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  • Letter
  • Open Access

Optical spin readout of single rubidium atoms trapped in solid neon

David M. Lancaster, Ugne Dargyte, and Jonathan D. Weinstein*

  • Department of Physics, University of Nevada, Reno NV 89557, USA

  • *weinstein@physics.unr.edu; https://www.weinsteinlab.org

Phys. Rev. Research 6, L012048 – Published 1 March, 2024

DOI: https://doi.org/10.1103/PhysRevResearch.6.L012048

Abstract

In this work, we optically resolve and detect individual rubidium atoms trapped in solid neon. Additionally, we optically pump the rubidium's spin state using polarized light and measure the spin state via laser-induced fluorescence. When combined with the previously demonstrated magnetic field sensing capabilities of matrix-isolated rubidium atoms, these results are very promising for nanoscale sensing and for performing nuclear magnetic resonance (NMR) spectroscopy of individual molecules cotrapped in the matrix.

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References (35)

  1. C. L. Degen, F. Reinhard, and P. Cappellaro, Quantum sensing, Rev. Mod. Phys. 89, 035002 (2017).
  2. J. R. Maze, P. L. Stanwix, J. S. Hodges, S. Hong, J. M. Taylor, P. Cappellaro, L. Jiang, M. V. Gurudev Dutt, E. Togan, A. S. Zibrov, A. Yacoby, R. L. Walsworth, and M. D. Lukin, Nanoscale magnetic sensing with an individual electronic spin in diamond, Nature (London) 455, 644 (2008).
  3. C. L. Degen, Scanning magnetic field microscope with a diamond single-spin sensor, Appl. Phys. Lett. 92, 243111 (2008).
  4. A. Ajoy, U. Bissbort, M. D. Lukin, R. L. Walsworth, and P. Cappellaro, Atomic-scale nuclear spin imaging using quantum-assisted sensors in diamond, Phys. Rev. X 5, 011001 (2015).
  5. S. Kolkowitz, Q. P. Unterreithmeier, S. D. Bennett, and M. D. Lukin, Sensing distant nuclear spins with a single electron spin, Phys. Rev. Lett. 109, 137601 (2012).
  6. T. H. Taminiau, J. J. T. Wagenaar, T. van der Sar, F. Jelezko, V. V. Dobrovitski, and R. Hanson, Detection and control of individual nuclear spins using a weakly coupled electron spin, Phys. Rev. Lett. 109, 137602 (2012).
  7. N. Zhao, J. Honert, B. Schmid, M. Klas, J. Isoya, M. Markham, D. Twitchen, F. Jelezko, R.-B. Liu, H. Fedder, and J. Wrachtrup, Sensing single remote nuclear spins, Nat. Nanotechnol. 7, 657 (2012).
  8. M. H. Abobeih, J. Randall, C. E. Bradley, H. P. Bartling, M. A. Bakker, M. J. Degen, M. Markham, D. J. Twitchen, and T. H. Taminiau, Atomic-scale imaging of a 27-nuclear-spin cluster using a quantum sensor, Nature (London) 576, 411 (2019).
  9. I. Lovchinsky, A. Sushkov, E. Urbach, N. P. de Leon, S. Choi, K. De Greve, R. Evans, R. Gertner, E. Bersin, C. Müller et al., Nuclear magnetic resonance detection and spectroscopy of single proteins using quantum logic, Science 351, 836 (2016).
  10. V. S. Perunicic, C. D. Hill, L. T. Hall, and L. C. L. Hollenberg, A quantum spin-probe molecular microscope, Nat. Commun. 7, 12667 (2016).
  11. B. L. Dwyer, L. V. H. Rodgers, E. K. Urbach, D. Bluvstein, S. Sangtawesin, H. Zhou, Y. Nassab, M. Fitzpatrick, Z. Yuan, K. De Greve, E. L. Peterson, H. Knowles, T. Sumarac, J.-P. Chou, A. Gali, V. V. Dobrovitski, M. D. Lukin, and N. P. de Leon, Probing spin dynamics on diamond surfaces using a single quantum sensor, PRX Quantum 3, 040328 (2022).
  12. E. Janitz, K. Herb, L. A. Völker, W. S. Huxter, C. L. Degen, and J. M. Abendroth, Diamond surface engineering for molecular sensing with nitrogenvacancy centers, J. Mater. Chem. C 10, 13533 (2022).
  13. Z. Yuan, L. V. H. Rodgers, J. Rovny, S. Sangtawesin, S. Srinivasan, J. Allred, N. P. de Leon, and P. Gumann, Ultrahigh vacuum surface chemistry for nanoscale sensors in diamond, in Quantum 2.0 Conference and Exhibition, Technical Digest Series (Optica Publishing Group, Boston, MA, 2022), paper QTu2A.11.
  14. S. Upadhyay, U. Dargyte, D. Patterson, and J. D. Weinstein, Ultralong spin-coherence times for rubidium atoms in solid parahydrogen via dynamical decoupling, Phys. Rev. Lett. 125, 043601 (2020).
  15. A. Kaczor, I. D. Reva, L. M. Proniewicz, and R. Fausto, Matrix-Isolated monomeric tryptophan: Electrostatic interactions as nontrivial factors stabilizing conformers, J. Phys. Chem. A 111, 2957 (2007).
  16. A. Kaczor, I. D. Reva, L. M. Proniewicz, and R. Fausto, Importance of entropy in the conformational equilibrium of phenylalanine: A matrix-isolation infrared spectroscopy and density functional theory study, J. Phys. Chem. A 110, 2360 (2006).
  17. S. G. Stepanian, I. D. Reva, E. D. Radchenko, and L. Adamowicz, Conformational behavior of α-alanine. matrix-isolation infrared and theoretical DFT and ab initio study, J. Phys. Chem. A 102, 4623 (1998).
  18. D. M. Lancaster, U. Dargyte, S. Upadhyay, and J. D. Weinstein, Radiative properties of rubidium atoms trapped in solid neon and parahydrogen, Phys. Rev. A 103, 052614 (2021).
  19. U. Dargyte, D. M. Lancaster, and J. D. Weinstein, Optical and spin-coherence properties of rubidium atoms trapped in solid neon, Phys. Rev. A 104, 032611 (2021).
  20. C. Chambers, T. Walton, D. Fairbank, A. Craycraft, D. Yahne, J. Todd, A. Iverson, W. Fairbank, A. Alamre, J. Albert et al. (nEXO Collaboration), Imaging individual barium atoms in solid xenon for barium tagging in nEXO, Nature (London) 569, 203 (2019).
  21. A. N. Kanagin, S. K. Regmi, P. Pathak, and J. D. Weinstein, Optical pumping of rubidium atoms frozen in solid argon, Phys. Rev. A 88, 063404 (2013).
  22. S. M. Mansfield and G. Kino, Solid immersion microscope, Appl. Phys. Lett. 57, 2615 (1990).
  23. W. S. Bakr, J. I. Gillen, A. Peng, S. Fölling, and M. Greiner, A quantum gas microscope for detecting single atoms in a Hubbard-regime optical lattice, Nature (London) 462, 74 (2009).
  24. I. Gerhardt, K. Sin, and T. Momose, Excitation and emission spectra of rubidium in rare-gas thin-films, J. Chem. Phys. 137, 014507 (2012).
  25. S. Upadhyay, U. Dargyte, V. D. Dergachev, R. P. Prater, S. A. Varganov, T. V. Tscherbul, D. Patterson, and J. D. Weinstein, Spin coherence and optical properties of alkali-metal atoms in solid parahydrogen, Phys. Rev. A 100, 063419 (2019).
  26. S. L. Kupferman and F. M. Pipkin, Properties of rubidium atoms trapped in a solid argon matrix, Phys. Rev. 166, 207 (1968).
  27. J. E. Sansonetti, W. C. Martin, and S. L. Young, Handbook of Basic Atomic Spectroscopic Data (version 1.1.3) (NIST, 2013) http://physics.nist.gov/PhysRefData/Handbook/.
  28. J. F. Barry, J. M. Schloss, E. Bauch, M. J. Turner, C. A. Hart, L. M. Pham, and R. L. Walsworth, Sensitivity optimization for NV-diamond magnetometry, Rev. Mod. Phys. 92, 015004 (2020).
  29. Z. Yuan, M. Fitzpatrick, L. V. H. Rodgers, S. Sangtawesin, S. Srinivasan, and N. P. de Leon, Charge state dynamics and optically detected electron spin resonance contrast of shallow nitrogen-vacancy centers in diamond, Phys. Rev. Res. 2, 033263 (2020).
  30. J.-C. Jaskula, B. J. Shields, E. Bauch, M. D. Lukin, A. S. Trifonov, and R. L. Walsworth, Improved quantum sensing with a single solid-state spin via spin-to-charge conversion, Phys. Rev. Appl. 11, 064003 (2019).
  31. J. Taylor, P. Cappellaro, L. Childress, L. Jiang, D. Budker, P. Hemmer, A. Yacoby, R. Walsworth, and M. Lukin, High-sensitivity diamond magnetometer with nanoscale resolution, Nat. Phys. 4, 810 (2008).
  32. S. L. Bayliss, P. Deb, D. W. Laorenza, M. Onizhuk, G. Galli, D. E. Freedman, and D. D. Awschalom, Enhancing spin coherence in optically addressable molecular qubits through host-matrix control, Phys. Rev. X 12, 031028 (2022).
  33. L. Robledo, L. Childress, H. Bernien, B. Hensen, P. F. Alkemade, and R. Hanson, High-fidelity projective read-out of a solid-state spin quantum register, Nature (London) 477, 574 (2011).
  34. B. J. Shields, Q. P. Unterreithmeier, N. P. de Leon, H. Park, and M. D. Lukin, Efficient readout of a single spin state in diamond via spin-to-charge conversion, Phys. Rev. Lett. 114, 136402 (2015).
  35. J. M. Martinis, Qubit metrology for building a fault-tolerant quantum computer, npj Quantum Inf. 1, 15005 (2015).

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