- Letter
- Open Access
Momentum imaging of electrons and recoil ions from anion–neutral interactions in a cryogenic ion storage ring
Phys. Rev. Research 7, L012082 – Published 25 March, 2025
DOI: https://doi.org/10.1103/PhysRevResearch.7.L012082
Abstract
We have momentum-analyzed electrons and recoil ions in triple coincidence with projectiles neutralized in 300-keV collisions. The experiment was performed at a cryogenic ion storage ring with an in-ring reaction microscope. Differential momentum distributions for detachment with simultaneous target ionization were obtained. At more than 15% of the detachment-only rate the ionization rate is surprisingly large. A correlated two-electron channel is found to be dominant. This is also unexpected because the projectile energy is well below the threshold for the correlated process.
Physics Subject Headings (PhySH)
Article Text
References (34)
- T. N. Rescigno, M. Baertschy, W. A. Isaacs, and C. W. McCurdy, Collisional breakup in a quantum system of three charged particles, Science 286, 2474 (1999).
- M. Schulz, R. Moshammer, D. Fischer, H. Kollmus, D. H. Madison, S. Jones, and J. Ullrich, Three-dimensional imaging of atomic four-body processes, Nature (London) 422, 48 (2003).
- H. Ehrhardt, K. Jung, G. Knoth, and P. Schlemmer, Z. Phys. D 1, 3 (1986).
- M. Schulz, in Ion-Atom Collisions. The Few-Body Problem in Dynamic Systems, edited by M. Schulz (deGruyter, Berlin, 2019), pp. 11–34.
- A. K. Edwards, in The Physics of Electronic and Atomic Collisions, edited by J. S. Risley and R. Geballe (University of Washington, Seattle, 1975), pp. 790–799.
- V. A. Esaulov, Electron detachment from atomic negative ions, Ann. Phys. Paris 11, 493 (1986).
- D. J. Pegg, Structure and dynamics of negative ions, Rep. Prog. Phys. 67, 857 (2004).
- F. Zappa, G. Jalbert, L. F. S. Coelho, A. B. Rocha, S. D. Magalhães, and N. V. de Castro Faria, Absolute electron detachment cross sections of atomic anions of the second and third periods incident on noble gases, Phys. Rev. A 69, 012703 (2004).
- H. Luna, F. Zappa, M. H. P. Martins, S. D. Magalhães, G. Jalbert, L. F. S. Coelho, and N. V. de Castro Faria, Comparative study of the collisional electron detachment of , and by light noble gases, Phys. Rev. A 63, 052716 (2001).
- B. Hird and F. Rahman, Charge neutralization of ions in thin rare-gas targets, Phys. Rev. A 26, 3108 (1982).
- N. Andersen, T. Andersen, L. Jepsen, and J. Macek, Electron detachment processes in keV -rare-gas collisions, J. Phys. B 17, 2281 (1984).
- J. S. Risley, Comparison of and detachment cross sections, Phys. Rev. A 10, 731 (1974).
- X. M. Zhang, S. M. Wu, G. W. Li, F. Q. Lu, J. Y. Tang, and F. J. Yang, Measurements of single-electron detachment cross-sections for and in collision with He and , Europhys. Lett. 56, 797 (2001).
- G. Jalbert, W. Wolff, S. D. Magalhaes, and N. V. de Castro Faria, Electron detachment of negative ions: The influence of the outermost electron and its neutral core atom in collision with He, Ne, and Ar, Phys. Rev. A 77, 012722 (2008).
- G. M. Sigaud, Free-collision model calculations for the electron detachment of anions by noble gases, J. Phys. B 41, 015205 (2007).
- T. Andersen, Atomic negative ions: Structure, dynamics and collisions, Phys. Rep. 394, 157 (2004).
- J. S. Risley, in Proceedings of the 11th International Conference on the Physics of Electronic and Atomic Collisions, Kyoto 1979, edited by N. Oda and K. Takayanagi (North-Holland, Amsterdam, 1980), p. 619.
- Y. N. Demkov and V. N. Ostrovsky, Zero-Range Potentials and their Applications in Atomic Physics (Plenum, New York, 1988).
- J. P. Gauyacq, Theoretical study of the detachment process in the zero-range potential approximation. collisions, J. Phys. B 13, 4417 (1980).
- J. P. Connerade and V. N. Ostrovsky, Electron detachment in collisions of negative ions with non-metallic clusters, J. Phys. B 35, L475 (2002).
- M. Schulz, F. Herrmann, W. Zhang, D. V. Chicharro, A. Dorn, M. Grieser, F. Grussie, H. Kreckel, O. Novotny, F. Trost, A. Wolf, T. Pfeifer, C. D. Schröter, and R. Moshammer, Multiple differential electron spectra from detachment in collisions of anions with atoms and molecules, Phys. Rev. A 110, 022818 (2024).
- M. E. Rudd, Y. K. Kim, D. H. Madison, and T. J. Gay, Electron production in proton collisions with atoms and molecules: energy distributions, Rev. Mod. Phys. 64, 441 (1992).
- N. Stolterfoht, R. A. Rivarola, and R. D. Dubois, Electron Emission in Heavy Ion-Atom Collisions (Springer, Berlin, 1997).
- L. H. Andersen, L. B. Nielsen, and J. Sörensen, Single and double ionisation of He and Ar by far and projectiles, J. Phys. B 21, 1587 (1988).
- F. Zappa, A. L. F. de Barros, L. F. S. Coelho, G. Jalbert, S. D. Magalhaes, and N. V. de Castro Faria, Ionization of helium by impact of negative B, O, and F ions, Phys. Rev. A 70, 034701 (2004).
- Z. Zhao, J. Li, and X. Zhang, Experimental study of ionization of Ar by impact of anions, Nucl. Instrum. Methods Phys. Res. B 283, 35 (2012).
- M. Schulz, T. Ferger, D. Fischer, R. Moshammer, and J. Ullrich, Multiple scattering mechanisms in simultaneous projectile-electron and target-electron ejection in collisions, Phys. Rev. A 74, 042705 (2006).
- J. A. Tanis, E. M. Bernstein, W. G. Graham, M. P. Stockli, M. Clark, R. H. McFarland, T. J. Morgan, K. H. Berkner, A. S. Schlachter, and J. W. Stearns, Resonant electron transfer and excitation in two-, three-, and four- electron and ions colliding with helium, Phys. Rev. Lett. 53, 2551 (1984).
- E. C. Montenegro, W. E. Meyerhof, and J. H. McGuire, Role of two-center electron-electron interaction in projectile electron excitation and loss, Adv. At. Mol. Opt. Phys. 34, 249 (1994).
- M. Scheer, R. C. Bilodeau, C. A. Brodie, and H. K. Haugen, Systematic study of the stable states of , and via infrared laser spectroscopy, Phys. Rev. A 58, 2844 (1998).
- R. von Hahn et al., The cryogenic storage ring CSR, Rev. Sci. Instrum. 87, 063115 (2016).
- J. Ullrich, R. Moshammer, A. Dorn, R. Dörner, L. Ph. H. Schmidt, and H. Schmidt-Böcking, Recoil-ion and electron momentum spectroscopy: Reaction-microscopes, Rep. Prog. Phys. 66, 1463 (2003).
- J. L. Wiza, Microchannel plate detectors, Nucl. Instrum. Methods 162, 587 (1979).
- H. Tawara and T. Kato, Total and partial ionization cross sections of atoms and ions by electron impact, At. Data Nucl. Data Tables 36, 167 (1987).