Reuse & Permissions

It is not necessary to obtain permission to reuse this article or its components as it is available under the terms of the Creative Commons Attribution 4.0 International license. This license permits unrestricted use, distribution, and reproduction in any medium, provided attribution to the author(s) and the published article's title, journal citation, and DOI are maintained. Please note that some figures may have been included with permission from other third parties. It is your responsibility to obtain the proper permission from the rights holder directly for these figures.

Export citation

Export citation

Choose format for download:

Download Citation
  • Letter
  • Open Access

Intertwined charge and spin density waves in a topological kagome material

Y. Chen1,2,3, J. Gaudet1,4,5, G. G. Marcus1, T. Nomoto6, T. Chen7, T. Tomita7, M. Ikhlas7, H. S. Suzuki7, Y. Zhao4,5 et al.

W. C. Chen4, J. Strempfer8, R. Arita6,9, S. Nakatsuji1,7,10,11,12, and C. Broholm1,4,13

Phys. Rev. Research 6, L032016 – Published 22 July, 2024

DOI: https://doi.org/10.1103/PhysRevResearch.6.L032016

Abstract

Using neutrons and x rays we show the topological kagome antiferromagnet Mn3Sn for T<285K forms a homogeneous spin and charge ordered state comprising a longitudinally polarized spin density wave with wave vector kβ=kβĉ, a helical modulated version of the room temperature antichiral magnetic order with kχ=kχĉ, and charge density waves with wave vectors 2kβ,2kχ, and kβ+kχ. Though kχ and kβ coincide for 200K<T<230K, they exhibit distinct continuous Tdependencies before locking to commensurate values of kβ=112c* and kχ=548c* at lowT. Density functional theory indicates this complex modulated state may be associated with the nesting of Fermi surfaces from correlated flat kagome bands, which host Weyl nodes that are annihilated as it forms.

View figure in article

Physics Subject Headings (PhySH)

Article Text

Supplemental Material

References (37)

  1. E. Liu, Y. Sun, N. Kumar, L. Muechler, A. Sun, L. Jiao, S.-Y. Yang, D. Liu, A. Liang, Q. Xu, J. Kroder, V. Süß, H. Borrmann, C. Shekhar, Z. Wang, C. Xi, W. Wang, W. Schnelle, S. Wirth, Y. Chen et al., Giant anomalous Hall effect in a ferromagnetic kagome-lattice semimetal, Nat. Phys. 14, 1125 (2018).
  2. S. Nakatsuji, N. Kiyohara, and T. Higo, Large anomalous Hall effect in a non-collinear antiferromagnet at room temperature, Nature (London) 527, 212 (2015).
  3. N. P. Armitage, E. J. Mele, and A. Vishwanath, Weyl and Dirac semimetals in three-dimensional solids, Rev. Mod. Phys. 90, 015001 (2018).
  4. B. R. Ortiz, L. C. Gomes, J. R. Morey, M. Winiarski, M. Bordelon, J. S. Mangum, L. W. H. Oswald, J. A. Rodriguez-Rivera, J. R. Neilson, S. D. Wilson, E. Ertekin, T. M. McQueen, and E. S. Toberer, New kagome prototype materials: discovery of KV3Sb5, RbV3Sb5, and CsV3Sb5, Phys. Rev. Mater. 3, 094407 (2019).
  5. Y.-X. Jiang, J.-X. Yin, M. M. Denner, N. Shumiya, B. R. Ortiz, G. Xu, Z. Guguchia, J. He, Md S. Hossain, X. Liu, J. Ruff, L. Kautzsch, S. S. Zhang, G. Chang, I. Belopolski, Q. Zhang, T. A. Cochran, D. Multer, M. Litskevich, Z.-J. Cheng et al., Unconventional chiral charge order in kagome superconductor KV3Sb5, Nat. Mater. 20, 1353 (2021).
  6. B. R. Ortiz, P. M. Sarte, E. M. Kenney, M. J. Graf, S. M. L. Teicher, R. Seshadri, and S. D. Wilson, Superconductivity in the Z2 kagome metal KV3Sb5, Phys. Rev. Mater. 5, 034801 (2021).
  7. B. R. Ortiz, S. M. L. Teicher, Y. Hu, J. L. Zuo, P. M. Sarte, E. C. Schueller, A. M. M. Abeykoon, M. J. Krogstad, S. Rosenkranz, R. Osborn, R. Seshadri, L. Balents, J. He, and Stephen D. Wilson, CsV3Sb5:AZ2 topological kagome metal with a superconducting ground state, Phys. Rev. Lett. 125, 247002 (2020).
  8. H. Li, T. T. Zhang, T. Yilmaz, Y. Y. Pai, C. E. Marvinney, A. Said, Q. W. Yin, C. S. Gong, Z. J. Tu, E. Vescovo, C. S. Nelson, R. G. Moore, S. Murakami, H. C. Lei, H. N. Lee, B. J. Lawrie, and H. Miao, Observation of unconventional charge density wave without acoustic phonon anomaly in kagome superconductors AV3sb5 (A=Rb, Cs), Phys. Rev. X 11, 031050 (2021).
  9. A. Moreo, S. Yunoki, and E. Dagotto, Phase separation scenario for manganese oxides and related materials, Science 283, 2034 (1999).
  10. K. Kuroda, T. Tomita, M.-T. Suzuki, C. Bareille, A. A. Nugroho, P. Goswami, M. Ochi, M. Ikhlas, M. Nakayama, S. Akebi, R. Noguchi, R. Ishii, N. Inami, K. Ono, H. Kumigashira, A. Varykhalov, T. Muro, T. Koretsune, R. Arita, S. Shin et al., Evidence for magnetic Weyl fermions in a correlated metal, Nat. Mater. 16, 1090 (2017).
  11. T. Chen, T. Tomita, S. Minami, M. Fu, T. Koretsune, M. Kitatani, I. Muhammad, D. Nishio-Hamane, R. Ishii, F. Ishii et al., Anomalous transport due to Weyl fermions in the chiral antiferromagnets Mn3X,X=Sn,Ge, Nat. Commun. 12, 572 (2021).
  12. J. W. Cable, N. Wakabayashi, and P. Radhakrishna, A neutron study of the magnetic structure of Mn3Sn, Solid State Commun. 88, 161 (1993).
  13. Y. Song, Y. Hao, S. Wang, J. Zhang, Q. Huang, X. Xing, and J. Chen, Complicated magnetic structure and its strong correlation with the anomalous Hall effect in Mn3Sn, Phys. Rev. B 101, 144422 (2020).
  14. S. Tomiyoshi and Y. Yamaguchi, Magnetic structure and weak ferromagnetism of Mn3Sn studied by polarized neutron diffraction, J. Phys. Soc. Jpn. 51, 2478 (1982).
  15. S. Tomiyoshi, Polarized neutron diffraction study of the spin structure of Mn3Sn, J. Phys. Soc. Jpn. 51, 803 (1982).
  16. H. Ohmori, S. Tomiyoshi, H. Yamauchi, and H. Yamamoto, Spin structure and weak ferromagnetism of Mn3Sn, J. Magn. Magn. Mater. 70, 249 (1987).
  17. P. J. Brown, V. Nunez, F. Tasset, J. B. Forsyth, and P. Radhakrishna, Determination of the magnetic structure of Mn3Sn using generalized neutron polarization analysis, J. Phys.: Condens. Matter 2, 9409 (1990).
  18. M. Ikhlas, T. Tomita, T. Koretsune, M.-T. Suzuki, D. Nishio-Hamane, R. Arita, Y. Otani, and S. Nakatsuji, Large anomalous Nernst effect at room temperature in a chiral antiferromagnet, Nat. Phys. 13, 1085 (2017).
  19. M. Kimata, H. Chen, K. Kondou, S. Sugimoto, P. K. Muduli, M. Ikhlas, Y. Omori, T. Tomita, A. H. MacDonald, S. Nakatsuji, and Y. Otani, Magnetic and magnetic inverse spin Hall effects in a non-collinear antiferromagnet, Nature (London) 565, 627 (2019).
  20. Z. Li, J. Zhuang, L. Wang, H. Feng, Q. Gao, X. Xu, W. Hao, X. Wang, C. Zhang, K. Wu, S. X. Dou, L. Chen, Z. Hu, and Y. Du, Realization of flat band with possible nontrivial topology in electronic kagome lattice, Sci. Adv. 4, eaau4511 (2018).
  21. N. J. Ghimire and I. I. Mazin, Topology and correlations on the kagome lattice, Nat. Mater. 19, 137 (2020).
  22. See Supplemental Material at http://link.aps.org/supplemental/10.1103/PhysRevResearch.6.L032016 for extra experimental details, data, and discussion about the phase transition.
  23. E. Fawcett, Spin-density-wave antiferromagnetism in chromium, Rev. Mod. Phys. 60, 209 (1988).
  24. X. Teng, L. Chen, F. Ye, E. Rosenberg, Z. Liu, J.-X. Yin, Y.-X. Jiang, J. S. Oh, M. Z. Hasan, K. J. Neubauer, B. Gao, Y. Xie, M. Hashimoto, D. Lu, C. Jozwiak, A. Bostwick, E. Rotenberg, R. J. Birgeneau, J.-H. Chu, M. Yi et al., Discovery of charge density wave in a kagome lattice antiferromagnet, Nature (London) 609, 490 (2022).
  25. X. Teng, J. S. Oh, H. Tan, L. Chen, J. Huang, B. Gao, J.-X. Yin, J.-H. Chu, M. Hashimoto, D. Lu, C. Jozwiak, A. Bostwick, E. Rotenberg, G. E. Granroth, B. Yan, R. J. Birgeneau, P. Dai, and M. Yi, Magnetism and charge density wave order in kagome FeGe, Nat. Phys. 19, 814 (2023).
  26. Y. Chen, J. Gaudet, S. Dasgupta, G. G. Marcus, J. Lin, T. Chen, T. Tomita, M. Ikhlas, Y. Zhao, W. C. Chen, M. B. Stone, O. Tchernyshyov, S. Nakatsuji, and C. Broholm, Antichiral spin order, its soft modes, and their hybridization with phonons in the topological semimetal Mn3Ge, Phys. Rev. B 102, 054403 (2020).
  27. J.-R. Soh, F. de Juan, N. Qureshi, H. Jacobsen, H.-Y. Wang, Y.-F. Guo, and A. T. Boothroyd, Ground-state magnetic structure of Mn3Ge, Phys. Rev. B 101, 140411(R) (2020).
  28. D. Khadka, T. R. Thapaliya, S. Hurtado Parra, X. Han, J. Wen, R. F. Need, P. Khanal, W. Wang, J. Zang, J. M. Kikkawa, L. Wu, and S. X. Huang, Kondo physics in antiferromagnetic Weyl semimetal Mn3+xSn1−x films, Sci. Adv. 6, eabc1977 (2020).
  29. S. Dasgupta and O. Tchernyshyov, Theory of spin waves in a hexagonal antiferromagnet, Phys. Rev. B 102, 144417 (2020).
  30. M. Ikhlas, T. Tomita, and S. Nakatsuji, Sample quality dependence of the magnetic properties in non-collinear antiferromagnet Mn3Sn, JPS Conf. Proc. 30, 011177 (2020).
  31. W. J. Feng, D. Li, W. J. Ren, Y. B. Li, W. F. Li, J. Li, Y. Q. Zhang, and Z. D. Zhang, Glassy ferromagnetism in Ni3Sn-type Mn3.1Sn0.9, Phys. Rev. B 73, 205105 (2006).
  32. X. Li, L. Xu, L. Ding, J. Wang, M. Shen, X. Lu, Z. Zhu, and K. Behnia, Anomalous Nernst and Righi-Leduc effects in Mn3Sn: Berry curvature and entropy flow, Phys. Rev. Lett. 119, 056601 (2017).
  33. N. H. Sung, F. Ronning, J. D. Thompson, and E. D. Bauer, Magnetic phase dependence of the anomalous Hall effect in Mn3Sn single crystals, Appl. Phys. Lett. 112, 132406 (2018).
  34. N. J. Ghimire, R. L. Dally, L. Poudel, D. C. Jones, D. Michel, N. T. Magar, M. Bleuel, M. A. McGuire, J. S. Jiang, J. F. Mitchell, J. W. Lynn, and I. I. Mazin, Competing magnetic phases and fluctuation-driven scalar spin chirality in the kagome metal YMn6Sn6, Sci. Adv. 6, eabe2680 (2020).
  35. P. Park, J. Oh, K. Uhlířová, J. Jackson, A. Deák, L. Szunyogh, K. H. Lee, H. Cho, H.-L. Kim, H. C. Walker, D. Adroja, V. Sechovský, and J.-G. Park, Magnetic excitations in non-collinear antiferromagnetic Weyl semimetal Mn3Sn, npj Quantum Mater. 3, 63 (2018).
  36. J. Liu and L. Balents, Anomalous Hall effect and topological defects in antiferromagnetic Weyl semimetals: Mn3Sn/Ge, Phys. Rev. Lett. 119, 087202 (2017).
  37. S. Nakatsuji and R. Arita, Topological magnets: Functions based on Berry phase and multipoles, Annu. Rev. Condens. Matter Phys. 13, 119 (2022).

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation