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Pressure and oxygen-isotope substitution on density-wave transitions in
Phys. Rev. Research 8, 013249 – Published 9 March, 2026
DOI: https://doi.org/10.1103/nrqn-m22c
Abstract
Understanding the interplay between magnetism and superconductivity in nickelate systems is a key objective in condensed matter physics. Gaining microscopic insights into magnetism—particularly as it emerges near superconductivity—requires a synergistic approach that combines complementary experimental techniques with controlled tuning of external parameters. In this paper, we present a systematic investigation of the three-layer Ruddlesden-Popper (RP) nickelate using muon-spin rotation/relaxation () and resistivity measurements. At ambient pressure, two incommensurate spin-density-wave (SDW) transitions are identified at and . Comparison of the observed internal magnetic fields with dipole-field calculations reveals a magnetic structure consistent with antiferromagnetically coupled SDW order on the outer two Ni-O layers, with smaller moments on the inner Ni-O layer. Above , the moments lie primarily in the plane, but below this temperature they undergo a subtle distortion and develop a -axis component. The internal fields at the muon stopping sites appear abruptly at , suggesting a first-order-like nature of the SDW transition, which is closely linked to the charge-density wave (CDW) order occurring at the same temperature (). Under applied pressure, all transition temperatures—including , and —are suppressed at a nearly uniform rate of K/GPa. This behavior contrasts with that of the two-layer RP nickelate , where pressure enhances the separation between the SDW and CDW transitions. The oxygen-isotope substitution () reveals that the CDW transition temperature shifts to higher values in the -substituted samples. The isotope effect on and differs significantly. Specifically, when the CDW and SDW orders are intertwined, a notable isotope effect is observed on , leading to equal transition temperatures and nearly identical isotope shifts for both and . In contrast, at , where the SDW transition occurs independently of the CDW, no isotope effect is detected.
Physics Subject Headings (PhySH)
See Also
Oxygen-isotope effect on the density wave transitions in
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