Reuse & Permissions

It is not necessary to obtain permission to reuse this article or its components as it is available under the terms of the Creative Commons Attribution 4.0 International license. This license permits unrestricted use, distribution, and reproduction in any medium, provided attribution to the author(s) and the published article's title, journal citation, and DOI are maintained. Please note that some figures may have been included with permission from other third parties. It is your responsibility to obtain the proper permission from the rights holder directly for these figures.

Export citation

Export citation

Choose format for download:

Download Citation
  • Open Access

Order by disorder in classical kagome antiferromagnets with chiral interactions

Jackson Pitts1, Finn Lasse Buessen2,3, Roderich Moessner4, Simon Trebst3, and Kirill Shtengel1,4

  • 1Department of Physics and Astronomy, University of California, Riverside, California 92521, USA
  • 2Department of Physics, University of Toronto, Toronto, Ontario M5S 1A7, Canada
  • 3Institute for Theoretical Physics, University of Cologne, Zülpicher Straße 77, 50937 Köln, Germany
  • 4Max-Planck-Institut für Physik komplexer Systeme, Nöthnitzer Straße 38, 01187 Dresden, Germany

Phys. Rev. Research 4, 043019 – Published 10 October, 2022

DOI: https://doi.org/10.1103/PhysRevResearch.4.043019

Abstract

The Heisenberg antiferromagnet on the kagome lattice is an archetypal instance of how large ground-state degeneracies arise, and how they may get resolved by thermal and quantum fluctuations. Augmenting the Heisenberg model by chiral spin interactions has proved to be of particular interest in the discovery of certain chiral quantum spin liquids. Here we consider the classical variant of this chiral kagome model and find that it exhibits, similar to the classical Heisenberg antiferromagnet, a remarkably large and structured ground-state manifold, which combines continuous and discrete degrees of freedom. This allows for a rich set of order-by-disorder phenomena. Degeneracy lifting occurs in a highly selective way, choosing already at the harmonic level specific triaxial states, which however retain an emergent Z2 degree of freedom (absent in the conventional Heisenberg model). We also study the competition of entropic and energetic ground-state selection as the model interpolates between the purely chiral and Heisenberg cases. For this mixed model, we find a “proximate ordered-by-disorder” finite-temperature regime where fluctuations overcome the energetic ground-state preference of the perturbation. Finally, a semiclassical route to a spin liquid is provided by quantum order by disorder in the purely chiral models, where the aforementioned Z2 degrees of freedom are elevated to the role of an emergent gauge field.

View figure in article

Physics Subject Headings (PhySH)

Article Text

References (62)

  1. R. B. Laughlin, Anomalous Quantum Hall Effect: An Incompressible Quantum Fluid with Fractionally Charged Excitations, Phys. Rev. Lett. 50, 1395 (1983).
  2. L. Balents, C. R. Dean, D. K. Efetov, and A. F. Young, Superconductivity and strong correlations in moiré flat bands, Nat. Phys. 16, 725 (2020).
  3. E. Y. Andrei and A. H. MacDonald, Graphene bilayers with a twist, Nat. Mater. 19, 1265 (2020).
  4. D. M. Kennes, M. Claassen, L. Xian, A. Georges, A. J. Millis, J. Hone, C. R. Dean, D. N. Basov, A. N. Pasupathy, and A. Rubio, Moiré heterostructures as a condensed-matter quantum simulator, Nat. Phys. 17, 155 (2021).
  5. R. Bistritzer and A. H. MacDonald, Moiré bands in twisted double-layer graphene, Proc. Natl. Acad. Sci. USA 108, 12233 (2011).
  6. G. H. Wannier, Antiferromagnetism. The triangular Ising net, Phys. Rev. 79, 357 (1950).
  7. R. Moessner, Magnets with strong geometric frustration, Can. J. Phys. 79, 1283 (2001).
  8. R. Moessner and A. P. Ramirez, Geometrical frustration, Phys. Today 59, 24 (2006).
  9. J. Villain, R. Bidaux, J.-P. Carton, and R. Conte, Order as an effect of disorder, J. Phys. France 41, 1263 (1980).
  10. C. L. Henley, Ordering by disorder: Ground-state selection in fcc vector antiferromagnets, J. Appl. Phys. 61, 3962 (1987).
  11. C. L. Henley, Ordering due to Disorder in a Frustrated Vector Antiferromagnet, Phys. Rev. Lett. 62, 2056 (1989).
  12. J. Villain, Insulating spin glasses, Z. Phys. B 33, 31 (1979).
  13. R. Moessner and J. T. Chalker, Properties of a Classical Spin Liquid: The Heisenberg Pyrochlore Antiferromagnet, Phys. Rev. Lett. 80, 2929 (1998).
  14. D. Bergman, J. Alicea, E. Gull, S. Trebst, and L. Balents, Order-by-disorder and spiral spin-liquid in frustrated diamond-lattice antiferromagnets, Nat. Phys. 3, 487 (2007).
  15. J.-S. Bernier, M. J. Lawler, and Y. B. Kim, Quantum Order by Disorder in Frustrated Diamond Lattice Antiferromagnets, Phys. Rev. Lett. 101, 047201 (2008).
  16. G. Chen, Quantum paramagnet and frustrated quantum criticality in a spin-one diamond lattice antiferromagnet, Phys. Rev. B 96, 020412(R) (2017).
  17. F. L. Buessen, M. Hering, J. Reuther, and S. Trebst, Quantum Spin Liquids in Frustrated Spin-1 Diamond Antiferromagnets, Phys. Rev. Lett. 120, 057201 (2018).
  18. V. Fritsch, J. Hemberger, N. Büttgen, E.-W. Scheidt, H.-A. Krug von Nidda, A. Loidl, and V. Tsurkan, Spin and Orbital Frustration in MnSc2S4, Phys. Rev. Lett. 92, 116401 (2004).
  19. S. Gao, O. Zaharko, V. Tsurkan, Y. Su, J. S. White, G. S. Tucker, B. Roessli, F. Bourdarot, R. Sibille, D. Chernyshov, T. Fennell, A. Loidl, and C. Rüegg, Spiral spin-liquid and the emergence of a vortex-like state in MnSc2S4, Nat. Phys. 13, 157 (2017).
  20. U. Hizi, P. Sharma, and C. L. Henley, Semiclassical Ordering in the Large-n Pyrochlore Antiferromagnet, Phys. Rev. Lett. 95, 167203 (2005).
  21. U. Hizi and C. L. Henley, Effective Hamiltonian for the pyrochlore antiferromagnet: Semiclassical derivation and degeneracy, Phys. Rev. B 73, 054403 (2006).
  22. J. D. M. Champion, M. J. Harris, P. C. W. Holdsworth, A. S. Wills, G. Balakrishnan, S. T. Bramwell, E. Čižmár, T. Fennell, J. S. Gardner, J. Lago, D. F. McMorrow, M. Orendáč, A. Orendáčová, D. McK. Paul, R. I. Smith, M. T. F. Telling, and A. Wildes, Er2Ti2O7: Evidence of quantum order by disorder in a frustrated antiferromagnet, Phys. Rev. B 68, 020401(R) (2003).
  23. M. E. Zhitomirsky, M. V. Gvozdikova, P. C. W. Holdsworth, and R. Moessner, Quantum Order by Disorder and Accidental Soft Mode in Er2Ti2O7, Phys. Rev. Lett. 109, 077204 (2012).
