani, Observation of chiral edge states with neutral fermions in synthetic Hall ribbons, Science 349, 1510 (2015).
  17. T. W. Zhou, T. Beller, G. Masini, J. Parravicini, G. Cappellini, C. Repellin, T. Giamarchi, J. Catani, M. Filippone, and L. Fallani, Measuring Hall voltage and Hall resistance in an atom-based quantum simulator, ArXiv:2411.09744.
  18. Z. W. Barber, J. E. Stalnaker, N. D. Lemke, N. Poli, C. W. Oates, T. M. Fortier, S. A. Diddams, L. Hollberg, C. W. Hoyt, A. V. Taichenachev, and V. I. Yudin, Optical lattice induced light shifts in an Yb atomic clock, Phys. Rev. Lett. 100, 103002 (2008).
  19. C. Chen, G. Bornet, M. Bintz, G. Emperauger, L. Leclerc, V. S. Liu, P. Scholl, D. Barredo, J. Hauschild, S. Chatterjee, M. Schuler, A. Läuchli, M. P. Zaletel, T. Lahaye, N. Y. Yao, and A. Browaeys, Continuous symmetry breaking in a two-dimensional Rydberg array, Nature 616, 691 (2023).
  20. D. Bluvstein et al., Logical quantum processor based on reconfigurable atom arrays, Nature 626, 58 (2024).
  21. N. Darkwah Oppong, G. Pasqualetti, O. Bettermann, P. Zechmann, M. Knap, I. Bloch, and S. Fölling, Probing transport and slow relaxation in the mass-imbalanced Fermi-Hubbard model, Phys. Rev. X 12, 031026 (2022).
  22. F. M. Surace, P. Fromholz, N. Darkwah Oppong, M. Dalmonte, and M. Aidelsburger, Ab initio derivation of lattice-gauge-theory dynamics for cold gases in optical lattices, PRX Quantum 4, 020330 (2023).
  23. A. González-Tudela, and J. I. Cirac, Cold atoms in twisted-bilayer optical potentials, Phys. Rev. A 100, 053604 (2019).
  24. X.-W. Luo, and C. Zhang, Spin-twisted optical lattices: Tunable flat bands and Larkin-Ovchinnikov superfluids, Phys. Rev. Lett. 126, 103201 (2021).
  25. G. Pagano, F. Scazza, and M. Foss-Feig, Fast and scalable quantum information processing with two-electron atoms in optical tweezer arrays, Adv. Quantum Tech. 2, 1800067 (2019).
  26. A. J. Daley, M. M. Boyd, J. Ye, and P. Zoller, Quantum computing with alkaline-earth-metal atoms, Phys. Rev. Lett. 101, 170504 (2008).
  27. D. González-Cuadra, D. Bluvstein, M. Kalinowski, R. Kaubruegger, N. Maskara, P. Naldesi, T. V. Zache, A. M. Kaufman, M. D. Lukin, H. Pichler, B. Vermersch, J. Ye, and P. Zoller, Fermionic quantum processing with programmable neutral atom arrays, Proc. Natl. Acad. Sci. USA 120, e2304294120 (2023).
  28. T. O. Höhn, E. Staub, G. Brochier, N. Darkwah Oppong, and M. Aidelsburger, State-dependent potentials for the 1S0 and 3P0 clock states of neutral ytterbium atoms, Phys. Rev. A 108, 053325 (2023).
  29. See Supplemental Material at http://link.aps.org/supplemental/10.1103/32q9-j82c, which includes Refs. [64, 65, 66, 67, 68, 69], for additional information about the experimental setup and sequences, the initial state characterization, read-out techniques, additional data and error analysis for the magic angle and tune-out measurements, experimental results on the Raman scattering rate and the differential light shift at fto and at the clock resonance, and a discussion of the expanded empirical polarizability model.
  30. M. S. Safronova, Z. Zuhrianda, U. I. Safronova, and C. W. Clark, Extracting transition rates from zero-polarizability spectroscopy, Phys. Rev. A 92, 040501(R) (2015).
  31. M. A. Norcia, A. W. Young, and A. M. Kaufman, Microscopic control and detection of ultracold strontium in optical-tweezer arrays, Phys. Rev. X 8, 041054 (2018).
  32. G. Unnikrishnan, P. Ilzhöfer, A. Scholz, C. Hölzl, A. Götzelmann, R. K. Gupta, J. Zhao, J. Krauter, S. Weber, N. Makki, H. P. Büchler, T. Pfau, and F. Meinert, Coherent control of the fine-structure qubit in a single alkaline-earth atom, Phys. Rev. Lett. 132, 150606 (2024).
