Reuse & Permissions

It is not necessary to obtain permission to reuse this article or its components as it is available under the terms of the Creative Commons Attribution 4.0 International license. This license permits unrestricted use, distribution, and reproduction in any medium, provided attribution to the author(s) and the published article's title, journal citation, and DOI are maintained. Please note that some figures may have been included with permission from other third parties. It is your responsibility to obtain the proper permission from the rights holder directly for these figures.

Export citation

Export citation

Choose format for download:

Download Citation
  • Open Access

Perfect crystal neutron loop cavity

Owen Lailey1,2,*, Dusan Sarenac3, David G. Cory1,4, Michael G. Huber5, and Dmitry A. Pushin1,2,†

  • *Contact author: oalailey@uwaterloo.ca
  • †Contact author: dmitry.pushin@uwaterloo.ca

Phys. Rev. Research 8, 043124 – Published 3 November, 2026

DOI: https://doi.org/10.1103/vqvb-4vgw

Abstract

Coherent control of neutrons via Bragg diffraction forms the foundation of perfect crystal neutron interferometry, facilitating both fundamental tests of quantum mechanics and applications in quantum information science. In cavity geometries, perfect crystals enable neutron confinement and have been employed in precision measurements of spin-orbit interactions and for neutron electric dipole moment (nEDM) searches. However, in these conventional configurations, neutrons undergo a single pass through the crystal geometry, placing a physical constraint on both crystal and in-flight interaction times and measurement sensitivity. In this work, we introduce a neutron loop cavity that coherently recirculates neutrons through repeated Bragg reflections between perfect silicon crystal blades. This structure is predicted to achieve a neutron unitary survival probability of ∼64% for 10 000 Bragg reflections, corresponding to confinement times on the order of seconds. We propose a Schwinger interaction measurement that achieves a π spin rotation in 800 Bragg reflections, representing more than a tenfold improvement in sensitivity over recent measurements. Further applications include nEDM searches targeting the 10−27 ecm scale, as well as experimental tests of neutron parity violation, the neutron lifetime, and the quantum Zeno effect with neutrons.

View figure in article

Physics Subject Headings (PhySH)

Article Text

References (72)

