- Letter
- Open Access
Ultrafast optical generation of antiferromagnetic meron-antimeron pairs with conservation of topological charge
Phys. Rev. Research 5, L022007 – Published 7 April, 2023
DOI: https://doi.org/10.1103/PhysRevResearch.5.L022007
Abstract
We propose a new mechanism to produce a meron-antimeron pair in a two dimensional antiferromagnet with an ultrafast laser pulse via a thermal Schwinger mechanism. Unlike ultrafast skyrmion nucleation, this process conserves total topological charge. We systematically show different stages of the dynamics and define proper topological invariants to characterize the configurations. The emergent structure can retain its topological structure for up to 100 ps. By introducing a topological structure factor we show that pair formation is robust against any random choice of initial magnetic configuration and can survive against disorder. Our findings demonstrate that the rich world of spin textures, which goes beyond conventional skyrmions, can be reached optically.
Physics Subject Headings (PhySH)
Article Text
References (39)
- A. Kirilyuk, A. V. Kimel, and T. Rasing, Ultrafast optical manipulation of magnetic order, Rev. Mod. Phys. 82, 2731 (2010).
- I. Radu, K. Vahaplar, C. Stamm, T. Kachel, N. Pontius, H. A. Dürr, T. A. Ostler, J. Barker, R. F. L. Evans, R. W. Chantrell, A. Tsukamoto, A. Itoh, A. Kirilyuk, T. Rasing, and A. V. Kimel, Transient ferromagnetic-like state mediating ultrafast reversal of antiferromagnetically coupled spins, Nature (London) 472, 205 (2011).
- Y. Yang, R. B. Wilson, J. Gorchon, C.-H. Lambert, S. Salahuddin, and J. Bokor, Ultrafast magnetization reversal by picosecond electrical pulses, Sci. Adv. 3, e1603117 (2017).
- E. Beaurepaire, J.-C. Merle, A. Daunois, and J.-Y. Bigot, Ultrafast Spin Dynamics in Ferromagnetic Nickel, Phys. Rev. Lett. 76, 4250 (1996).
- G. P. Zhang and W. Hübner, Laser-Induced Ultrafast Demagnetization in Ferromagnetic Metals, Phys. Rev. Lett. 85, 3025 (2000).
- B. Koopmans, J. J. M. Ruigrok, F. D. Longa, and W. J. M. de Jonge, Unifying Ultrafast Magnetization Dynamics, Phys. Rev. Lett. 95, 267207 (2005).
- B. Koopmans, G. Malinowski, F. Dalla Longa, D. Steiauf, M. Fähnle, T. Roth, M. Cinchetti, and M. Aeschlimann, Explaining the paradoxical diversity of ultrafast laser-induced demagnetization, Nat. Mater. 9, 259 (2010).
- J. K. Dewhurst, P. Elliott, S. Shallcross, E. K. U. Gross, and S. Sharma, Laser-Induced Intersite Spin Transfer, Nano Lett. 18, 1842 (2018).
- F. Willems, C. von Korff Schmising, C. Strüber, D. Schick, D. W. Engel, J. K. Dewhurst, P. Elliott, S. Sharma, and S. Eisebitt, Optical inter-site spin transfer probed by energy and spin-resolved transient absorption spectroscopy, Nat. Commun. 11, 871 (2020).
- J. K. Dewhurst, S. Shallcross, P. Elliott, S. Eisebitt, C. V. K. Schmising, and S. Sharma, Angular momentum redistribution in laser-induced demagnetization, Phys. Rev. B 104, 054438 (2021).
- E. Golias, I. Kumberg, I. Gelen, S. Thakur, J. Gördes, R. Hosseinifar, Q. Guillet, J. K. Dewhurst, S. Sharma, C. Schüßler-Langeheine, N. Pontius, and W. Kuch, Ultrafast Optically Induced Ferromagnetic State in an Elemental Antiferromagnet, Phys. Rev. Lett. 126, 107202 (2021).
- F. Büttner, B. Pfau, M. Böttcher, M. Schneider, G. Mercurio, C. M. Günther, P. Hessing, C. Klose, A. Wittmann, K. Gerlinger, L. M. Kern, C. Strüber, C. von Korff Schmising, J. Fuchs, D. Engel, A. Churikova, S. Huang, D. Suzuki, I. Lemesh, M. Huang, L. Caretta, D. Weder, J. H. Gaida, M. Möller, T. R. Harvey, S. Zayko, K. Bagschik, R. Carley, L. Mercadier, J. Schlappa, A. Yaroslavtsev, L. Le Guyarder, N. Gerasimova, A. Scherz, C. Deiter, R. Gort, D. Hickin, J. Zhu, M. Turcato, D. Lomidze, F. Erdinger, A. Castoldi, S. Maffessanti, M. Porro, A. Samartsev, J. Sinova, C. Ropers, J. H. Mentink, B. Dupé, G. S. D. Beach, and S. Eisebitt, Observation of fluctuation-mediated picosecond nucleation of a topological phase, Nat. Mater. 20, 30 (2021).
- A. Fert, V. Cros, and J. Sampaio, Skyrmions on the track, Nat. Nanotechnol. 8, 152 (2013).
- E. Viñas Boström, A. Rubio, and C. Verdozzi, Microscopic theory of light-induced ultrafast skyrmion excitation in transition metal films, npj Comput. Mater. 8, 62 (2022).
- C. Heo, N. S. Kiselev, A. K. Nandy, S. Blügel, and T. Rasing, Switching of chiral magnetic skyrmions by picosecond magnetic field pulses via transient topological states, Sci. Rep. 6, 27146 (2016).
- A. Ono and S. Ishihara, Photoinduced topological spin texture in a metallic ferromagnet, J. Phys. Soc. Jpn. 88, 023703 (2019).
