- Letter
- Open Access
Protection of correlation-induced phase instabilities by exceptional susceptibilities
Phys. Rev. Research 6, L022031 – Published 6 May, 2024
DOI: https://doi.org/10.1103/PhysRevResearch.6.L022031
Abstract
At thermal equilibrium, we find that generalized susceptibilities encoding the static physical response properties of Hermitian many-electron systems possess inherent non-Hermitian (NH) matrix symmetries. This leads to the generic occurrence of exceptional points (EPs), i.e., NH spectral degeneracies, in the generalized susceptibilities of prototypical Fermi-Hubbard models, as a function of a single parameter such as chemical potential. We demonstrate that these EPs are necessary to promote correlation-induced thermodynamic instabilities, such as phase separation occurring in the proximity of a Mott transition, to a topologically stable phenomenon.
Physics Subject Headings (PhySH)
Article Text
Supplemental Material
References (100)
- K. v. Klitzing, G. Dorda, and M. Pepper, New method for high-accuracy determination of the fine-structure constant based on quantized Hall resistance, Phys. Rev. Lett. 45, 494 (1980).
- R. B. Laughlin, Quantized Hall conductivity in two dimensions, Phys. Rev. B 23, 5632(R) (1981).
- B. I. Halperin, Quantized Hall conductance, current-carrying edge states, and the existence of extended states in a two-dimensional disordered potential, Phys. Rev. B 25, 2185 (1982).
- D. J. Thouless, M. Kohmoto, M. P. Nightingale, and M. den Nijs, Quantized Hall conductance in a two-dimensional periodic potential, Phys. Rev. Lett. 49, 405 (1982).
- B. Bernevig and T. Hughes, Topological Insulators and Topological Superconductors (Princeton University Press, Princeton, 2013).
- M. Z. Hasan and C. L. Kane, Colloquium: Topological insulators, Rev. Mod. Phys. 82, 3045 (2010).
- X.-L. Qi and S.-C. Zhang, Topological insulators and superconductors, Rev. Mod. Phys. 83, 1057 (2011).
- X. Chen, Z.-C. Gu, and X.-G. Wen, Local unitary transformation, long-range quantum entanglement, wave function renormalization, and topological order, Phys. Rev. B 82, 155138 (2010).
- S. D. Huber, Topological mechanics, Nat. Phys. 12, 621 (2016).
- B. Bradlyn, L. Elcoro, J. Cano, M. G. Vergniory, Z. Wang, C. Felser, M. I. Aroyo, and B. A. Bernevig, Topological quantum chemistry, Nature (London) 547, 298 (2017).
- T. Ozawa, H. M. Price, A. Amo, N. Goldman, M. Hafezi, L. Lu, M. C. Rechtsman, D. Schuster, J. Simon, O. Zilberberg, and I. Carusotto, Topological photonics, Rev. Mod. Phys. 91, 015006 (2019).
- Z. Gong, Y. Ashida, K. Kawabata, K. Takasan, S. Higashikawa, and M. Ueda, Topological phases of non-Hermitian systems, Phys. Rev. X 8, 031079 (2018).
- Z.-D. Song, L. Elcoro, and B. A. Bernevig, Twisted bulk-boundary correspondence of fragile topology, Science 367, 794 (2020).
- H. Xue, Y. Yang, and B. Zhang, Topological acoustics, Nat. Rev. Mater. 7, 974 (2022).
- E. J. Bergholtz, J. C. Budich, and F. K. Kunst, Exceptional topology of non-Hermitian systems, Rev. Mod. Phys. 93, 015005 (2021).
- G. Rohringer, A. Valli, and A. Toschi, Local electronic correlation at the two-particle level, Phys. Rev. B 86, 125114 (2012).
- P. Thunström, O. Gunnarsson, S. Ciuchi, and G. Rohringer, Analytical investigation of singularities in two-particle irreducible vertex functions of the Hubbard atom, Phys. Rev. B 98, 235107 (2018).
- N. Bickers, Self-consistent many-body theory for condensed matter systems, in Theoretical Methods for Strongly Correlated Electrons (Springer, New York, 2004), pp. 237–296.
- K. Kawabata, K. Shiozaki, M. Ueda, and M. Sato, Symmetry and topology in non-Hermitian physics, Phys. Rev. X 9, 041015 (2019).
- D. Bernard and A. LeClair, A classification of 2D random Dirac fermions, J. Phys. A: Math. Gen. 35, 2555 (2002).
- C.-H. Liu and S. Chen, Topological classification of defects in non-Hermitian systems, Phys. Rev. B 100, 144106 (2019).
- M. V. Berry, Physics of nonhermitian degeneracies, Czech. J. Phys. 54, 1039 (2004).
- W. D. Heiss and H. L. Harney, The chirality of exceptional points, Eur. Phys. J. D 17, 149 (2001).
- W. D. Heiss, The physics of exceptional points, J. Phys. A: Math. Theor. 45, 444016 (2012).
- D. Heiss, Circling exceptional points, Nat. Phys. 12, 823 (2016).
- H. Shen, B. Zhen, and L. Fu, Topological band theory for non-Hermitian Hamiltonians, Phys. Rev. Lett. 120, 146402 (2018).
- K. Kawabata, T. Bessho, and M. Sato, Classification of exceptional points and non-Hermitian topological semimetals, Phys. Rev. Lett. 123, 066405 (2019).
- Z. Yang, A. P. Schnyder, J. Hu, and C.-K. Chiu, Fermion doubling theorems in two-dimensional non-Hermitian systems for Fermi points and exceptional points, Phys. Rev. Lett. 126, 086401 (2021).
- M. Stålhammar and E. J. Bergholtz, Classification of exceptional nodal topologies protected by symmetry, Phys. Rev. B 104, L201104 (2021).
- M. Reitner, P. Chalupa, L. Del Re, D. Springer, S. Ciuchi, G. Sangiovanni, and A. Toschi, Attractive effect of a strong electronic repulsion: The physics of vertex divergences, Phys. Rev. Lett. 125, 196403 (2020).
- G. Kotliar, S. Murthy, and M. J. Rozenberg, Compressibility divergence and the finite temperature Mott transition, Phys. Rev. Lett. 89, 046401 (2002).
- P. Werner and A. J. Millis, Doping-driven Mott transition in the one-band Hubbard model, Phys. Rev. B 75, 085108 (2007).
- M. Eckstein, M. Kollar, M. Potthoff, and D. Vollhardt, Phase separation in the particle-hole asymmetric Hubbard model, Phys. Rev. B 75, 125103 (2007).
- R. Nourafkan, M. Côté, and A.-M. S. Tremblay, Charge fluctuations in lightly hole-doped cuprates: Effect of vertex corrections, Phys. Rev. B 99, 035161 (2019).
- T. Yoshida, R. Peters, and N. Kawakami, Non-Hermitian perspective of the band structure in heavy-fermion systems, Phys. Rev. B 98, 035141 (2018).
- K. Kimura, T. Yoshida, and N. Kawakami, Chiral-symmetry protected exceptional torus in correlated nodal-line semimetals, Phys. Rev. B 100, 115124 (2019).
- R. Aquino and D. G. Barci, Two-dimensional Fermi liquid dynamics with density-density and quadrupolar interactions, Phys. Rev. B 100, 115117 (2019).
- T. Yoshida, R. Peters, N. Kawakami, and Y. Hatsugai, Exceptional band touching for strongly correlated systems in equilibrium, Prog. Theor. Exp. Phys. 2020, 12A109 (2020).
- R. Aquino and D. G. Barci, Exceptional points in Fermi liquids with quadrupolar interactions, Phys. Rev. B 102, 201110 (2020).
- Y. Nagai, Y. Qi, H. Isobe, V. Kozii, and L. Fu, DMFT reveals the non-Hermitian topology and Fermi arcs in heavy-fermion systems, Phys. Rev. Lett. 125, 227204 (2020).