  33. M. Ammenwerth, H. Timme, F. Gyger, R. Tao, I. Bloch, and J. Zeiher, Realization of a fast triple-magic all-optical qutrit in 88Sr, Phys. Rev. Lett. 135, 143401 (2025).
  34. A. Cooper, J. P. Covey, I. S. Madjarov, S. G. Porsev, M. S. Safronova, and M. Endres, Alkaline-earth atoms in optical tweezers, Phys. Rev. X 8, 041055 (2018).
  35. A. Heinz, A. J. Park, N. Šantić, J. Trautmann, S. G. Porsev, M. S. Safronova, I. Bloch, and S. Blatt, State-dependent optical lattices for the strontium optical qubit, Phys. Rev. Lett. 124, 203201 (2020).
  36. L. Franchi, L. F. Livi, G. Cappellini, G. Binella, M. Inguscio, J. Catani, and L. Fallani, State-dependent interactions in ultracold 174Yb probed by optical clock spectroscopy, New J. Phys. 19, 103037 (2017).
  37. R. Bouganne, M. B. Aguilera, A. Dareau, E. Soave, J. Beugnon, and F. Gerbier, Clock spectroscopy of interacting bosons in deep optical lattices, New J. Phys. 19, 113006 (2017).
  38. C. D. Herold, V. D. Vaidya, X. Li, S. L. Rolston, J. V. Porto, and M. S. Safronova, Precision measurement of transition matrix elements via light shift cancellation, Phys. Rev. Lett. 109, 243003 (2012).
  39. A. Ratkata, P. D. Gregory, A. D. Innes, A. J. Matthies, L. A. McArd, J. M. Mortlock, M. S. Safronova, S. L. Bromley, and S. L. Cornish, Measurement of the tune-out wavelength for 133Cs at 880 nm, Phys. Rev. A 104, 052813 (2021).
  40. F. Schmidt, D. Mayer, M. Hohmann, T. Lausch, F. Kindermann, and A. Widera, Precision measurement of the 87Rb tune-out wavelength in the hyperfine ground state F=1 at 790 nm, Phys. Rev. A 93, 022507 (2016).
  41. W. Kao, Y. Tang, N. Q. Burdick, and B. L. Lev, Anisotropic dependence of tune-out wavelength near Dy 741-nm transition, Opt. Express 25, 3411 (2017).
  42. J. Catani, G. Barontini, G. Lamporesi, F. Rabatti, G. Thalhammer, F. Minardi, S. Stringari, and M. Inguscio, Entropy exchange in a mixture of ultracold atoms, Phys. Rev. Lett. 103, 140401 (2009).
  43. R. M. Kroeze, R. A. Villela, E. Zu, T. O. Höhn, and M. Aidelsburger, Isotope-agnostic motional ground-state cooling of neutral Yb atoms, Phys. Rev. Res. (to be published).
  44. S. Dörscher, R. Schwarz, A. Al-Masoudi, S. Falke, U. Sterr, and C. Lisdat, Lattice-induced photon scattering in an optical lattice clock, Phys. Rev. A 97, 063419 (2018).
  45. R. Yamamoto, J. Kobayashi, T. Kuno, K. Kato, and Y. Takahashi, An ytterbium quantum gas microscope with narrow-line laser cooling, New J. Phys. 18, 023016 (2016).
  46. A. Jenkins, J. W. Lis, A. Senoo, W. F. McGrew, and A. M. Kaufman, Ytterbium nuclear-spin qubits in an optical tweezer array, Phys. Rev. X 12, 021027 (2022).
  47. S. Ma, A. P. Burgers, G. Liu, J. Wilson, B. Zhang, and J. D. Thompson, Universal gate operations on nuclear spin qubits in an optical tweezer array of 171Yb atoms, Phys. Rev. X 12, 021028 (2022).
  48. M. A. Norcia et al., Midcircuit qubit measurement and rearrangement in a 171Yb atomic array, Phys. Rev. X 13, 041034 (2023).
  49. M. A. Norcia et al., Iterative assembly of 171Yb atom arrays with cavity-enhanced optical lattices, PRX Quantum 5, 030316 (2024).
  50. J. L. Siegel, W. F. McGrew, Y. S. Hassan, C.-C. Chen, K. Beloy, T. Grogan, X. Zhang, and A. D. Ludlow, Excited-band coherent delocalization for improved optical lattice clock performance, Phys. Rev. Lett. 132, 133201 (2024).
