- Open Access
Resolving quantum Cooper-pair tunneling in graphene Josephson junctions under near-infrared illumination
Phys. Rev. Research 8, 013079 – Published 26 January, 2026
DOI: https://doi.org/10.1103/d38l-1g8r
Abstract
We report the observation of discrete supercurrent suppression steps arising from quantum Cooper-pair tunneling in superconductor-graphene-superconductor (SGS) Josephson junctions under near-infrared illumination. This quantum phenomenon remains robust against variations in photon energy, optical power, bath temperature, and dc bias. The nearly identical step spacing observed in SGS Josephson junctions with different graphene channel lengths indicates the dominant role of the superconductor-graphene interface in governing Cooper-pair transport. In contrast, the discrete steps vanish in the negative differential resistance regime, where quasiparticle transport dominates, confirming their microscopic Cooper-pair tunneling origin.
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References (40)
- L. J. Geerligs, V. F. Anderegg, J. Romijn, and J. E. Mooij, Single Cooper pair tunneling in small-capacitance junctions, Phys. Rev. Lett. 65, 377 (1990).
- M. Watanabe and D. B. Haviland, Coulomb blockade and coherent single Cooper pair tunneling in single Josephson junctions, Phys. Rev. Lett. 86, 5120 (2001).
- M. Titov and C. W. J. Beenakker, Josephson effect in ballistic graphene, Phys. Rev. B 74, 041401(R) (2006).
- H. B. Heersche, P. Jarillo-Herrero, J. B. Oostinga, L. M. K. Vandersypen, and A. F. Morpurpo, Bipolar supercurrent in graphene, Nature (London) 446, 56 (2007).
- G. H. Lee and H. J. Lee, Proximity coupling in superconductor-graphene heterostructures, Rep. Prog. Phys. 81, 056502 (2018).
- E. D. Walsh, W. Jung, G. H. Lee, D. K. Efetov, B. I. Wu, K. F. Huang, T. A. Ohki, T. Taniguchi, K. Watanabe, P. Kim, D. Englund, and K. C. Fong, Josephson junction infrared single-photon detector, Science 372, 409 (2021).
- G. H. Lee, D. K. Efetov, W. Jung, L. Ranzani, E. D. Walsh, T. A. Ohki, T. Taniguchi, K. Watanabe, P. Kim, D. Englund, and K. C. Fong, Graphene-based Josephson junction microwave bolometer, Nature (London) 586, 42 (2020).
- R. Kokkoniemi, J. P. Girard, D. Hazra, A. Laitinen, J. Govenius, R. E. Lake, I. Sallinen, V. Vesterinen, M. Partanen, J. Y. Tan, K. W. Chan, K. Y. Tan, P. Hakonen, and M. Mottonen, Bolometer operating at the threshold for circuit quantum electrodynamics, Nature (London) 586, 47 (2020).
- W. Miao, F. M. Li, Q. H. Luo, Q. C. Wang, J. Q. Zhong, Z. Wang, K. M. Zhou, Y. Ren, W. Zhang, J. Li, S. C. Shi, C. Yu, Z. Z. He, Q. B. Liu, and Z. H. Feng, A terahertz detector based on superconductor-graphene-superconductor Josephson junction, Carbon 202, 112 (2023).
- Z. Z. He, C. Yu, Q. B. Liu, X. B. Song, X. D. Gao, J. C. Guo, C. J. Zhou, S. J. Cai, and Z. H. Feng, High temperature RF performances of epitaxial bilayer graphene field-effect transistors on SiC substrate, Carbon 164, 435 (2020).
- C. Yu, Q. B. Liu, J. Li, W. L. Lu, Z. Z. He, S. J. Cai, and Z. H. Feng, Preparation and electrical transport properties of quasi free standing bilayer graphene on SiC(0001) substrate by H intercalation, Appl. Phys. Lett. 105, 183105 (2014).
