- Letter
- Open Access
Characterization of ionization using the circular dichroic phase
Phys. Rev. Research 6, L012002 – Published 3 January, 2024
DOI: https://doi.org/10.1103/PhysRevResearch.6.L012002
Abstract
A strong helicity dependence of reconstruction of attosecond bursts by beating of two-photon transitions (RABBITT) with circularly polarized XUV and IR pulses was reported by Han et al. [Nat. Phys. 19, 230 (2023) and arXiv:2302.04137]. They attributed a circular dichroic phase in RABBITT to the helical structure of the photoelectron wave packets in the final state. We exploit this effect to determine the magnitude and phase of two-photon ionization amplitudes. In -electron targets (H, He, Li), such a determination is fully ab initio and requires no further approximations. In heavier noble gases like Ar, characterization of two-photon ionization amplitudes can be made from the circular dichroic phase with minimal and very realistic assumptions.
Physics Subject Headings (PhySH)
Corrections
15 February, 2024
Correction: A source in the abstract and in Ref. [7] contained an incorrect article ID and has been fixed.
Article Text
References (30)
- R. Cireasa, A. E. Boguslavskiy, B. Pons, M. C. H. Wong, D. Descamps, S. Petit, H. Ruf, N. Thiré, A. Ferré, J. Suarez et al., Probing molecular chirality on a sub-femtosecond timescale, Nat. Phys. 11, 654 (2015).
- I. Barth and O. Smirnova, Nonadiabatic tunneling in circularly polarized laser fields: Physical picture and calculations, Phys. Rev. A 84, 063415 (2011).
- I. Barth and O. Smirnova, Spin-polarized electrons produced by strong-field ionization, Phys. Rev. A 88, 013401 (2013).
- S. Walker, L. Kolanz, J. Venzke, and A. Becker, Selectivity in electron emission induced by ultrashort circularly polarized laser pulses, Phys. Rev. Res. 3, 043051 (2021).
- I. A. Ivanov and A. S. Kheifets, Time delay in atomic photoionization with circularly polarized light, Phys. Rev. A 87, 033407 (2013).
- N. Mayer, S. Patchkovskii, F. Morales, M. Ivanov, and O. Smirnova, Imprinting chirality on atoms using synthetic chiral light fields, Phys. Rev. Lett. 129, 243201 (2022).
- M. Han, J.-B. Ji, T. Balčiūnas, K. Ueda, and H. J. Wörner, Attosecond circular-dichroism chronoscopy of electron vortices, Nat. Phys. 19, 230 (2023).
- M. Han, J.-B. Ji, L. C. Sum, K. Ueda, and H. J. Wörner, Separation of Wigner and continuum-continuum delays by mirror-symmetry-broken attosecond interferometry, arXiv:2302.04137.
- E. Shigemasa, J. Adachi, K. Soejima, N. Watanabe, A. Yagishita, and N. A. Cherepkov, Direct determination of partial wave contributions in the shape resonance of CO molecules, Phys. Rev. Lett. 80, 1622 (1998).
- Z.-M. Wang and D. S. Elliot, Determination of cross sections and continuum phases of rubidium through complete measurements of atomic multiphoton ionization, Phys. Rev. Lett. 84, 3795 (2000).
- P. M. Paul, E. S. Toma, P. Breger, G. Mullot, F. Augé, P. Balcou, H. G. Muller, and P. Agostini, Observation of a train of attosecond pulses from high harmonic generation, Science 292, 1689 (2001).
- Y. Mairesse, A. de Bohan, L. J. Frasinski, H. Merdji, L. C. Dinu, P. Monchicourt, P. Breger, M. Kovacev, R. Taïeb, B. Carré et al., Attosecond synchronization of high-harmonic soft x-rays, Science 302, 1540 (2003).
- J. M. Dahlström et al., Theory of attosecond delays in laser-assisted photoionization, Chem. Phys. 414, 53 (2013).