  1. H. Rauch and S. A. Werner, Neutron Interferometry: Lessons in Experimental Quantum Mechanics, Wave-Particle Duality, and Entanglement, 2nd ed. (Oxford University Press, Oxford, 2015), Vol. 12.
  2. H. Rauch, A. Zeilinger, G. Badurek, A. Wilfing, W. Bauspiess, and U. Bonse, Verification of coherent spinor rotation of fermions, Phys. Lett. A 54, 425 (1975).
  3. R. Colella, A. W. Overhauser, and S. A. Werner, Observation of gravitationally induced quantum interference, Phys. Rev. Lett. 34, 1472 (1975).
  4. D. A. Pushin, M. G. Huber, M. Arif, and D. G. Cory, Experimental realization of decoherence-free subspace in neutron interferometry, Phys. Rev. Lett. 107, 150401 (2011).
  5. K. Li, M. Arif, D. G. Cory, R. Haun, B. Heacock, M. G. Huber, J. Nsofini, D. A. Pushin, P. Saggu, D. Sarenac, et al., Neutron limit on the strongly-coupled chameleon field, Phys. Rev. D 93, 062001 (2016).
  6. B. Heacock, T. Fujiie, R. W. Haun, A. Henins, K. Hirota, T. Hosobata, M. G. Huber, M. Kitaguchi, D. A. Pushin, H. Shimizu, M. Takeda, R. Valdillez, Y. Yamagata, and A. R. Young, Pendellösung interferometry probes the neutron charge radius, lattice dynamics, and fifth forces, Science 373, 1239 (2021).
  7. A. Danner, H. Lemmel, R. Wagner, S. Sponar, and Y. Hasegawa, Neutron interferometer experiments studying fundamental features of quantum mechanics, Atoms 11, 98 (2023).
  8. C. W. Clark, R. Barankov, M. G. Huber, M. Arif, D. G. Cory, and D. A. Pushin, Controlling neutron orbital angular momentum, Nature (London) 525, 504 (2015).
  9. D. Sarenac, M. G. Huber, B. Heacock, M. Arif, C. W. Clark, D. G. Cory, C. B. Shahi, and D. A. Pushin, Holography with a neutron interferometer, Opt. Express 24, 22528 (2016).
  10. N. Geerits, H. Lemmel, A.-S. Berger, and S. Sponar, Phase vortex lattices in neutron interferometry, Commun. Phys. 6, 209 (2023).
  11. M. Schuster, H. Rauch, E. Seidl, E. Jericha, and C. Carlile, Test of a perfect crystal neutron storage device, Phys. Lett. A 144, 297 (1990).
  12. M. Schuster, E. Jericha, C. Carlile, and H. Rauch, A cold neutron storage device and a neutron resonator, Phys. B: Condens. Matter 180–181, 997 (1992).
  13. E. Jericha, C. Carlile, and H. Rauch, Performance of an improved perfect crystal neutron storage cavity, Nucl. Instrum. Methods Phys. Res. Sect. A 379, 330 (1996).
  14. E. Jericha, C. Carlile, M. Jäkel, and H. Rauch, Cold neutron storage by perfect crystals, Phys. B: Condens. Matter 234–236, 1066 (1997).
  15. M. R. Jaekel, C. J. Carlile, E. Jericha, D. E. Schwab, and H. Rauch, New measurements with a perfect crystal cavity for neutrons, in EUV, X-Ray, and Neutron Optics and Sources, Proceedings of SPIE Vol. 3767 (SPIE, Bellingham, WA, 1999), pp. 353–359.
  16. M. Jaekel, E. Jericha, and H. Rauch, New developments in cold neutron storage with perfect crystals, Nucl. Instrum. Methods Phys. Res. Sect. A 539, 335 (2005).
  17. T. R. Gentile, M. G. Huber, D. D. Koetke, M. Peshkin, M. Arif, T. Dombeck, D. S. Hussey, D. L. Jacobson, P. Nord, D. A. Pushin, and R. Smither, Direct observation of neutron spin rotation in Bragg scattering due to the spin-orbit interaction in silicon, Phys. Rev. C 100, 034005 (2019).
  18. T. Dombeck, R. Ringo, D. D. Koetke, H. Kaiser, K. Schoen, S. A. Werner, and D. Dombeck, Measurement of the neutron reflectivity for Bragg reflections off a perfect silicon crystal, Phys. Rev. A 64, 053607 (2001).
