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  • Letter
  • Open Access

Zero-field atomic magnetometer to extract longitudinal magnetic field

Shuying Wang1,2,3, Jixi Lu1,2,4,*, Kaixuan Zhang4, Le Zhao1,2, Yibo Qi1,2, and Jiancheng Fang1,2,4,†

  • 1School of Instrumentation and Optoelectronic Engineering, Beihang University, Beijing 100191, China
  • 2Hefei National Laboratory, Hefei 230088, China
  • 3Shen Yuan Honors College, Beihang University, Beijing 100191, China
  • 4National Institute of Extremely-Weak Magnetic Field Infrastructure, Hangzhou 310051, China

  • *Contact author: lujixi@buaa.edu.cn
  • †Contact author: fangjiancheng@buaa.edu.cn

Phys. Rev. Research 7, L032024 – Published 1 August, 2025

DOI: https://doi.org/10.1103/yjc6-b26g

Abstract

Zero-field atomic ensembles enable the development of ultrahigh-sensitivity magnetometry. However, their intrinsic insensitivity to longitudinal magnetic fields along the pumping direction poses a fundamental limitation, restricting precise weak-field quantification and complex system decoupling. Herein, we propose a novel zero-field weak parametric modulation scheme capable of ultrahigh-sensitivity extraction of longitudinal magnetic fields. Transverse modulation is employed to manifest the electron spin polarization projection induced by the longitudinal fields. Based on the perturbation model established, first-order parametric resonance associated with the longitudinal magnetic field yields significant signal enhancement under low-frequency and weak modulation conditions, while simultaneously suppressing spin-exchange relaxation caused by magnetic field modulation. We experimentally achieved a longitudinal measurement sensitivity of 16fT/Hz1/2, more than an order of magnitude improved over traditional schemes, with a bandwidth of 70 Hz. Benefiting from low spin relaxation, the noise floor of the transverse magnetic field measurement is preserved at 4 fT/Hz1/2. The proposed scheme pushes the boundaries of existing weak magnetic field measurement, providing critical capabilities for state-of-the-art precision experiments including new physical quantity detection.

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References (46)

  1. W. Happer and H. Tang, Spin-exchange shift and narrowing of magnetic resonance lines in optically pumped alkali vapors, Phys. Rev. Lett. 31, 273 (1973).
  2. J. C. Allred, R. N. Lyman, T. W. Kornack, and M. V. Romalis, High-sensitivity atomic magnetometer unaffected by spin-exchange relaxation, Phys. Rev. Lett. 89, 130801 (2002).
  3. I. K. Kominis, T. W. Kornack, J. C. Allred, and M. V. Romalis, A subfemtotesla multichannel atomic magnetometer, Nature (London) 422, 596 (2003).
  4. J. Kitching, Chip-scale atomic devices, Appl. Phys. Rev. 5, 031302 (2018).
  5. M. Jiang, H. Su, A. Garcon, X. Peng, and D. Budker, Search for axion-like dark matter with spin-based amplifiers, Nat. Phys. 17, 1402 (2021).
  6. X. Zhang, J. Hu, and N. Zhao, Stable atomic magnetometer in parity-time symmetry broken phase, Phys. Rev. Lett. 130, 023201 (2023).
  7. T. M. Tierney, N. Holmes, S. Mellor, J. D. López, G. Roberts, R. M. Hill, E. Boto, J. Leggett, V. Shah, M. J. Brookes, R. Bowtell, and G. R. Barnes, Optically pumped magnetometers: From quantum origins to multi-channel magnetoencephalography, NeuroImage 199, 598 (2019).
  8. E. Boto, N. Holmes, J. Leggett, G. Roberts, V. Shah, S. S. Meyer, L. D. Muñoz, K. J. Mullinger, T. M. Tierney, S. Bestmann, G. R. Barnes, R. Bowtell, and M. J. Brookes, Moving magnetoencephalography towards real-world applications with a wearable system, Nature (London) 555, 657 (2018).
  9. M. Rea, E. Boto, N. Holmes, R. Hill, J. Osborne, N. Rhodes, J. Leggett, L. Rier, R. Bowtell, V. Shah, and M. J. Brookes, A 90-channel triaxial magnetoencephalography system using optically pumped magnetometers, Ann. N. Y. Acad. Sci. 1517, 107 (2022).
  10. X. Li, B. Han, K. Zhang, Z. Liu, S. Wang, Y. Yan, and J. Lu, All-optical dual-axis zero-field atomic magnetometer using light-shift modulation, Phys. Rev. Appl. 21, 014023 (2024).
  11. K. Wei, W. Ji, C. Fu, A. Wickenbrock, V. V. Flambaum, J. Fang, and D. Budker, Constraints on exotic spin-velocity-dependent interactions, Nat. Commun. 13, 7387 (2022).
  12. H. B. Dang, A. C. Maloof, and M. V. Romalis, Ultrahigh sensitivity magnetic field and magnetization measurements with an atomic magnetometer, Appl. Phys. Lett. 97, 151110 (2010).
  13. J. A. Tarduno, R. D. Cottrell, R. K. Bono, N. Rayner, W. J. Davis, T. Zhou, F. Nimmo, A. Hofmann, J. Jodder, M. Ibañez-Mejia, M. K. Watkeys, H. Oda, and G. Mitra, Hadaean to Palaeoarchaean stagnant-lid tectonics revealed by zircon magnetism, Nature (London) 618, 531 (2023).
  14. W. Franzen and A. G. Emslie, Atomic orientation by optical pumping, Phys. Rev. 108, 1453 (1957).
  15. W. Happer, Optical pumping, Rev. Mod. Phys. 44, 169 (1972).
  16. H. G. Dehmelt, Modulation of a light beam by precessing absorbing atoms, Phys. Rev. 105, 1924 (1957).
  17. D. Budker and M. V. Romalis, Optical magnetometry, Nature Phys 3, 227 (2007).
  18. S.-Q. Liu, Q.-Q. Yu, H. Zhou, and D. Sheng, Sensitive and stable atomic vector magnetometer to detect weak fields using two orthogonal multipass cavities, Phys. Rev. Appl. 19, 044062 (2023).
  19. E. Boto, V. Shah, R. M. Hill, N. Rhodes, J. Osborne, C. Doyle, N. Holmes, M. Rea, J. Leggett, R. Bowtell, and M. J. Brookes, Triaxial detection of the neuromagnetic field using optically-pumped magnetometry: feasibility and application in children, NeuroImage 252, 119027 (2022).
  20. Y. Yan, J. Lu, S. Zhang, F. Lu, K. Yin, K. Wang, B. Zhou, and G. Liu, Three-axis closed-loop optically pumped magnetometer operated in the SERF regime, Opt. Express 30, 18300 (2022).
  21. W. Happer and W. A. Van Wijngaarden, An optical pumping primer, Hyperfine Interact. 38, 435 (1987).
  22. T. W. Kornack and M. V. Romalis, Dynamics of two overlapping spin ensembles interacting by spin exchange, Phys. Rev. Lett. 89, 253002 (2002).
  23. R. Li, W. Quan, W. Fan, L. Xing, and J. Fang, Influence of magnetic fields on the bias stability of atomic gyroscope operated in spin-exchange relaxation-free regime, Sens. Actuators, A 266, 130 (2017).
  24. Y. Chen, Y. Lu, and J. Fang, Spin exchange collision mixing of the K and Rb ac Stark shifts, Phys. Rev. A 94, 052705 (2016).
  25. E. Klinger, T. Liu, M. Padniuk, M. Engler, T. Kornack, S. Pustelny, D. F. Jackson Kimball, D. Budker, and A. Wickenbrock, Optimization of nuclear polarization in an alkali-noble gas comagnetometer, Phys. Rev. Appl. 19, 044092 (2023).
  26. W. Xiao, Y. Wu, X. Zhang, Y. Feng, C. Sun, T. Wu, J. Chen, X. Peng, and H. Guo, Single-beam three-axis optically pumped magnetometers with sub-100 femtotesla sensitivity, Appl. Phys. Express 14, 066002 (2021).
  27. J. Zhang, T. Chen, C. Wei, Z. Ou, H. Yue, and Y. Liu, Single-beam three-axis SERF atomic magnetometer based on coordinate system rotation, Opt. Express 32, 17165 (2024).
  28. T. W. Kornack, R. K. Ghosh, and M. V. Romalis, Nuclear spin gyroscope based on an atomic co-magnetometer, Phys. Rev. Lett. 95, 230801 (2005).
  29. M. Xu, M. Jiang, Y. Wang, H. Su, Y. Huang, and X. Peng, Cooperative spin amplifier for enhanced quantum sensing, Phys. Rev. Lett. 133, 133202 (2024).
  30. L. Jiang, W. Quan, F. Liu, W. Fan, L. Xing, L. Duan, W. Liu, and J. Fang, Closed-loop control of compensation point in the K-Rb-Ne21 comagnetometer, Phys. Rev. Appl. 12, 024017 (2019).
  31. F. Lu, J. Lu, B. Li, Y. Yan, S. Zhang, K. Yin, M. Ye, and B. Han, Triaxial vector operation in near-zero field of atomic magnetometer with femtotesla sensitivity, IEEE Trans. Instrum. Meas. 71, 1501210 (2022).
  32. J. Osborne, J. Orton, O. Alem, and V. Shah, Fully integrated, standalone zero field optically pumped magnetometer for biomagnetism, in Steep Dispersion Engineering and Opto-Atomic Precision Metrology XI, Vol. 10548 (SPIE, San Francisco, 2018), pp. 89–95.
  33. L. Li, J. Tang, B. Zhao, L. Cao, Y. Zhang, and Y. Zhai, Analysis and suppression of the three-axis crosstalk effect in the modulated SERF atomic magnetometer, Measurement 218, 113161 (2023).
  34. Y. Suo, X. Song, L. Jiang, L. Jia, T. Long, and Z. Wu, Suppression of modulation-magnetic-fields crosstalk for single-beam optically-pumped magnetometers, Measurement 217, 113059 (2023).
  35. V. Shah and M. V. Romalis, Spin-exchange relaxation-free magnetometry using elliptically polarized light, Phys. Rev. A 80, 013416 (2009).
  36. J. Lu, Z. Qian, J. Fang, and W. Quan, Effects of AC magnetic field on spin-exchange relaxation of atomic magnetometer, Appl. Phys. B 122, 59 (2016).
  37. J. Dupont-Roc, Détermination par des méthodes optiques des trois composantes d'un champ magnétique très faible, Rev. Phys. Appl. (Paris) 5, 853 (1970).
  38. L. Li, J. Tang, B. Zhao, L. Cao, B. Zhou, and Y. Zhai, Single-beam triaxial spin-exchange relaxation-free atomic magnetometer utilizing transverse modulation fields, J. Phys. D: Appl. Phys. 55, 505001 (2022).
  39. S. J. Seltzer and M. V. Romalis, Unshielded three-axis vector operation of a spin-exchange-relaxation-free atomic magnetometer, Appl. Phys. Lett. 85, 4804 (2004).
  40. H. Huang, H. Dong, L. Chen, and Y. Gao, Single-beam three-axis atomic magnetometer, Appl. Phys. Lett. 109, 062404 (2016).
  41. J. Dupont-Roc, Étude théorique de diverses résonances observables en champ nul sur des atomes ≪ habillés par des photons de radiofréquence, J. Phys. France 32, 135 (1971).
  42. Z. Li, R. T. Wakai, and T. G. Walker, Parametric modulation of an atomic magnetometer, Appl. Phys. Lett. 89, 134105 (2006).
  43. J. Wang, W. Fan, K. Yin, Y. Yan, B. Zhou, and X. Song, Combined effect of pump-light intensity and modulation field on the performance of optically pumped magnetometers under zero-field parametric modulation, Phys. Rev. A 101, 053427 (2020).
  44. J. M. Brown, S. J. Smullin, T. W. Kornack, and M. V. Romalis, New limit on Lorentz and CPT-violating neutron spin interactions, Phys. Rev. Lett. 105, 151604 (2010).
  45. Y. Wang, Y. Huang, C. Guo, M. Jiang, X. Kang, H. Su, Y. Qin, W. Ji, D. Hu, X. Peng, and D. Budker, Search for exotic parity-violation interactions with quantum spin amplifiers, Sci. Adv. 9, eade0353 (2023).
  46. S. Wang, “Available Data associated with Manuscript LZ17931WR” [Data set], Zenodo (2025), https://doi.org/10.5281/zenodo.15661690.

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