- R. Rausch, R. Peters, and T. Yoshida, Exceptional points in the one-dimensional Hubbard model, New J. Phys. 23, 013011 (2021).
- C. Lehmann, M. Schüler, and J. C. Budich, Dynamically induced exceptional phases in quenched interacting semimetals, Phys. Rev. Lett. 127, 106601 (2021).
- L. Crippa, G. Sangiovanni, and J. C. Budich, Spontaneous formation of exceptional points at the onset of magnetism, Phys. Rev. Lett. 130, 186403 (2023).
- B. Michen, T. Micallo, and J. C. Budich, Exceptional non-Hermitian phases in disordered quantum wires, Phys. Rev. B 104, 035413 (2021).
- B. Michen and J. C. Budich, Mesoscopic transport signatures of disorder-induced non-Hermitian phases, Phys. Rev. Res. 4, 023248 (2022).
- M.-A. Miri and A. Alù, Exceptional points in optics and photonics, Science 363, eaar7709 (2019).
- S. Weimann, M. Kremer, Y. Plotnik, Y. Lumer, S. Nolte, K. G. Makris, M. Segev, M. C. Rechtsman, and A. Szameit, Topologically protected bound states in photonic parity–time-symmetric crystals, Nat. Mater. 16, 433 (2017).
- K. Takata and M. Notomi, Photonic topological insulating phase induced solely by gain and loss, Phys. Rev. Lett. 121, 213902 (2018).
- Y. Zhiyenbayev, Y. Kominis, C. Valagiannopoulos, V. Kovanis, and A. Bountis, Enhanced stability, bistability, and exceptional points in saturable active photonic couplers, Phys. Rev. A 100, 043834 (2019).
- Y. Ashida, Z. Gong, and M. Ueda, Non-Hermitian physics, Adv. Phys. 69, 249 (2020).
- S. Weidemann, M. Kremer, T. Helbig, T. Hofmann, A. Stegmaier, M. Greiter, R. Thomale, and A. Szameit, Topological funneling of light, Science 368, 311 (2020).
- H. Menke and M. M. Hirschmann, Topological quantum wires with balanced gain and loss, Phys. Rev. B 95, 174506 (2017).
- G. Rohringer, H. Hafermann, A. Toschi, A. A. Katanin, A. E. Antipov, M. I. Katsnelson, A. I. Lichtenstein, A. N. Rubtsov, and K. Held, Diagrammatic routes to nonlocal correlations beyond dynamical mean field theory, Rev. Mod. Phys. 90, 025003 (2018).
- Here we have shortened the notation of the Fourier transform of the time-ordered operators to make their properties in the following derivations more transparent, in Eq. (1) the time ordering is acting first on the time arguments of the operators and then the respective integrals are performed.
- G. Rohringer, New routes toward a theoretical treatment of nonlocal electronic correlations, Ph.D. thesis, Technischen Universität Wien, 2014.
- D. Springer, P. Chalupa, S. Ciuchi, G. Sangiovanni, and A. Toschi, Interplay between local response and vertex divergences in many-fermion systems with on-site attraction, Phys. Rev. B 101, 155148 (2020).
- A detailed derivation can be found in the Supplemental Material [67].
- R. D. Hill and S. R. Waters, On -real and -Hermitian matrices, Linear Algebra Appl. 169, 17 (1992).
- A. Lee, Centrohermitian and skew-centrohermitian matrices, Linear Algebra Appl. 29, 205 (1980), Special Volume Dedicated to Alson S. Householder.
- R. D. Hill, R. G. Bates, and S. R. Waters, On centrohermitian matrices, SIAM J. Matrix Anal. Appl. 11, 128 (1990).
- J. C. Budich, J. Carlström, F. K. Kunst, and E. J. Bergholtz, Symmetry-protected nodal phases in non-Hermitian systems, Phys. Rev. B 99, 041406 (2019).
- See the Supplemental Material for a short discussion on the differences between the susceptibility matrix properties of Fermi-Dirac and Bose-Einstein statistics [67].
- For the effect of the -symmetry on the generalized susceptibilities, see Refs. [16, 18].
- S. Pairault, D. Sénéchal, and A.-M. S. Tremblay, Strong-coupling perturbation theory of the Hubbard model, Eur. Phys. J. B 16, 85 (2000).
- D. R. Fus, Breakdown of the many-electron perturbation expansion beyond particle-hole symmetry: An atomic limit study, Bachelor thesis, Technischen Universität Wien, 2022.
- H. Eßl, M. Reitner, G. Sangiovanni, and A. Toschi, General shiba mapping for on-site four-point correlation functions, arXiv:2402.16115 [cond-mat.str-el].
- See Supplemental Material at http://link.aps.org/supplemental/10.1103/PhysRevResearch.6.L022031 for more details on the symmetry properties of the generalized susceptibilities and further information.
- W. Metzner and D. Vollhardt, Correlated lattice fermions in dimensions, Phys. Rev. Lett. 62, 324 (1989).
- A. Georges, G. Kotliar, W. Krauth, and M. J. Rozenberg, Dynamical mean-field theory of strongly correlated fermion systems and the limit of infinite dimensions, Rev. Mod. Phys. 68, 13 (1996).
- M. Wallerberger, A. Hausoel, P. Gunacker, A. Kowalski, N. Parragh, F. Goth, K. Held, and G. Sangiovanni, w2dynamics: Local one- and two-particle quantities from dynamical mean field theory, Comput. Phys. Commun. 235, 388 (2019).
- A. Kowalski, M. Reitner, L. D. Re, M. Chatzieleftheriou, A. Amaricci, A. Toschi, L. de' Medici, G. Sangiovanni, and T. Schäfer, Thermodynamic stability at the two-particle level, arXiv:2309.11108 [cond-mat.str-el].
- Further, the corresponding weight must be , which is, in general, fulfilled away from PHS for [30].
- A schematic illustration of this regime can be found in the Supplemental Material [67].
- P. Chalupa, T. Schäfer, M. Reitner, D. Springer, S. Andergassen, and A. Toschi, Fingerprints of the local moment formation and its Kondo screening in the generalized susceptibilities of many-electron problems, Phys. Rev. Lett. 126, 056403 (2021).
- T. B. Mazitov and A. A. Katanin, Local magnetic moment formation and Kondo screening in the half-filled single-band Hubbard model, Phys. Rev. B 105, L081111 (2022).
- T. B. Mazitov and A. A. Katanin, Effect of local magnetic moments on spectral properties and resistivity near interaction- and doping-induced Mott transitions, Phys. Rev. B 106, 205148 (2022).
- S. Adler, F. Krien, P. Chalupa-Gantner, G. Sangiovanni, and A. Toschi, Non-perturbative intertwining between spin and charge correlations: A “smoking gun” single-boson-exchange result, SciPost Phys. 16, 054 (2024).
- T. Schäfer, G. Rohringer, O. Gunnarsson, S. Ciuchi, G. Sangiovanni, and A. Toschi, Divergent precursors of the Mott-Hubbard transition at the two-particle level, Phys. Rev. Lett. 110, 246405 (2013).
- V. Janiš and V. Pokorný, Critical metal-insulator transition and divergence in a two-particle irreducible vertex in disordered and interacting electron systems, Phys. Rev. B 90, 045143 (2014).
- E. Kozik, M. Ferrero, and A. Georges, Nonexistence of the Luttinger-Ward functional and misleading convergence of skeleton diagrammatic series for Hubbard-like models, Phys. Rev. Lett. 114, 156402 (2015).
- A. Stan, P. Romaniello, S. Rigamonti, L. Reining, and J. A. Berger, Unphysical and physical solutions in many-body theories: from weak to strong correlation, New J. Phys. 17, 093045 (2015).
- R. Rossi and F. Werner, Skeleton series and multivaluedness of the self-energy functional in zero space-time dimensions, J. Phys. A: Math. Theor. 48, 485202 (2015).
- T. Ribic, G. Rohringer, and K. Held, Nonlocal correlations and spectral properties of the Falicov-Kimball model, Phys. Rev. B 93, 195105 (2016).
- R. Rossi, F. Werner, N. Prokof'ev, and B. Svistunov, Shifted-action expansion and applicability of dressed diagrammatic schemes, Phys. Rev. B 93, 161102(R) (2016).
- O. Gunnarsson, T. Schäfer, J. P. F. LeBlanc, J. Merino, G. Sangiovanni, G. Rohringer, and A. Toschi, Parquet decomposition calculations of the electronic self-energy, Phys. Rev. B 93, 245102 (2016).
- T. Schäfer, S. Ciuchi, M. Wallerberger, P. Thunström, O. Gunnarsson, G. Sangiovanni, G. Rohringer, and A. Toschi, Nonperturbative landscape of the Mott-Hubbard transition: Multiple divergence lines around the critical endpoint, Phys. Rev. B 94, 235108 (2016).
- O. Gunnarsson, G. Rohringer, T. Schäfer, G. Sangiovanni, and A. Toschi, Breakdown of traditional many-body theories for correlated electrons, Phys. Rev. Lett. 119, 056402 (2017).
- W. Tarantino, B. S. Mendoza, P. Romaniello, J. A. Berger, and L. Reining, Many-body perturbation theory and non-perturbative approaches: screened interaction as the key ingredient, J. Phys.: Condens. Matter 30, 135602 (2018).
- J. Vučičević, N. Wentzell, M. Ferrero, and O. Parcollet, Practical consequences of the Luttinger-Ward functional multivaluedness for cluster DMFT methods, Phys. Rev. B 97, 125141 (2018).
- P. Chalupa, P. Gunacker, T. Schäfer, K. Held, and A. Toschi, Divergences of the irreducible vertex functions in correlated metallic systems: Insights from the Anderson impurity model, Phys. Rev. B 97, 245136 (2018).
- C. Melnick and G. Kotliar, Fermi-liquid theory and divergences of the two-particle irreducible vertex in the periodic Anderson lattice, Phys. Rev. B 101, 165105 (2020).
- A. J. Kim and V. Sacksteder, Multivaluedness of the Luttinger-Ward functional in the fermionic and bosonic system with replicas, Phys. Rev. B 101, 115146 (2020).
- E. G. C. P. van Loon, F. Krien, and A. A. Katanin, Bethe-Salpeter equation at the critical end point of the Mott transition, Phys. Rev. Lett. 125, 136402 (2020).
- K. Van Houcke, E. Kozik, R. Rossi, Y. Deng, and F. Werner, Physical and unphysical regimes of self-consistent many-body perturbation theory, arXiv:2102.04508 [cond-mat.str-el].
- E. A. Stepanov, S. Brener, V. Harkov, M. I. Katsnelson, and A. I. Lichtenstein, Spin dynamics of itinerant electrons: Local magnetic moment formation and berry phase, Phys. Rev. B 105, 155151 (2022).
- E. G. C. P. van Loon, Two-particle correlations and the metal-insulator transition: Iterated perturbation theory revisited, Phys. Rev. B 105, 245104 (2022).
- A. J. Kim and E. Kozik, Misleading convergence of the skeleton diagrammatic technique: when the correct solution can be found, arXiv:2212.14768 [cond-mat.str-el].
- M. Pelz, S. Adler, M. Reitner, and A. Toschi, Highly nonperturbative nature of the Mott metal-insulator transition: Two-particle vertex divergences in the coexistence region, Phys. Rev. B 108, 155101 (2023).
- L. Del Re and G. Rohringer, Fluctuations analysis of spin susceptibility: Néel ordering revisited in dynamical mean field theory, Phys. Rev. B 104, 235128 (2021).
- In contrast, for the situation of the generalized susceptibility in the channel, see the Supplemental Material [67].