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Moiré-resonant surface state in ultrathin
Phys. Rev. Research 8, 033058 – Published 13 July, 2026
DOI: https://doi.org/10.1103/cvqr-4wkd
Abstract
has emerged as a prototypical candidate for altermagnetism. In the face of daunting evidence for magnetic order in the bulk, the focus naturally shifted to surfaces and ultrathin films, where Coulomb interactions are dimensionally quenched and electron correlations strongly enhanced. Here, we examine atomically ordered, ultrathin grown on using a combination of scanning tunneling microscopy (STM), density functional theory, and density matrix renormalization group methods. We observe a nonmagnetic charge order that is imprinted by the incommensurate moiré stacking with the substrate and enhanced by the electronic Fermi-surface scattering within the flat-band surface state. We further identify a nonmagnetic, metastable surface reconstruction that arises from surface phonon softening and can be toggled reversibly via STM tip manipulation. Spin-polarized STM measurements, however, reveal no evidence of magnetic order on the surface. Our findings of a nonmagnetic charge modulation position ultrathin as an intriguing platform for exploring moiré-assisted electronic orders.
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