- C. Riedl, C. Coletti, T. Iwasaki, A. A. Zakharov, and U. Starke, Quasi-free-standing epitaxial graphene on SiC obtained by hydrogen intercalation, Phys. Rev. Lett. 103, 246804 (2009).
- L. Banszerus, M. Schmitz, S. Engels, M. Goldsche, K. Watanabe, T. Taniguchi, B. Beschoten, and C. Stampfer, Ballistic transport exceeding 28 µm in CVD grown graphene, Nano Lett. 16, 1387 (2016).
- D. Drung, High- and low- dc SQUID electronics, Supercond. Sci. Technol. 16, 1320 (2003).
- A. I. Golovashkin, I. E. Leksina, G. P. Motulevich, and A. A. Shubin, The optical properties of niobium, Sov. Phys. JETP 29, 27 (1969).
- A. Wallraff, A. Lukashenko, C. Coqui, A. Kemp, T. Duty, and A. V. Ustinov, Switching current measurements of large area Josephson tunnel junctions, Rev. Sci. Instrum. 74, 3740 (2003).
- G. H. Lee, S. Kim, S. H. Jhi, and H. J. Lee, Ultimately short ballistic vertical graphene Josephson junctions, Nat. Commun. 6, 6181 (2015).
- G. H. Park, W. Lee, S. Park, K. Watanabe, T. Taniguchi, G. Y. Cho, and G. H. Lee, Controllable Andreev bound states in bilayer graphene Josephson junctions from short to long junction limits, Phys. Rev. Lett. 132, 226301 (2024).
- Y. Nam, D. K. Ki, D. S. Delgado, and A. F. Morpurgo, Electron-hole collision limited transport in charge-neutral bilayer graphene, Nat. Phys. 13, 1207 (2017).
- P. Dubos, H. Courtois, B. Pannetier, F. K. Wilhelm, A. D. Zaikin, and G. Schon, Josephson critical current in a long mesoscopic SNS junction, Phys. Rev. B 63, 064502 (2001).
- D. Jeong, J. H. Choi, G. H. Lee, S. Jo, Y. J. Doh, and H. J. Lee, Observation of supercurrent in PbIn-graphene-PbIn Josephson junction, Phys. Rev. B 83, 094503 (2011).
- C. T. Ke, I. V. Borzenets, A. W. Draelos, F. Amet, Y. Bomze, G. Jones, M. Craciun, S. Russo, M. Yamamoto, S. Tarucha, and G. Finkelstein, Critical current scaling in long diffusive graphene-based Josephson junctions, Nano Lett. 16, 4788 (2016).
- C. Li, S. Gueron, A. Chepelianskii, and H. Bouchiat, Full range of proximity effect probed with superconductor/graphene/superconductor junctions, Phys. Rev. B 94, 115405 (2016).
- R. S. Shaikhaidarov, K. H. Kim, J. W. Dunstan, I. V. Antonov, S. Linzen, M. Ziegler, D. S. Golubev, V. N. Antonov, E. V. Il'ichev, and O. V. Astafiev, Quantized current steps due to the a.c. coherent quantum phase-slip effect, Nature (London) 608, 45 (2022).
- D. Fukuda, G. Fujii, A. Yoshizawa, H. Tsuchida, R. M. T. Damayanthi, H. Takahashi, S. Inoue, and M. Ohkubo, High speed photon number resolving detector with titanium transition edge sensor, J. Low Temp. Phys. 151, 100 (2008).
- W. Zhang, Y. Gen, Z. Wang, J. Q. Zhong, P. Z. Li, W. Miao, Y. Ren, Q. J. Yao, J. F. Wang, and S. C. Shi, Development of titanium-based transition-edge single-photon detector, IEEE Trans. Appl. Supercond. 29, 2100505 (2019).
- R. Barends, J. J. A. Baselmans, S. J. C. Yates, J. R. Gao, J. N. Hovenier, and T. M. Klapwijk, Quasiparticle relaxation in optically excited high-Q superconducting resonators, Phys. Rev. Lett. 100, 257002 (2008).
- J. Hu, J. M. Matin, P. Nicaise, F. Boussaha, C. Chaumont, M. Piat, V. D. Pham, and P. Bonifacio, Investigation of quasi-particle relaxation in strongly disordered superconductor resonators, Supercond. Sci. Technol. 37, 055014 (2024).
- S. B. Kaplan, C. C. Chi, D. N. Langenberg, J. J. Chang, S. Jafarey, and D. J. Scalapino, Quasiparticle and phonon lifetimes in superconductors, Phys. Rev. B 14, 4854 (1976).
- R. Barends, S. van Vliet, J. J. A. Baselmans, S. J. C. Yates, J. R. Gao, and T. M. Klapwijk, Enhancement of quasiparticle recombination in Ta and Al superconductors by implantation of magnetic and nonmagnetic atoms, Phys. Rev. B 79, 020509 (2009).
- P. J. de Visser, J. J. A. Baselmans, P. Diener, S. J. C. Yates, A. Endo, and T. M. Klapwijk, Number fluctuations of sparse quasiparticles in a superconductor, Phys. Rev. Lett. 106, 167004 (2011).
- L. Lolli, G. Brida, I. P. Degiovanni, M. Gramegna, E. Monticone, F. Piacentini, C. Portesi, M. Rajteri, I. R. Berchera, E. Taralli, and P. Traina, Ti/Au TES as superconducting detector for quantum technologies, Int. J. Quantum Inf. 9, 405 (2011).
- P. Z. Li, Y. Geng, W. Zhang, J. Q. Zhong, Z. Wang, K. M. Zhou, W. Miao, Y. Ren, F. Wu, K. Zhang, Q. J. Yao, and S. C. Shi, Development of self-aligned Ti optical transition-edge sensors at 1550 nm, J. Low Temp. Phys. 209, 248 (2022).
- A. G. Kozorezov, A. F. Volkov, J. K. Wigmore, A. Peacock, A. Poelaert, and R. den Hartog, Quasiparticle-phonon downconversion in nonequilibrium superconductors, Phys. Rev. B 61, 11807 (2000).
- K. D. Irwin, An application of electrothermal feedback for high resolution cryogenic particle detection, Appl. Phys. Lett. 66, 1998 (1995).
- A. Seredinski, A. W. Draelos, E. G. Arnault, M. T. Wei, H. Li, T. Fleming, K. Watanabe, T. Taniguchi, F. Amet, and G. Finkelstein, Quantum Hall-based superconducting interference device, Sci. Adv. 5, eaaw8693 (2019).
- C. Girit, V. Bouchiat, O. Naaman, Y. Zhang, M. F. Crommie, A. Zettl, and I. Siddiqi, Tunable graphene dc superconducting quantum interference device, Nano Lett. 9, 198 (2008).
- J. Sarkar, K. V. Salunkhe, S. Mandal, S. Ghatak, A. H. Marchawala, I. Das, K. Watanabe, T. Taniguchi, R. Vijay, and M. M. Deshmukh, Quantum-noise-limited microwave amplification using a graphene Josephson junction, Nat. Nanotechnol. 17, 1147 (2022).
- F. E. Schmidt, M. D. Jenkins, K. Watanabe, T. Taniguchi, and G. A. Steele, A ballistic graphene superconducting microwave circuit, Nat. Commun. 9, 4069 (2018).
- J. I-Jan Wang, D. Rodan-Legrain, L. Bretheau, D. L. Campbell, B. Kannan, D. Kim, M. Kjaergaard, P. Krantz, G. O. Samach, F. Yan, J. L. Yoder, K. Watanabe, T. Taniguchi, T. P. Orlando, S. Gustavsson, P. Jarillo-Herrero, and W. D. Oliver, Coherent control of a hybrid superconducting circuit made with graphene-based van der Waals heterostructures, Nat. Nanotechnol. 14, 120 (2018).