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Acoustically driven magnons in CrSBr bilayers

Anton Shubnic1,*, Igor Chestnov1, Igor Lobanov1, Valery Uzdin1, Ivan Iorsh1,2,†, and Ivan A. Shelykh3,‡

  • *Contact author: anton.shubnic@metalab.ifmo.ru
  • †Contact author: ivan.iorsh@queensu.ca
  • ‡Contact author: shelykh@hi.is

Phys. Rev. Research 8, 043135 – Published 6 November, 2026

DOI: https://doi.org/10.1103/xdkq-h9km

Abstract

We study the coupling between spin excitations and acoustic waves in bilayers of CrSBr, an ambiently stable two-dimensional (2D) magnetic material. We demonstrate that a strong dependence of interlayer exchange coupling on strain makes possible the resonant generation of magnons by an acoustic wave. It is shown that the parameters of the generation, in particular, the resonant frequency, can be tuned by an external magnetic field, which makes CrSBr a promising platform for spintronics applications.

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References (43)

  1. K. S. Novoselov, A. K. Geim, S. V. Morozov, D. Jiang, Y. Zhang, S. V. Dubonos, I. V. Grigorieva, and A. A. Firsov, Electric field effect in atomically thin carbon films, Science 306, 666 (2004).
  2. Y. Luo, J. Zhao, A. Fieramosca, Q. Guo, H. Kang, X. Liu, T. C. H. Liew, D. Sanvitto, Z. An, S. Ghosh, Z. Wang, H. Xu, and Q. Xiong, Strong light-matter coupling in van der Waals materials, Light: Sci. Appl. 13, 203 (2024).
  3. W. Tang, H. Liu, Z. Li, A. Pan, and Y.-J. Zeng, Spin-orbit torque in van der Waals-layered materials and heterostructures, Adv. Sci. 8, 2100847 (2021).
  4. B. Huang, G. Clark, E. Navarro-Moratalla, D. R. Klein, R. Cheng, K. L. Seyler, D. Zhong, E. Schmidgall, M. A. McGuire, D. H. Cobden, W. Yao, D. Xiao, P. Jarillo-Herrero, and X. Xu, Layer-dependent ferromagnetism in a van der Waals crystal down to the monolayer limit, Nature (London) 546, 270 (2017).
  5. H. H. Kim, B. Yang, T. Patel, F. Sfigakis, C. Li, S. Tian, H. Lei, and A. W. Tsen, One million percent tunnel magnetoresistance in a magnetic van der Waals heterostructure, Nano Lett. 18, 4885 (2018).
  6. S. Jiang, L. Li, Z. Wang, K. F. Mak, and J. Shan, Controlling magnetism in 2D CrI3 by electrostatic doping, Nat. Nanotechnol. 13, 549 (2018).
  7. Z. Sun, Y. Yi, T. Song, G. Clark, B. Huang, Y. Shan, S. Wu, D. Huang, C. Gao, Z. Chen, M. McGuire, T. Cao, D. Xiao, W.-T. Liu, W. Yao, X. Xu, and S. Wu, Giant nonreciprocal second-harmonic generation from antiferromagnetic bilayer CrI3, Nature (London) 572, 497 (2019).
  8. Y. Zhumagulov, S. Chiavazzo, I. A. Shelykh, and O. Kyriienko, Robust polaritons in magnetic monolayers of CrI3, Phys. Rev. B 108, L161402 (2023).
  9. B. Huang, M. A. McGuire, A. F. May, D. Xiao, P. Jarillo-Herrero, and X. Xu, Emergent phenomena and proximity effects in two-dimensional magnets and heterostructures, Nat. Mater. 19, 1276 (2020).
  10. N. P. Wilson, K. Lee, J. Cenker, K. Xie, A. H. Dismukes, E. J. Telford, J. Fonseca, S. Sivakumar, C. Dean, T. Cao, X. Roy, X. Xu, and X. Zhu, Interlayer electronic coupling on demand in a 2D magnetic semiconductor, Nat. Mater. 20, 1657 (2021).
  11. F. Wu, I. Gutiérrez-Lezama, S. A. López-Paz, M. Gibertini, K. Watanabe, T. Taniguchi, F. O. von Rohr, N. Ubrig, and A. F. Morpurgo, Quasi-1D electronic transport in a 2D magnetic semiconductor, Adv. Mater. 34, 2109759 (2022).
  12. C. Boix-Constant, S. Mañas-Valero, A. M. Ruiz, A. Rybakov, K. A. Konieczny, S. Pillet, J. J. Baldoví, and E. Coronado, Probing the spin dimensionality in single-layer CrSBr van der Waals heterostructures by magneto-transport measurements, Adv. Mater. 34, 2204940 (2022).
  13. K. Lee, A. H. Dismukes, E. J. Telford, R. A. Wiscons, J. Wang, X. Xu, C. Nuckolls, C. R. Dean, X. Roy, and X. Zhu, Magnetic order and symmetry in the 2D semiconductor CrSBr, Nano Lett. 21, 3511 (2021).
  14. E. J. Telford, A. H. Dismukes, K. Lee, M. Cheng, A. Wieteska, A. K. Bartholomew, Y.-S. Chen, X. Xu, A. N. Pasupathy, X. Zhu, C. R. Dean, and X. Roy, Layered antiferromagnetism induces large negative magnetoresistance in the van der Waals semiconductor CrSBr, Adv. Mater. 32, 2003240 (2020).
  15. Y. Wang, S.-S. Wang, Y. Lu, J. Jiang, and S. A. Yang, Strain-induced isostructural and magnetic phase transitions in monolayer MoN2, Nano Lett. 16, 4576 (2016).
  16. K. Bagani, A. Vervelaki, D. Jetter, A. Devarakonda, M. A. Tschudin, B. Gross, D. G. Chica, D. A. Broadway, C. R. Dean, X. Roy, P. Maletinsky, and M. Poggio, Imaging strain-controlled magnetic reversal in thin CrSBr, Nano Lett. 24, 13068 (2024).
  17. E. Uykur, A. A. Tsirlin, F. Long, M. Wenzel, M. Dressel, K. Mosina, Z. Sofer, M. Helm, and S. Zhou, Phonon and magnon dynamics across the antiferromagnetic transition in the two-dimensional layered van der Waals material CrSBr, Phys. Rev. B 111, 174434 (2025).
  18. X. Xu, X. Wang, P. Chang, X. Chen, L. Guan, and J. Tao, Strong spin-phonon coupling in two-dimensional magnetic semiconductor CrSBr, J. Phys. Chem. C 126, 10574 (2022).
  19. F. Fei, Y. Mao, W. Fang, W. Liu, J. P. Rollins, A. L. N. Kondusamy, B. Lv, Y. Ping, Y. Wang, and J. Xiao, Spin-mechanical coupling in 2D antiferromagnet CrSBr, Nano Lett. 24, 10467 (2024).
  20. J. Cenker, S. Sivakumar, K. Xie, A. Miller, P. Thijssen, Z. Liu, A. Dismukes, J. Fonseca, E. Anderson, X. Zhu, X. Roy, D. Xiao, J.-H. Chu, T. Cao, and X. Xu, Reversible strain-induced magnetic phase transition in a van der Waals magnet, Nat. Nanotechnol. 17, 256 (2022).
  21. N. Liu, C. Wang, Y. Zhang, F. Pang, Z. Cheng, Y. Zhang, and W. Ji, Intralayer strain tuned interlayer magnetism in bilayer CrSBr, Phys. Rev. B 109, 214422 (2024).
  22. C. Kittel, Physical theory of ferromagnetic domains, Rev. Mod. Phys. 21, 541 (1949).
  23. C. Kittel, Interaction of spin waves and ultrasonic waves in ferromagnetic crystals, Phys. Rev. 110, 836 (1958).
  24. Y. J. Bae, J. Wang, A. Scheie, J. Xu, D. G. Chica, G. M. Diederich, J. Cenker, M. E. Ziebel, Y. Bai, H. Ren, C. R. Dean, M. Delor, X. Xu, X. Roy, A. D. Kent, and X. Zhu, Exciton-coupled coherent magnons in a 2D semiconductor, Nature (London) 609, 282 (2022).
  25. J. Chen, K. Yamamoto, C. Kang, R. Yuan, K. Yu, C. Hu, J. Hu, L. Sheng, J. Wang, S. Liu, D. Yu, J.-P. Ansermet, Y.-J. Zeng, S. Maekawa, and H. Yu, Surface magnon propagation in a van der Waals antiferromagnet, Phys. Rev. Lett. 136, 056702 (2026).
  26. Y. J. Bae, T. Handa, Y. Dai, J. Wang, H. Liu, A. Scheie, D. G. Chica, M. E. Ziebel, A. D. Kent, X. Xu, K. Shen, X. Roy, and X. Zhu, Transient magnetoelastic coupling in CrSBr, Phys. Rev. B 109, 104401 (2024).
  27. X. Shen, J. Cao, B. Cong, B. Zou, W. Liang, Z. Peng, J. Zhao, and A. Kavokin, Electron-phonon coupling probed by ultrafast coherent phonon spectroscopy in bulk van der Waals CrSBr, Phys. Rev. B 113, 125406 (2026).
  28. X. Shen, B. Cong, J. Cao, J. Huang, W. Liang, J. Zhao, and B. Zou, Orthogonal magnon-phonon coupling enables information encoding in bulk CrSBr, J. Phys. Chem. Lett. 16, 12625 (2025).
  29. K. Yang, G. Wang, L. Liu, D. Lu, and H. Wu, Triaxial magnetic anisotropy in the two-dimensional ferromagnetic semiconductor CrSBr, Phys. Rev. B 104, 144416 (2021).
  30. See Supplemental Material at http://link.aps.org/supplemental/10.1103/xdkq-h9km for the details of the parametrization of the continuous model, the derivation of the LLG equations, and the details of the DFT calculations, which also includes Refs. [37, 38, 39, 40, 41, 42, 43].
  31. T. M. J. Cham, D. G. Chica, X. Huang, K. Watanabe, T. Taniguchi, X. Roy, Y. K. Luo, and D. C. Ralph, Spin-filter tunneling detection of antiferromagnetic resonance with electrically tunable damping, Science 389, 479 (2025).
  32. O. Göser, W. Paul, and H. Kahle, Magnetic properties of CrSBr, J. Magn. Magn. Mater. 92, 129 (1990).
  33. N. Stetzuhn, A. M. Kumar, S. Kovalchuk, D. Yagodkin, L. Simon, S. Mañas-Valero, E. Coronado, T. Taniguchi, K. Watanabe, D. Gill, S. Sharma, P. W. Brouwer, C. von Korff Schmising, S. Eisebitt, and K. I. Bolotin, Tunable magnons in a dual-gated 2D antiferromagnet, Nat. Commun. 17, 5262 (2026).
  34. H. Li, Y. Yang, Z. Xia, Y. Wang, J. Wei, J. He, and R. Wang, Stacking effects on magnetic, vibrational, and optical properties of CrSBr bilayers, Phys. Rev. B 111, 125411 (2025).
  35. P. S. Shaban, I. S. Lobanov, V. M. Uzdin, and I. V. Iorsh, Skyrmion dynamics in moiré magnets, Phys. Rev. B 108, 174440 (2023).
  36. G. M. Diederich, J. Cenker, Y. Ren, J. Fonseca, D. G. Chica, Y. J. Bae, X. Zhu, X. Roy, T. Cao, D. Xiao, and X. Xu, Tunable interaction between excitons and hybridized magnons in a layered semiconductor, Nat. Nanotechnol. 18, 23 (2023).
  37. J. J. Mortensen, A. H. Larsen, M. Kuisma, A. V. Ivanov, A. Taghizadeh, A. Peterson, A. Haldar, A. O. Dohn, C. Schäfer, E. Jónsson, et al., GPAW: An open Python package for electronic structure calculations, J. Chem. Phys. 160, 092503 (2024).
  38. J. J. Mortensen, L. B. Hansen, and K. W. Jacobsen, Real-space grid implementation of the projector augmented wave method, Phys. Rev. B 71, 035109 (2005).
  39. J. Enkovaara, C. Rostgaard, J. J. Mortensen, J. Chen, M. Dułak, L. Ferrighi, J. Gavnholt, C. Glinsvad, V. Haikola, H. A. Hansen, H. H. Kristoffersen, M. Kuisma, A. H. Larsen, L. Lehtovaara, M. Ljungberg, O. Lopez-Acevedo, P. G. Moses, J. Ojanen, T. Olsen, and V. Petzold, Electronic structure calculations with GPAW: A real-space implementation of the projector augmented-wave method, J. Phys.: Condens. Matter 22, 253202 (2010).
  40. J. P. Perdew, K. Burke, and M. Ernzerhof, Generalized gradient approximation made simple, Phys. Rev. Lett. 77, 3865 (1996).
  41. P. T. Jochym, Elastic, Release v5. 1.0-14-g6596fd4, 2018, https://wolf.ifj.edu.pl/~jochym/Elastic.pdf.
  42. P. T. Jochym, K. Parlinski, and M. Sternik, TiC lattice dynamics from ab initio calculations, Eur. Phys. J. B 10, 9 (1999).
  43. P. T. Jochym and K. Parlinski, Ab initio lattice dynamics and elastic constants of ZrC, Eur. Phys. J. B 15, 265 (2000).

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