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Single-pass synchronized two-color attosecond x-ray free-electron laser featuring attosecond time jitter

Chuan Yang1,2,*, Yixuan Liu3, Chao Feng3, Juhao Wu4, and Weiqing Zhang5,†

  • *Contact author: yangc@mail.iasf.ac.cn
  • †Contact author: weiqingzhang@dicp.ac.cn

Phys. Rev. Research 8, 023048 – Published 15 April, 2026

DOI: https://doi.org/10.1103/cw2t-yvwd

Abstract

Two-color attosecond x-ray pulses are the key to advancing the study of ultrafast dynamics in quantum systems. In this work, we propose a single-pass free-electron laser scheme generating synchronized attosecond two-color x-ray pulses with femtosecond separation and tens-of-gigawatts peak power. By modulating a chirped electron beam with an infrared laser, we create a periodic train of ultrashort current spikes. This scheme utilizes the limited gain bandwidth of the free-electron laser as a filter, allowing only two adjacent current spikes with different resonance wavelengths to lase. This scheme holds promise for delivering sub-300-as two-color x-ray pulses with an intrinsic timing jitter below 100 as. This work provides insights and technical support for generating two-color attosecond x-ray free-electron laser pulses with robust time jitter.

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