  19. M. Huber, B. Heacock, I. Taminiau, D. G. Cory, D. Sarenac, R. Valdillez, and D. A. Pushin, Achieving a near-ideal silicon crystal neutron interferometer using submicrometer fabrication techniques, Phys. Rev. Res. 6, 043079 (2024).
  20. H. Lemmel, M. Jentschel, H. Abele, F. Lafont, B. Guerard, C. P. Sasso, G. Mana, and E. Massa, Neutron interference from a split-crystal interferometer, J. Appl. Crystallogr. 55, 870 (2022).
  21. J. Nsofini, K. Ghofrani, D. Sarenac, D. G. Cory, and D. A. Pushin, Quantum-information approach to dynamical diffraction theory, Phys. Rev. A 94, 6 (2016).
  22. J. Nsofini, D. Sarenac, K. Ghofrani, M. G. Huber, M. Arif, D. G. Cory, and D. A. Pushin, Noise refocusing in a five-blade neutron interferometer, J. Appl. Phys. 122, 054501 (2017).
  23. J. Nsofini, D. Sarenac, D. G. Cory, and D. A. Pushin, Coherence optimization in neutron interferometry through defocusing, Phys. Rev. A 99, 043614 (2019).
  24. O. Nahman-Lévesque, D. Sarenac, D. G. Cory, B. Heacock, M. G. Huber, and D. A. Pushin, Generalizing the quantum information model for dynamic diffraction, Phys. Rev. A 105, 022403 (2022).
  25. O. Nahman-Lévesque, D. Sarenac, O. Lailey, D. G. Cory, M. G. Huber, and D. A. Pushin, Quantum information approach to the implementation of a neutron cavity, New J. Phys. 25, 073016 (2023).
  26. W. Bond, M. Duguay, and P. Rentzepis, Proposed resonator for an x-ray laser, Appl. Phys. Lett. 10, 216 (1967).
  27. R. D. Deslattes, X-ray monochromators and resonators from single crystals, Appl. Phys. Lett. 12, 133 (1968).
  28. R. Cotterill, A universal planar x-ray resonator, Appl. Phys. Lett. 12, 403 (1968).
  29. P. Liu, P. Pradhan, X. Shi, D. Shu, K. Kauchha, Z. Qiao, K. Tamasaku, T. Osaka, D. Zhu, T. Sato, J. MacArthur, X. Huang, L. Assoufid, M. White, K.-J. Kim, and Y. Shvyd’ko, X-ray optics for the cavity-based x-ray free-electron laser, J. Synchrotron Radiat. 31, 751 (2024).
  30. U. Bonse and E. te Kaat, A two-crystal x-ray interferometer, Z. Phys. 214, 16 (1968).
  31. M. D. Le, T. Guidi, R. Bewley, J. R. Stewart, E. M. Schooneveld, D. Raspino, D. E. Pooley, J. Boxall, K. F. Gascoyne, N. J. Rhodes, S. R. Moorby, D. J. Templeman, L. C. Afford, S. P. Waller, D. Zacek, and R. C. R. Shaw, Upgrade of the MARI spectrometer at ISIS, Nucl. Instrum. Methods Phys. Res. Sect. A 1056, 168646 (2023).
  32. National Institute of Standards and Technology, NCNR guide upgrade, NIST Center for Neutron Research, 2026, https://www.nist.gov/ncnr/facilities-upgrades-during-unplanned-outage/ncnr-guide-upgrade.
  33. H. Abele, D. Dubbers, H. Häse, M. Klein, A. Knöpfler, M. Kreuz, T. Lauer, B. Märkisch, D. Mund, V. Nesvizhevsky, A. Petoukhov, C. Schmidt, M. Schumann, and T. Soldner, Characterization of a ballistic supermirror neutron guide, Nucl. Instrum. Methods Phys. Res. Sect. A 562, 407 (2006).
  34. A. Authier, S. Lagomarsino, and B. K. Tanner, X-ray and Neutron Dynamical Diffraction: Theory and Applications (Springer Science & Business Media, New York, 2012), Vol. 357.
  35. J. Schwinger, On the polarization of fast neutrons, Phys. Rev. 73, 407 (1948).
  36. C. Shull, Neutron spin-neutron orbit interaction with slow neutrons, Phys. Rev. Lett. 10, 297 (1963).
  37. C. Shull and R. Nathans, Search for a neutron electric dipole moment by a scattering experiment, Phys. Rev. Lett. 19, 384 (1967).