  24. L. Savary, K. A. Ross, B. D. Gaulin, J. P. C. Ruff, and L. Balents, Order by Quantum Disorder in Er2Ti2O7, Phys. Rev. Lett. 109, 167201 (2012).
  25. J. T. Chalker, P. C. W. Holdsworth, and E. F. Shender, Hidden Order in a Frustrated System: Properties of the Heisenberg Kagome Antiferromagnet, Phys. Rev. Lett. 68, 855 (1992).
  26. A. B. Harris, C. Kallin, and A. J. Berlinsky, Possible Néel orderings of the kagome antiferromagnet, Phys. Rev. B 45, 2899 (1992).
  27. I. Ritchey, P. Chandra, and P. Coleman, Spin folding in the two-dimensional Heisenberg kagome antiferromagnet, Phys. Rev. B 47, 15342 (1993).
  28. D. A. Huse and A. D. Rutenberg, Classical antiferromagnets on the kagome lattice, Phys. Rev. B 45, 7536 (1992).
  29. A. Chubukov, Order from Disorder in a Kagome Antiferromagnet, Phys. Rev. Lett. 69, 832 (1992).
  30. M. E. Zhitomirsky, Octupolar ordering of classical kagome antiferromagnets in two and three dimensions, Phys. Rev. B 78, 094423 (2008).
  31. G.-W. Chern and R. Moessner, Dipolar Order by Disorder in the Classical Heisenberg Antiferromagnet on the Kagome Lattice, Phys. Rev. Lett. 110, 077201 (2013).
  32. S. Yan, D. A. Huse, and S. R. White, Spin-liquid ground state of the s = 1/2 kagome Heisenberg antiferromagnet, Science 332, 1173 (2011).
  33. Y.-C. He, M. P. Zaletel, M. Oshikawa, and F. Pollmann, Signatures of Dirac Cones in a DMRG Study of the Kagome Heisenberg Model, Phys. Rev. X 7, 031020 (2017).
  34. M. Hermele, Y. Ran, P. A. Lee, and X.-G. Wen, Properties of an algebraic spin liquid on the kagome lattice, Phys. Rev. B 77, 224413 (2008).
  35. Y. Huh, L. Fritz, and S. Sachdev, Quantum criticality of the kagome antiferromagnet with Dzyaloshinskii–Moriya interactions, Phys. Rev. B 81, 144432 (2010).
  36. H. J. Changlani, D. Kochkov, K. Kumar, B. K. Clark, and E. Fradkin, Macroscopically Degenerate Exactly Solvable Point in the Spin-1/2 Kagome Quantum Antiferromagnet, Phys. Rev. Lett. 120, 117202 (2018).
  37. A. E. B. Nielsen, G. Sierra, and J. I. Cirac, Local models of fractional quantum Hall states in lattices and physical implementation, Nat. Commun. 4, 2864 (2013).
  38. B. Bauer, L. Cincio, B. Keller, M. Dolfi, G. Vidal, S. Trebst, and A. Ludwig, Chiral spin liquid and emergent anyons in a kagome lattice Mott insulator, Nat. Commun. 5, 5137 (2014).
  39. V. Kalmeyer and R. B. Laughlin, Equivalence of the Resonating-Valence-Bond and Fractional Quantum Hall States, Phys. Rev. Lett. 59, 2095 (1987).
  40. B. Bauer, B. P. Keller, S. Trebst, and A. W. W. Ludwig, Symmetry-protected non-Fermi liquids, kagome spin liquids, and the chiral Kondo lattice model, Phys. Rev. B 99, 035155 (2019).
  41. P. A. Lee, N. Nagaosa, and X.-G. Wen, Doping a Mott insulator: Physics of high-temperature superconductivity, Rev. Mod. Phys. 78, 17 (2006).
  42. O. I. Motrunich and M. P. A. Fisher, d-wave correlated critical Bose liquids in two dimensions, Phys. Rev. B 75, 235116 (2007).
  43. E. F. Shender and P. C. W. Holdsworth, Fluctuations and Order: The New Synthesis (Springer, New York, 1996), Chap. 16, pp. 259–280
  44. R. J. Baxter, Colorings of a hexagonal lattice, J. Math. Phys. 11, 784 (1970).
  45. T. Bilitewski, M. E. Zhitomirsky, and R. Moessner, Jammed Spin Liquid in the Bond-Disordered Kagome Antiferromagnet, Phys. Rev. Lett. 119, 247201 (2017).
  46. R. Moessner and J. T. Chalker, Low-temperature properties of classical geometrically frustrated antiferromagnets, Phys. Rev. B 58, 12049 (1998).
  47. A. Banerjee, C. A. Bridges, J.-Q. Yan, A. A. Aczel, L. Li, M. B. Stone, G. E. Granroth, M. D. Lumsden, Y. Yiu, J. Knolle, et al., Proximate Kitaev quantum spin liquid behaviour in a honeycomb magnet, Nat. Mater. 15, 733 (2016).
  48. A. