- Letter
- Open Access
Giant optomechanical coupling and dephasing protection with cavity exciton-polaritons
Phys. Rev. Research 5, L042035 – Published 7 December, 2023
DOI: https://doi.org/10.1103/PhysRevResearch.5.L042035
Abstract
Electronic resonances can significantly enhance photon-phonon coupling but are normally avoided in cavity optomechanics due to absorption losses and dephasing by inhomogeneous broadening. We demonstrate experimentally that exciton-polaritons in semiconductor microcavities enable single-particle resonant optomechanical couplings with GHz vibrations reaching record values in the tens of MHz range. Moreover, this resonant enhancement is protected from inhomogeneous broadening by the Rabi gap. Single-polariton nonlinearities and the optomechanical strong-coupling regime become accessible in this platform.
Physics Subject Headings (PhySH)
Article Text
Supplemental Material
References (44)
- M. Aspelmeyer, T. J. Kippenberg, and F. Marquardt, Cavity optomechanics, Rev. Mod. Phys. 86, 1391 (2014).
- P. Forn-Díaz, L. Lamata, E. Rico, J. Kono, and E. Solano, Ultrastrong coupling regimes of light-matter interaction, Rev. Mod. Phys. 91, 025005 (2019).
- A. Frisk Kockum, A. Miranowicz, S. De Liberato, S. Savasta, and F. Nori, Ultrastrong coupling between light and matter, Nat. Rev. Phys. 1, 19 (2019).
- S. Hughes, A. Settineri, S. Savasta, and F. Nori, Resonant Raman scattering of single molecules under simultaneous strong cavity coupling and ultrastrong optomechanical coupling in plasmonic resonators: Phonon-dressed polaritons, Phys. Rev. B 104, 045431 (2021).
- P. F. Cohadon, A. Heidmann, and M. Pinard, Cooling of a mirror by radiation pressure, Phys. Rev. Lett. 83, 3174 (1999).
- C. Baker, W. Hease, D.-T. Nguyen, A. Andronico, S. Ducci, G. Leo, and I. Favero, Photoelastic coupling in gallium arsenide optomechanical disk resonators, Opt. Express 22, 14072 (2014).
- M. Rossi, D. Mason, J. Chen, Y. Tsaturyan, and A. Schliesser, Measurement-based quantum control of mechanical motion, Nature (London) 563, 53 (2018).
- H. Ren, M. H. Matheny, G. S. MacCabe, J. Luo, H. Pfeifer, M. Mirhosseini, and O. Painter, Two-dimensional optomechanical crystal cavity with high quantum cooperativity, Nat. Commun. 11, 3373 (2020).
- B. Jusserand, A. N. Poddubny, A. V. Poshakinskiy, A. Fainstein, and A. Lemaître, Polariton resonances for ultrastrong coupling cavity optomechanics in GaAs-AlAs multiple quantum wells, Phys. Rev. Lett. 115, 267402 (2015).
- P. T. Rakich, P. Davids, and Z. Wang, Tailoring optical forces in waveguides through radiation pressure and electrostrictive forces, Opt. Express 18, 14439 (2010).
- P. T. Rakich, C. Reinke, R. Camacho, P. Davids, and Z. Wang, Giant enhancement of stimulated brillouin scattering in the subwavelength limit, Phys. Rev. X 2, 011008 (2012).
- A. Fainstein, N. D. Lanzillotti-Kimura, B. Jusserand, and B. Perrin, Strong optical-mechanical coupling in a vertical GaAs/AlAs microcavity for subterahertz phonons and near-infrared light, Phys. Rev. Lett. 110, 037403 (2013).
- P. E. Allain, B. Guha, C. Baker, D. Parrain, A. Lemaître, G. Leo, and I. Favero, Electro-optomechanical modulation instability in a semiconductor resonator, Phys. Rev. Lett. 126, 243901 (2021).
- M. Kobecki, A. V. Scherbakov, S. M. Kukhtaruk, D. D. Yaremkevich, T. Henksmeier, A. Trapp, D. Reuter, V. E. Gusev, A. V. Akimov, and M. Bayer, Giant photoelasticity of polaritons for detection of coherent phonons in a superlattice with quantum sensitivity, Phys. Rev. Lett. 128, 157401 (2022).
- I. Carusotto and C. Ciuti, Quantum fluids of light, Rev. Mod. Phys. 85, 299 (2013).
- O. Kyriienko, T. C. H. Liew, and I. A. Shelykh, Optomechanics with cavity polaritons: Dissipative coupling and unconventional bistability, Phys. Rev. Lett. 112, 076402 (2014).
- J. Restrepo, C. Ciuti, and I. Favero, Single-polariton optomechanics, Phys. Rev. Lett. 112, 013601 (2014).
- J. Restrepo, I. Favero, and C. Ciuti, Fully coupled hybrid cavity optomechanics: Quantum interferences and correlations, Phys. Rev. A 95, 023832 (2017).
- E. S. Vyatkin and A. N. Poddubny, Optomechanical amplification driven by interference of phonon-exciton and phonon-photon couplings, Phys. Rev. B 104, 075447 (2021).
- D. L. Chafatinos, A. S. Kuznetsov, S. Anguiano, A. E. Bruchhausen, A. A. Reynoso, K. Biermann, P. V. Santos, and A. Fainstein, Polariton-driven phonon laser, Nat. Commun. 11, 4552 (2020).
- A. A. Reynoso, G. Usaj, D. L. Chafatinos, F. Mangussi, A. E. Bruchhausen, A. S. Kuznetsov, K. Biermann, P. V. Santos, and A. Fainstein, Optomechanical parametric oscillation of a quantum light-fluid in a lattice, Phys. Rev. B 105, 195310 (2022).
- D. L. Chafatinos, A. S. Kuznetsov, P. Sesin, I. Papuccio, A. A. Reynoso, A. E. Bruchhausen, G. Usaj, K. Biermann, P. V. Santos, and A. Fainstein, Asynchronous locking in metamaterials of fluids of light and sound, Nat. Commun. 14, 3485 (2023).
- N. Carlon Zambon, Z. Denis, R. De Oliveira, S. Ravets, C. Ciuti, I. Favero, and J. Bloch, Enhanced cavity optomechanics with quantum-well exciton polaritons, Phys. Rev. Lett. 129, 093603 (2022).
- I. Diniz, S. Portolan, R. Ferreira, J. M. Gerard, P. Bertet, and A. Auffeves, Strongly coupling a cavity to inhomogeneous ensembles of emitters: Potential for long-lived solid-state quantum memories, Phys. Rev. A 84, 063810 (2011).
- S. Putz, D. O. Krimer, R. Amsüss, A. Valookaran, T. Nöbauer, J. Schmiedmayer, S. Rotter, and J. Majer, Protecting a spin ensemble against decoherence in the strong-coupling regime of cavity QED, Nat. Phys. 10, 720 (2014).
- M. Trigo, A. Bruchhausen, A. Fainstein, B. Jusserand, and V. Thierry-Mieg, Confinement of acoustical vibrations in a semiconductor planar phonon cavity, Phys. Rev. Lett. 89, 227402 (2002).
- See Supplemental Material at http://link.aps.org/supplemental/10.1103/PhysRevResearch.5.L042035 for a detailed description of the studied samples and their characterization, the experimental setups, and the models used to evaluate and the Brillouin efficiency.
- A. S. Kuznetsov, D. H. O. Machado, K. Biermann, and P. V. Santos, Electrically driven microcavity exciton-polariton optomechanics at 20 GHz, Phys. Rev. X 11, 021020 (2021).
- D. H. O. Machado, A. Crespo-Poveda, A. S. Kuznetsov, K. Biermann, L. V. A. Scalvi, and P. V. Santos, Generation and propagation of superhigh-frequency bulk acoustic waves in GaAs, Phys. Rev. Appl. 12, 044013 (2019).
- B. Jusserand and M. Cardona, in Light Scattering in Solids V, edited by M. Cardona and G. Güntherodt (Springer, Heidelberg, 1989).
- A. Fainstein, B. Jusserand, and V. Thierry-Mieg, Raman scattering enhancement by optical confinement in a semiconductor planar microcavity, Phys. Rev. Lett. 75, 3764 (1995).
- G. Rozas, A. E. Bruchhausen, A. Fainstein, B. Jusserand, and A. Lemaître, Polariton path to fully resonant dispersive coupling in optomechanical resonators, Phys. Rev. B 90, 201302(R) (2014).
- S. Anguiano, A. E. Bruchhausen, B. Jusserand, I. Favero, F. R. Lamberti, L. Lanco, I. Sagnes, A. Lemaître, N. D. Lanzillotti-Kimura, P. Senellart, and A. Fainstein, Micropillar resonators for optomechanics in the extremely high 19–95-GHz frequency range, Phys. Rev. Lett. 118, 263901 (2017).
- F. R. Lamberti, Q. Yao, L. Lanco, D. T. Nguyen, M. Esmann, A. Fainstein, P. Sesin, S. Anguiano, V. Villafañe, A. Bruchhausen, P. Senellart, I. Favero, and N. D. Lanzillotti-Kimura, Optomechanical properties of GaAs/AlAs micropillar resonators operating in the 18 GHz range, Opt. Express 25, 24437 (2017).
- V. Villafañe, P. Sesin, P. Soubelet, S. Anguiano, A. E. Bruchhausen, G. Rozas, C. Gomez Carbonell, A. Lemaître, and A. Fainstein, Optoelectronic forces with quantum wells for cavity optomechanics in GaAs/AlAs semiconductor microcavities, Phys. Rev. B 97, 195306 (2018).
- A. Tredicucci, Y. Chen, V. Pellegrini, M. Börger, L. Sorba, F. Beltram, and F. Bassani, Controlled exciton-photon interaction in semiconductor bulk microcavities, Phys. Rev. Lett. 75, 3906 (1995).
- Y. Chen, A. Tredicucci, and F. Bassani, Bulk exciton polaritons in GaAs microcavities, Phys. Rev. B 52, 1800 (1995).
- B. Sermage, S. Long, I. Abram, J. Y. Marzin, J. Bloch, R. Planel, and V. Thierry-Mieg, Time-resolved spontaneous emission of excitons in a microcavity: Behavior of the individual exciton-photon mixed states, Phys. Rev. B 53, 16516 (1996).
- D. Gammon, S. Rudin, T. L. Reinecke, D. S. Katzer, and C. S. Kyono, Phonon broadening of excitons in quantum wells, Phys. Rev. B 51, 16785 (1995).
- R. Houdré, R. P. Stanley, and M. Ilegems, Vacuum-field Rabi splitting in the presence of inhomogeneous broadening: Resolution of a homogeneous linewidth in an inhomogeneously broadened system, Phys. Rev. A 53, 2711 (1996).
- D. M. Whittaker, P. Kinsler, T. A. Fisher, M. S. Skolnick, A. Armitage, A. M. Afshar, M. D. Sturge, and J. S. Roberts, Motional narrowing in semiconductor microcavities, Phys. Rev. Lett. 77, 4792 (1996).
- H. Suchomel, S. Kreutzer, M. Jörg, S. Brodbeck, M. Pieczarka, S. Betzold, C. P. Dietrich, G. Sek, C. Schneider, and S. Höfling, Room temperature strong coupling in a semiconductor microcavity with embedded algaas quantum wells designed for polariton lasing, Opt. Express 25, 24816 (2017).
- V. Savona, L. C. Andreani, P. Schwendimann, and A. Quattropani, Quantum well excitons in semiconductor microcavities: Unified treatment of weak and strong coupling regimes, Solid State Commun. 93, 733 (1995).
- A. S. Kuznetsov, K. Biermann, A. A. Reynoso, A. Fainstein, and P. V. Santos, Microcavity phonoritons-a coherent optical-to-microwave interface, Nat. Commun. 14, 5470 (2023).