  38. V. Fedorov, I. Kuznetsov, E. Lapin, S. Y. Semenikhin, and V. Voronin, Neutron spin optics in noncentrosymmetric crystals as a new way for nEDM search, Nucl. Instrum. Methods Phys. Res. Sect. B 252, 131 (2006).
  39. V. V. Fedorov, M. Jentschel, I. A. Kuznetsov, E. G. Lapin, E. Lelièvre-Berna, V. Nesvizhevsky, A. Petoukhov, S. Yu. Semenikhin, T. Soldner, V. V. Voronin, and Y. P. Braginetz, Measurement of the neutron electric dipole moment via spin rotation in a non-centrosymmetric crystal, Phys. Lett. B 694, 22 (2010).
  40. V. Fedorov and V. Voronin, Modern status of searches for nEDM, using neutron optics and diffraction in noncentrosymmetric crystals, in Proceedings of the International Conference on Neutron Optics (NOP2017), JPS Conference Proceedings Vol. 22 (Physical Society of Japan, Tokyo, 2018), p. 011007.
  41. A. Zeilinger, M. A. Horne, and H. J. Bernstein, Symmetry violations and Schwinger scattering in neutron interferometry, J. Phys. Colloq. 45, C3-209 (1984).
  42. C. Abel, S. Afach, N. J. Ayres, C. A. Baker, G. Ban, G. Bison, K. Bodek, V. Bondar, M. Burghoff, E. Chanel, et al., Measurement of the permanent electric dipole moment of the neutron, Phys. Rev. Lett. 124, 081803 (2020).
  43. S. Lamoreaux and R. Golub, Experimental searches for the neutron electric dipole moment, J. Phys. G: Nucl. Part. Phys. 36, 104002 (2009).
  44. M. R. Schindler and R. P. Springer, The theory of parity violation in few-nucleon systems, Prog. Part. Nucl. Phys. 72, 1 (2013).
  45. W. M. Snow, C. D. Bass, T. D. Bass, B. E. Crawford, K. Gan, B. R. Heckel, D. Luo, D. M. Markoff, A. M. Micherdzinska, H. P. Mumm, J. S. Nico, A. K. Opper, M. Sarsour, E. I. Sharapov, H. E. Swanson, S. B. Walbridge, and V. Zhumabekova, Upper bound on parity-violating neutron spin rotation in He4, Phys. Rev. C 83, 022501 (2011).
  46. C. D. Bass, T. D. Bass, B. Heckel, C. Huffer, D. Luo, D. Markoff, A. Micherdzinska, W. Snow, H. Swanson, and S. Walbridge, A liquid helium target system for a measurement of parity violation in neutron spin rotation, Nucl. Instrum. Methods Phys. Res. Sect. A 612, 69 (2009).
  47. R. Musedinovic, L. S. Blokland, C. B. Cude-Woods, M. Singh, M. A. Blatnik, N. Callahan, J. H. Choi, S. M. Clayton, B. W. Filippone, W. R. Fox, et al., Measurement of the free neutron lifetime in a magneto-gravitational trap with in situ detection, Phys. Rev. C 111, 045501 (2025).
  48. J. Caylor, R. Biswas, B. Crawford, M. S. Dewey, N. Fomin, G. L. Greene, S. F. Hoogerheide, J. Hungria-Negron, H. P. Mumm, J. S. Nico, F. E. Wietfeldt, D. O. Valete, and J. Zuchegno, Detection of molecular hydrogen in a neutron beam lifetime experiment, Phys. Rev. C 112, 065501 (2025).
  49. Y. Fuwa, T. Hasegawa, K. Hirota, T. Hoshino, R. Hosokawa, G. Ichikawa, S. Ieki, T. Ino, Y. Iwashita, M. Kitaguchi, et al., Improved measurements of neutron lifetime with cold neutron beam at J-PARC, arXiv:2412.19519.
  50. T. Chowdhury and S. Ipek, Neutron lifetime anomaly and Big Bang nucleosynthesis, Can. J. Phys. 102, 96 (2024).
  51. B. Misra and E. G. Sudarshan, The Zeno's paradox in quantum theory, J. Math. Phys. 18, 756 (1977).
  52. W. M. Itano, D. J. Heinzen, J. J. Bollinger, and D. J. Wineland, Quantum Zeno effect, Phys. Rev. A 41, 2295 (1990).
  53. M. C. Fischer, B. Gutiérrez-Medina, and M. G. Raizen, Observation of the quantum Zeno and anti-Zeno effects in an unstable system, Phys. Rev. Lett. 87, 040402 (2001).
  54. P. Kwiat, H. Weinfurter, T. Herzog, A. Zeilinger, and M. A. Kasevich, Interaction-free measurement, Phys. Rev. Lett. 74, 4763 (1995).
  55. S. Pascazio, M. Namiki, G. Badurek, and H. Rauch, Quantum Zeno effect with neutron spin, Phys. Lett. A 179, 155 (1993).
  56. H. Rauch, Quantum Zeno-effect with polarized neutrons, Phys. B: Condens. Matter 297, 299 (2001).
  57. P. Facchi, Y. Nakaguro, H. Nakazato, S. Pascazio, M. Unoki, and K. Yuasa, Optimization of a neutron-spin test of the quantum Zeno effect, Phys. Rev. A 68, 012107 (2003).
  58. P. Lewalle, Y. Zhang, and K. B. Whaley, Optimal Zeno dragging for quantum control: A shortcut to Zeno with action-based scheduling optimization, PRX Quantum 5, 020366 (2024).
  59. S. Hacohen-Gourgy, L. P. García-Pintos, L. S. Martin, J. Dressel, and I. Siddiqi, Incoherent qubit control using the quantum Zeno effect, Phys. Rev. Lett. 120, 020505 (2018).
  60. T. R. Gentile, P. Nacher, B. Saam, and T. G. Walker, Optically polarized He3, Rev. Mod. Phys. 89, 045004 (2017).
  61. S. A. Werner, R. Colella, A. W. Overhauser, and C. Eagen, Observation of the phase shift of a neutron due to precession in a magnetic field, Phys. Rev. Lett. 35, 1053 (1975).
  62. M. G. Huber, M. Arif, T. C. Black, W. C. Chen, T. R. Gentile, D. S. Hussey, D. A. Pushin, F. E. Wietfeldt, and L. Yang, Precision measurement of the n−He3 incoherent scattering length using neutron interferometry, Phys. Rev. Lett. 102, 200401 (2009).
  63. M. G. Huber, M. Arif, W. C. Chen, T. R. Gentile, D. S. Hussey, T. C. Black, D. A. Pushin, C. B. Shahi, F. E. Wietfeldt, and L. Yang, Neutron interferometric measurement of the scattering length difference between the triplet and singlet, Phys. Rev. C 90, 064004 (2014).
  64. D. Burgarth, P. Facchi, G. Gramegna, and K. Yuasa, One bound to rule them all: From adiabatic to Zeno, Quantum 6, 737 (2022).
  65. Y. Aharonov and A. Casher, Topological quantum effects for neutral particles, Phys. Rev. Lett. 53, 319 (1984).
  66. A. Cimmino, G. I. Opat, A. G. Klein, S. A. Werner, S. Werner, M. Arif, and R. Clothier, Observation of the topological Aharonov-Casher phase shift by neutron interferometry, Phys. Rev. Lett. 63, 380 (1989).
  67. S. Boffi and G. Caglioti, Further remarks on the coherence properties of a thermal neutron beam, Nuov. Cim. B 3, 262 (1971).
  68. M. Silverman, On the feasibility of a neutron Hanbury Brown—Twiss experiment with gravitationally-induced phase shift, Phys. Lett. A 132, 154 (1988).
  69. M. Iannuzzi, A. Orecchini, F. Sacchetti, P. Facchi, and S. Pascazio, Direct experimental evidence of free-fermion antibunching, Phys. Rev. Lett. 96, 080402 (2006).
  70. M. Iannuzzi, R. Messi, D. Moricciani, A. Orecchini, F. Sacchetti, P. Facchi, and S. Pascazio, Further evidence of antibunching of two coherent beams of fermions, Phys. Rev. A 84, 015601 (2011).
  71. O. Lailey, D. Sarenac, D. G. Cory, M. G. Huber, and D. A. Pushin, Unified quantum walk model for internal crystal effects in dynamical diffraction, Phys. Rev. A 114, 032210 (2026).
  72. O. Lailey, Unified QI model code [Computer software], Zenodo, 2026, https://doi.org/10.5281/zenodo.23345317.

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation