- Letter
- Open Access
Observation of period doubling and higher multiplicities in a driven single-spin system
Phys. Rev. Research 8, L032011 – Published 21 July, 2026
DOI: https://doi.org/10.1103/wj1t-vk39
Abstract
One of the prime features of quantum systems strongly driven by external time-periodic fields is the subharmonic response with integer multiples of the drive period due to long-lived interference. Here, we demonstrate experimentally, based on a careful theoretical analysis, period doubling and higher multiplicities () for one of the most fundamental systems, namely, an individual spin . Nitrogen-vacancy centers in diamond support sufficiently stable coherent dynamics owing to long coherence times and allow for optical addressability of their spin states. This allows to monitor coherent period -tupling oscillations over a broad set of driving parameters in the vicinity of the ideal manifolds. In this domain, superimposed low-frequency modulations serve as unique proxy for the approach toward period -tupling.
Physics Subject Headings (PhySH)
Article Text
Supplemental Material
References (29)
- S. Kohler, J. Lehmann, and P. Hänggi, Driven quantum transport on the nanoscale, Phys. Rep. 406, 379 (2005).
- M. Grifoni and P. Hänggi, Driven quantum tunneling, Phys. Rep. 304, 229 (1998).
- C. Deng, J.-L. Orgiazzi, F. Shen, S. Ashhab, and A. Lupascu, Observation of Floquet states in a strongly driven artificial atom, Phys. Rev. Lett. 115, 133601 (2015).
- F. Grossmann, T. Dittrich, P. Jung, and P. Hänggi, Coherent destruction of tunneling, Phys. Rev. Lett. 67, 516 (1991).
- Q. Miao and Y. Zeng, Coherent destruction of tunneling in two-level system driven across avoided crossing via photon statistics, Sci. Rep. 6, 28959 (2016).
- Y. Kayanuma, Role of phase coherence in the transition dynamics of a periodically driven two-level system, Phys. Rev. A 50, 843 (1994).
- M. Sillanpää, T. Lehtinen, A. Paila, Y. Makhlin, and P. Hakonen, Continuous-time monitoring of Landau-Zener interference in a Cooper pair box, Phys. Rev. Lett. 96, 187002 (2006).
- L. Magazzù, P. Forn-Díaz, R. Belyansky, J.-L. Orgiazzi, M. Yurtalan, M. Otto, L. A., C. Wilson, and M. Grifoni, Probing the strongly driven spin-boson model in a superconducting quantum circuit, Nat. Commun. 9, 1403 (2018).
- J. Romhányi, G. Burkard, and A. Pályi, Subharmonic transitions and Bloch-Siegert shift in electrically driven spin resonance, Phys. Rev. B 92, 054422 (2015).
- K. R. K. Rao and D. Suter, Nonlinear dynamics of a two-level system of a single spin driven beyond the rotating-wave approximation, Phys. Rev. A 95, 053804 (2017).
- M. I. Dykman, Coherent multiple-period states of periodically modulated qubits, Phys. Rev. A 100, 042101 (2019).
- F. Jelezko and J. Wrachtrup, Single defect centres in diamond: A review, Phys. Status Solidi (a) 203, 3207 (2006).
- J. M. Taylor, P. Cappellaro, L. Childress, L. Jiang, D. Budker, P. R. Hemmer, A. Yacoby, R. Walsworth, and M. D. Lukin, High-sensitivity diamond magnetometer with nanoscale resolution, Nat. Phys. 4, 810 (2008).
- F. Dolde, H. Fedder, M. W. Doherty, T. Nöbauer, F. Rempp, G. Balasubramanian, T. Wolf, F. Reinhard, L. C. Hollenberg, F. Jelezko, et al., Electric-field sensing using single diamond spins, Nat. Phys. 7, 459 (2011).
- V. Gramich, S. Gasparinetti, P. Solinas, and J. Ankerhold, Lamb-shift enhancement and detection in strongly driven superconducting circuits, Phys. Rev. Lett. 113, 027001 (2014).
- L. Guo, Phase Space Crystals (Institute of Physics Publishing, 2021).
- See Supplemental Material at http://link.aps.org/supplemental/10.1103/wj1t-vk39 for the theoretical framework, extended NV-center modeling, numerical simulations, data-analysis and fitting procedures, additional period--tupling data for , and experimental details, which includes Ref. [29].
- J. P. Tetienne, L. Rondin, P. Spinicelli, M. Chipaux, T. Debuisschert, J.-F. Roch, and V. Jacques, Magnetic-field-dependent photodynamics of single NV defects in diamond: An application to qualitative all-optical magnetic imaging, New J. Phys. 14, 103033 (2012).
- V. Jacques, P. Neumann, J. Beck, M. Markham, D. Twitchen, J. Meijer, F. Kaiser, G. Balasubramanian, F. Jelezko, and J. Wrachtrup, Dynamic polarization of single nuclear spins by optical pumping of nitrogen-vacancy color centers in diamond at room temperature, Phys. Rev. Lett. 102, 057403 (2009).
- J. M. Binder, A. Stark, N. Tomek, J. Scheuer, F. Frank, K. D. Jahnke, C. Müller, S. Schmitt, M. H. Metsch, T. Unden, et al., Qudi: A modular Python suite for experiment control and data processing, SoftwareX 6, 85 (2017).
- D. A. Broadway, J. D. A. Wood, L. T. Hall, A. Stacey, M. Markham, D. A. Simpson, J.-P. Tetienne, and L. C. L. Hollenberg, Anticrossing spin dynamics of diamond nitrogen-vacancy centers and all-optical low-frequency magnetometry, Phys. Rev. Appl. 6, 064001 (2016).
- L. Robledo, H. Bernien, T. Van Der Sar, and R. Hanson, Spin dynamics in the optical cycle of single nitrogen-vacancy centres in diamond, New J. Phys. 13, 025013 (2011).
- S. Pezzagna and J. Meijer, Quantum computer based on color centers in diamond, Appl. Phys. Rev. 8, 011308 (2021).
- J. Zhang, P. W. Hess, A. Kyprianidis, P. Becker, A. Lee, J. Smith, G. Pagano, I.-D. Potirniche, A. C. Potter, A. Vishwanath, N. Y. Yao, and C. Monroe, Observation of a discrete time crystal., Nature (London) 543, 217 (2017).
- K. Sacha and J. Zakrzewsk, Time crystals: A review, Rep. Prog. Phys. 81, 016401 (2018).
- J. Smits, L. Liao, H. T. C. Stoof, and P. van der Straten, Observation of a space-time crystal in a superfluid quantum gas, Phys. Rev. Lett. 121, 185301 (2018).
- S. Choi, J. Choi, R. Landig, G. Kucsko, H. Zhou, J. Isoya, F. Jelezko, S. Onoda, H. Sumiya, V. Khemani, C. von Keyserlingk, N. Y. Yao, E. Demler, and M. D. Lukin, Observation of discrete time-crystalline order in a disordered dipolar many-body system, Nature (London) 543, 221 (2017).
- L. J. Il Moon, P. M. Schindler, R. J. Smith, E. Druga, Z.-R. Zhang, M. Bukov, and A. Ajoy, Discrete time crystal sensing, Nat. Phys. 22, 367 (2026).
- S. Felton, A. M. Edmonds, M. E. Newton, P. M. Martineau, D. Fisher, D. J. Twitchen, and J. M. Baker, Hyperfine interaction in the ground state of the negatively charged nitrogen vacancy center in diamond, Phys. Rev. B 79, 075203 (2009).