Reuse & Permissions

It is not necessary to obtain permission to reuse this article or its components as it is available under the terms of the Creative Commons Attribution 4.0 International license. This license permits unrestricted use, distribution, and reproduction in any medium, provided attribution to the author(s) and the published article's title, journal citation, and DOI are maintained. Please note that some figures may have been included with permission from other third parties. It is your responsibility to obtain the proper permission from the rights holder directly for these figures.

Export citation

Export citation

Choose format for download:

Download Citation
  • Open Access

Percolation of a cohesive fine particle in a static bed

Jizhi Zhang1, Qiong Zhang2, Julio M. Ottino2,3,4, Paul B. Umbanhowar2, and Richard M. Lueptow2,3,4,*

  • *Contact author: r-lueptow@northwestern.edu

Phys. Rev. Research 8, 033336 – Published 18 September, 2026

DOI: https://doi.org/10.1103/ndnk-2x1g

Abstract

Percolation of fine particles (fines) in a static bed of larger particles is central to many industrial and natural processes. Noncohesive fines either pass through the bed or become trapped depending on multiple factors including particle sizes, friction and restitution coefficients, and size polydispersity. Here, we consider the additional factor of cohesion in the single-particle limit. We use the discrete element method to simulate gravity-driven percolation of non-self-interacting cohesive fine particles through a static bed of randomly packed large particles; fines interact with bed particles but not with each other. A large-to-fine particle diameter ratio of seven geometrically permits noncohesive fines to pass the narrowest pore throats formed by the large particles so they can freely percolate. However, sufficiently large cohesion and friction lead to nongeometric trapping. Fines are trapped when they fail to rebound after a collision, due to large cohesion, low restitution, and low collision velocity, and any subsequent rolling or sliding is insufficient to cause detachment. This establishes a sequence of local interactions—collision, adhesion, and postcontact motion—that governs the ultimate fate of a fine particle. A collisional model that incorporates a trapping probability per collision and a collision frequency predicts the trapping distance in the regime dominated by collision-induced trapping. For nonrebounding collisions, frictional effects are enhanced by cohesion and, when large enough, prevent the fine particle from subsequently detaching. A static equilibrium condition based on force balance predicts whether a fine particle remains stationary after contact. These results show that percolation of cohesive fine particles in the single-particle limit is not determined by geometric accessibility alone, but also by particle-scale interaction dynamics that can override geometric expectations.

View figure in article

Physics Subject Headings (PhySH)

Article Text

References (48)