- J. Sörngard, J. M. Dahlström, and E. Lindroth, Study of the possibilities with combinations of circularly and linearly polarized light for attosecond delay investigations, J. Phys. B 53, 134003 (2020).
- U. Fano, Propensity rules: An analytical approach, Phys. Rev. A 32, 617 (1985).
- D. Busto, J. Vinbladh, S. Zhong, M. Isinger, S. Nandi, S. Maclot, P. Johnsson, M. Gisselbrecht, A. L'Huillier, E. Lindroth et al., Fano's propensity rule in angle-resolved attosecond pump-probe photoionization, Phys. Rev. Lett. 123, 133201 (2019).
- D. I. R. Boll, L. Martini, A. Palacios, and O. A. Fojón, Two-color polarization control of angularly resolved attosecond time delays, Phys. Rev. A 107, 043113 (2023).
- A. S. Kheifets, Under-threshold RABBITT in argon, J. Phys. B 56, 095201 (2023).
- A. S. Kheifets and Z. Xu, Polarization control of RABBITT in noble gas atoms, J. Phys. B 56, 155601 (2023).
- W. Jiang, G. S. J. Armstrong, J. Tong, Y. Xu, Z. Zuo, J. Qiang, P. Lu, D. D. A. Clarke, J. Benda, A. Fleischer et al., Atomic partial wave meter by attosecond coincidence metrology, Nat. Commun. 13, 5072 (2022).
- S. Heuser, A. Jiménez Galán, C. Cirelli, C. Marante, M. Sabbar, R. Boge, M. Lucchini, L. Gallmann, I. Ivanov, A. S. Kheifets et al., Angular dependence of photoemission time delay in helium, Phys. Rev. A 94, 063409 (2016).
- I. A. Ivanov and A. S. Kheifets, Angle-dependent time delay in two-color photoemission of He and Ne, Phys. Rev. A 96, 013408 (2017).
- T. Mazza, M. Ilchen, A. J. Rafipoor, C. Callegari, P. Finetti, O. Plekan, K. C. Prince, R. Richter, M. B. Danailov, A. Demidovich et al., Determining the polarization state of an extreme ultraviolet free-electron laser beam using atomic circular dichroism, Nat. Commun. 5, 3648 (2014).
- M. Swoboda, T. Fordell, K. Klünder, J. M. Dahlström, M. Miranda, C. Buth, K. J. Schafer, J. Mauritsson, A. L'Huillier, and M. Gisselbrecht, Phase measurement of resonant two-photon ionization in helium, Phys. Rev. Lett. 104, 103003 (2010).
- L. Drescher, T. Witting, O. Kornilov, and M. J. J. Vrakking, Phase dependence of resonant and antiresonant two-photon excitations, Phys. Rev. A 105, L011101 (2022).
- L. Neoriĉić, D. Busto, H. Laurell, R. Weissenbilder, M. Ammitzböll, S. Luo, J. Peschel, H. Wikmark, J. Lahl, S. Maclot et al., Resonant two-photon ionization of helium atoms studied by attosecond interferometry, Front. Phys. 10 (2022).
- A. Autuori, D. Platzer, M. Lejman, G. Gallician, L. Maëder, A. Covolo, L. Bosse, M. Dalui, D. Bresteau, J.-F. Hergott et al., Anisotropic dynamics of two-photon ionization: An attosecond movie of photoemission, Sci. Adv. 8, eabl7594 (2022).
- D. M. Villeneuve, P. Hockett, M. J. J. Vrakking, and H. Niikura, Coherent imaging of an attosecond electron wave packet, Science 356, 1150 (2017).
- A. S. Kheifets and A. W. Bray, RABBITT phase transition across the ionization threshold, Phys. Rev. A 103, L011101 (2021).
- A. Kheifets, Revealing the target electronic structure with under-threshold RABBITT, Atoms 9, 66 (2021).