- S. Ghosh, F. Freimuth, O. Gomonay, S. Blügel, and Y. Mokrousov, Driving spin chirality by electron dynamics in laser-excited antiferromagnets, Commun. Phys. 5, 69 (2022).
- N. Nagaosa and Y. Tokura, Topological properties and dynamics of magnetic skyrmions, Nat. Nanotechnol. 8, 899 (2013).
- J. Preskill, Magnetic Monopoles, Annu. Rev. Nucl. Part. Sci. 34, 461 (1984).
- M. N. Saha, The origin of mass in Neutrons and Protons, Indian J. Phys. 10, 141 (1936).
- O. Gould and A. Rajantie, Magnetic Monopole Mass Bounds from Heavy-Ion Collisions and Neutron Stars, Phys. Rev. Lett. 119, 241601 (2017).
- T. Kobayashi, Monopole-antimonopole pair production in primordial magnetic fields, Phys. Rev. D 104, 043501 (2021).
- N. Gao, S. G. Je, M. Y. Im, J. W. Choi, M. Yang, Q. Li, T. Y. Wang, S. Lee, H. S. Han, K. S. Lee, W. Chao, C. Hwang, J. Li, and Z. Q. Qiu, Creation and annihilation of topological meron pairs in in-plane magnetized films, Nat. Commun. 10, 5603 (2019).
- X. Lu, R. Fei, L. Zhu, and L. Yang, Meron-like topological spin defects in monolayer CrCl3, Nat. Commun. 11, 4724 (2020).
- M. Augustin, S. Jenkins, R. F. L. Evans, K. S. Novoselov, and E. J. G. Santos, Properties and dynamics of meron topological spin textures in the two-dimensional magnet CrCl3, Nat. Commun. 12, 185 (2021).
- X. Z. Yu, W. Koshibae, Y. Tokunaga, K. Shibata, Y. Taguchi, N. Nagaosa, and Y. Tokura, Transformation between meron and skyrmion topological spin textures in a chiral magnet, Nature (London) 564, 95 (2018).
- X. Zhang, Y. Zhou, and M. Ezawa, Antiferromagnetic skyrmion: Stability, creation and manipulation, Sci. Rep. 6, 24795 (2016); P. M. Buhl, F. Freimuth, S. Blügel, and Y. Mokrousov, Topological spin Hall effect in antiferromagnetic skyrmions, Phys. Status Solidi RRL 11, 1700007 (2017); B. Göbel, A. Mook, J. Henk, and I. Mertig, Antiferromagnetic skyrmion crystals: Generation, topological Hall, and topological spin Hall effect, Phys. Rev. B 96, 060406 (2017).
- W. Koshibae, N. Furukawa, and N. Nagaosa, Real-Time Quantum Dynamics of Interacting Electrons: Self-Organized Nanoscale Structure in a Spin-Electron Coupled System, Phys. Rev. Lett. 103, 266402 (2009).
- A. Ono and S. Ishihara, Double-Exchange Interaction in Optically Induced Nonequilibrium State: A Conversion from Ferromagnetic to Antiferromagnetic Structure, Phys. Rev. Lett. 119, 207202 (2017).
- M. D. Petrović, B. S. Popescu, U. Bajpai, P. Plecháč, and B. K. Nikolić, Spin and Charge Pumping by a Steady or Pulse-Current-Driven Magnetic Domain Wall: A Self-Consistent Multiscale Time-Dependent Quantum-Classical Hybrid Approach, Phys. Rev. Appl. 10, 054038 (2018).
- J. García-Palacios and F. J. Lázaro, Langevin-dynamics study of the dynamical properties of small magnetic particles, Phys. Rev. B 58, 14937 (1998).
- S. Ghosh and A. Manchon, Nonequilibrium spin density and spin-orbit torque in a three-dimensional topological insulator/antiferromagnet heterostructure, Phys. Rev. B 100, 014412 (2019).
- I. K. Affleck and N. S. Manton, Monopole pair production in a magnetic field, Nucl. Phys. B 194, 38 (1982); I. K. Affleck, O. Alvarez, and N. S. Manton, Pair production at strong coupling in weak external fields, ibid. 197, 509 (1982).
- O. Gould, S. Mangles, A. Rajantie, S. Rose, and C. Xie, Observing thermal Schwinger pair production, Phys. Rev. A 99, 052120 (2019).
- S. Digal and A. M. Srivastava, Formation of Topological Defects with Explicit Symmetry Breaking, Phys. Rev. Lett. 76, 583 (1996); E. J. Copeland and P. M. Saffin, Bubble collisions in Abelian gauge theories and the geodesic rule, Phys. Rev. D 54, 6088 (1996); S. Digal, S. Sengupta, and A. M. Srivastava, Vortex-antivortex pair production in a first order phase transition, ibid. 56, 2035 (1997).
- T. W. B. Kibble, Topology of cosmic domains and strings, J. Phys. A: Math. Gen. 9, 1387 (1976).
- P. Rybakov, Topological excitations in field theory models of superconductivity and magnetism, Ph.D. thesis (2021) V. M. Kuchkin, B. Barton-Singer, F. N. Rybakov, S. Blügel, B. J. Schroers, and N. S. Kiselev, Magnetic skyrmions, chiral kinks, and holomorphic functions, Phys. Rev. B 102, 144422 (2020).
- F. N. Rybakov, A. B. Borisov, S. Blügel, and N. S. Kiselev, New Type of Stable Particlelike States in Chiral Magnets, Phys. Rev. Lett. 115, 117201 (2015).
- F. N. Rybakov, N. S. Kiselev, A. B. Borisov, L. Döring, C. Melcher, and S. Blügel, Magnetic hopfions in solids, APL Mater. 10, 111113 (2022).