  51. J. Ang’ong’a, C. Huang, J. P. Covey, and B. Gadway, Gray molasses cooling of 39K atoms in optical tweezers, Phys. Rev. Res. 4, 013240 (2022).
  52. A. T. Grier, I. Ferrier-Barbut, B. S. Rem, M. Delehaye, L. Khaykovich, F. Chevy, and C. Salomon, Λ-enhanced sub-Doppler cooling of lithium atoms in D1 gray molasses, Phys. Rev. A 87, 063411 (2013).
  53. A. M. Kaufman, B. J. Lester, and C. A. Regal, Cooling a single atom in an optical tweezer to its quantum ground state, Phys. Rev. X 2, 041014 (2012).
  54. J. D. Thompson, T. G. Tiecke, A. S. Zibrov, V. Vuletić, and M. D. Lukin, Coherence and Raman sideband cooling of a single atom in an optical tweezer, Phys. Rev. Lett. 110, 133001 (2013).
  55. S. E. Hamann, D. L. Haycock, G. Klose, P. H. Pax, I. H. Deutsch, and P. S. Jessen, Resolved-sideband Raman cooling to the ground state of an optical lattice, Phys. Rev. Lett. 80, 4149 (1998).
  56. A. J. Kerman, Raman sideband cooling and cold atomic collisions in optical lattices, Ph.D. thesis, Stanford University, California, 2002.
  57. N. Nemitz, T. Ohkubo, M. Takamoto, I. Ushijima, M. Das, N. Ohmae, and H. Katori, Frequency ratio of Yb and Sr clocks with 5 ×10−17 uncertainty at 150 seconds averaging time, Nat. Photon. 10, 258 (2016).
  58. T. A. Savard, K. M. O’Hara, and J. E. Thomas, Laser-noise-induced heating in far-off resonance optical traps, Phys. Rev. A 56, R1095 (1997).
  59. N. Poli, Z. W. Barber, N. D. Lemke, C. W. Oates, L. S. Ma, J. E. Stalnaker, T. M. Fortier, S. A. Diddams, L. Hollberg, J. C. Bergquist, A. Brusch, S. Jefferts, T. Heavner, and T. Parker, Frequency evaluation of the doubly forbidden 1S0→3P0 transition in bosonic 174Yb, Phys. Rev. A 77, 050501(R) (2008).
  60. L. Henriet, J. S. Douglas, D. E. Chang, and A. Albrecht, Critical open-system dynamics in a one-dimensional optical-lattice clock, Phys. Rev. A 99, 023802 (2019).
  61. R. Bekenstein, I. Pikovski, H. Pichler, E. Shahmoon, S. F. Yelin, and M. D. Lukin, Quantum metasurfaces with atom arrays, Nat. Phys. 16, 676 (2020).
  62. S. J. Masson, J. P. Covey, S. Will, and A. Asenjo-Garcia, Dicke superradiance in ordered arrays of multilevel atoms, PRX Quantum 5, 010344 (2024).
  63. T. O. Höhn, R. A. Villela, E. Zu, L. Bezzo, R. M. Kroeze, and M. Aidelsburger, Data for: Determining the 3P0 excited-state tune-out wavelength of 174Yb in a triple-magic lattice (2025), Edmond, V2, https://doi.org/10.17617/3.72JC1R.
  64. L. Riegger, N. Darkwah Oppong, M. Höfer, D. R. Fernandes, I. Bloch, and S. Fölling, Localized magnetic moments with tunable spin exchange in a gas of ultracold fermions, Phys. Rev. Lett. 120, 143601 (2018).
  65. D. A. Steck, http://steck.us/teaching Quantum and Atom Optics (2007).
  66. S. G. Porsev, Y. G. Rakhlina, and M. G. Kozlov, Electric-dipole amplitudes, lifetimes, and polarizabilities of the low-lying levels of atomic ytterbium, Phys. Rev. A 60, 2781 (1999).
  67. K. Blagoev, and V. Komarovskii, Lifetimes of levels of neutral and singly ionized lanthanide atoms, At. Data Nucl. Data Tables 56, 1 (1994).
  68. A. V. Taichenachev, V. I. Yudin, C. W. Oates, C. W. Hoyt, Z. W. Barber, and L. Hollberg, Magnetic field-induced spectroscopy of forbidden optical transitions with application to lattice-based optical atomic clocks, Phys. Rev. Lett. 96, 083001 (2006).
  69. B. H. Bransden, and C. J. Joachain, Physics of Atoms and Molecules (Pearson Education, Prentice Hall, New York, 2003).

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