  1. H. M. Jaeger, S. R. Nagel, and R. P. Behringer, Granular solids, liquids, and gases, Rev. Mod. Phys. 68, 1259 (1996).
  2. J. Duran, Sands, Powders, and Grains: An Introduction to the Physics of Granular Materials (Springer New York, New York, NY, 2012).
  3. C. Bemrose and J. Bridgwater, A review of attrition and attrition test methods, Powder Technol. 49, 97 (1987).
  4. D. Schulze, Powders and Bulk Solids: Behavior, Characterization, Storage and Flow (Springer Berlin, Heidelberg, 2008).
  5. M. Sharma and Y. Yortsos, Fines migration in porous media, AIChE J. 33, 1654 (1987).
  6. W. Fang, S. Chen, S. Li, and I. Zuriguel, Clogging transition of granular flow in porous structures, Phys. Rev. Res. 6, 033046 (2024).
  7. I. Ippolito, L. Samson, S. Bourles, and J.-P. Hulin, Diffusion of a single particle in a 3d random packing of spheres, Eur. Phys. J. E 3, 227 (2000).
  8. F. Lominé and L. Oger, Dispersion of particles by spontaneous interparticle percolation through unconsolidated porous media, Phys. Rev. E 79, 051307 (2009).
  9. D. R. Vyas, S. Gao, P. B. Umbanhowar, J. M. Ottino, and R. M. Lueptow, Impacts of packed bed polydispersity and deformation on fine particle transport, AIChE J. 70, e18499 (2024).
  10. J. Bridgwater, N. Sharpe, and D. Stocker, Particle mixing by percolation, Trans. Inst. Chem. Eng. 47, T114 (1969).
  11. J. Bridgwater and N. Ingram, Rate of spontaneous inter-particle percolation, Trans. Inst. Chem. Eng. 49, 163 (1971).
  12. J. Masliyah and J. Bridgwater, Particle percolation: A numerical study, Trans. Inst. Chem. Eng. 52, 31 (1974).
  13. S. Gao, J. M. Ottino, P. B. Umbanhowar, and R. M. Lueptow, Percolation of a fine particle in static granular beds, Phys. Rev. E 107, 014903 (2023).
  14. D. R. Vyas, R. M. Lueptow, J. M. Ottino, and P. B. Umbanhowar, Fine particle percolation dynamics in porous media, Phys. Rev. Res. 8, 013201 (2026).
  15. S. Remond, DEM simulation of small particles clogging in the packing of large beads, Physica A 389, 4485 (2010).
  16. R. S. Sharma and A. Sauret, Experimental models for cohesive granular materials: A review, Soft Matter 21, 2193 (2025).
  17. S. Iveson, J. Litster, and B. Ennis, Fundamental studies of granule consolidation part 1: Effects of binder content and binder viscosity, Powder Technol. 88, 15 (1996).
  18. J. Visser, Van der Waals and other cohesive forces affecting powder fluidization, Powder Technol. 58, 1 (1989).
  19. L. Bocquet, E. Charlaix, S. Ciliberto, and J. Crassous, Moisture-induced ageing in granular media and the kinetics of capillary condensation, Nature (London) 396, 735 (1998).
  20. T. C. Halsey and A. J. Levine, How sandcastles fall, Phys. Rev. Lett. 80, 3141 (1998).
  21. J. S. Marshall, Discrete-element modeling of particulate aerosol flows, J. Comput. Phys. 228, 1541 (2009).
  22. S. Krijt, C. Dominik, and A. Tielens, Rolling friction of adhesive microspheres, J. Phys. D 47, 175302 (2014).
  23. H. Abbasfard, G. Evans, and R. Moreno-Atanasio, Effect of van der Waals force cut-off distance on adhesive collision parameters in DEM simulation, Powder Technol. 299, 9 (2016).
  24. E. Murphy and S. Subramaniam, Binary collision outcomes for inelastic soft-sphere models with cohesion, Powder Technol. 305, 462 (2017).
  25. W. C. Q. LaMarche, P. Liu, K. M. Kellogg, A. M. Lattanzi, and C. M. Hrenya, Toward general regime maps for cohesive-particle flows: Force versus energy-based descriptions and relevant dimensionless groups, AIChE J. 67, e17337 (2021).
  26. Y. Wang, Y. Wang, M. Zhou, and L. Duan, Energy dissipation mechanisms in particle collisions on submicron particle-layers: Experimental and DEM analysis, Chem. Eng. Sci. 316, 121933 (2025).
  27. A. Castellanos, J. M. Valverde, and M. A. S. Quintanilla, Aggregation and sedimentation in gas-fluidized beds of cohesive powders, Phys. Rev. E 64, 041304 (2001).
  28. J. Tomas, Fundamentals of cohesive powder consolidation and flow, Granular Matter 6, 75 (2004).
  29. K. M. Kellogg, P. Liu, C. Q. LaMarche, and C. M. Hrenya, Continuum theory for rapid cohesive-particle flows: General balance equations and discrete-element-method-based closure of cohesion-specific quantities, J. Fluid Mech. 832, 345 (2017).
  30. K. M. Kellogg, P. Liu, and C. M. Hrenya, Discrete-element-method-based determination of particle-level inputs for the continuum theory of flows with moderately cohesive particles, Processes 11, 2553 (2023).
  31. S. Mandal, M. Nicolas, and O. Pouliquen, Insights into the rheology of cohesive granular media, Proc. Natl. Acad. Sci. USA 117, 8366 (2020).
  32. S. Mandal, M. Nicolas, and O. Pouliquen, Rheology of cohesive granular media: Shear banding, hysteresis, and nonlocal effects, Phys. Rev. X 11, 021017 (2021).
  33. S. Plimpton, Fast parallel algorithms for short-range molecular dynamics, J. Comput. Phys. 117, 1 (1995).
  34. A. P. Thompson, H. M. Aktulga, R. Berger, D. S. Bolintineanu, W. M. Brown, P. S. Crozier, P. J. In't Veld, A. Kohlmeyer, S. G. Moore, T. D. Nguyen, et al., LAMMPS—A flexible simulation tool for particle-based materials modeling at the atomic, meso, and continuum scales, Comput. Phys. Commun. 271, 108171 (2022).
  35. D. R. Vyas, J. M. Ottino, R. M. Lueptow, and P. B. Umbanhowar, Improved velocity-Verlet algorithm for the discrete element method, Comput. Phys. Commun. 310, 109524 (2025).
  36. C. Thornton, S. J. Cummins, and P. W. Cleary, An investigation of the comparative behaviour of alternative contact force models during elastic collisions, Powder Technol. 210, 189 (2011).
  37. D. Antypov and J. A. Elliott, On an analytical solution for the damped Hertzian spring, Europhys. Lett. 94, 50004 (2011).
  38. R. D. Mindlin, Compliance of elastic bodies in contact, J. Appl. Mech. 16, 259 (1949).
  39. S. Luding, Cohesive, frictional powders: Contact models for tension, Granular Matter 10, 235 (2008).
  40. Y. Wang, F. Alonso-Marroquin, and W. W. Guo, Rolling and sliding in 3-D discrete element models, Particuology 23, 49 (2015).
  41. S. T. Nase, W. L. Vargas, A. A. Abatan, and J. McCarthy, Discrete characterization tools for cohesive granular material, Powder Technol. 116, 214 (2001).
  42. P.-G. De Gennes, F. Brochard-Wyart, and D. Quéré, Capillarity and Wetting Phenomena: Drops, Bubbles, Pearls, Waves (Springer New York, New York, NY, 2003).
  43. V. Ralaiarisoa, P. Dupont, A. O. E. Moctar, F. Naaim-Bouvet, L. Oger, and A. Valance, Particle impact on a cohesive granular media, Phys. Rev. E 105, 054902 (2022).
  44. A. Jarray, H. Shi, B. J. Scheper, M. Habibi, and S. Luding, Cohesion-driven mixing and segregation of dry granular media, Sci. Rep. 9, 13480 (2019).
  45. B. V. Derjaguin, V. M. Muller, and Y. P. Toporov, Effect of contact deformations on the adhesion of particles, J. Colloid Interface Sci. 53, 314 (1975).
  46. K. L. Johnson, K. Kendall, and A. D. Roberts, Surface energy and the contact of elastic solids, Proc. R. Soc. London A 324, 301 (1971).
  47. D. Tabor, Surface forces and surface interactions, J. Colloid Interface Sci. 58, 2 (1977).
  48. J. Zhang, v1.0.0, Percolation_of_a_cohesive_fine_particle_in_a_static_bed, 2026.

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation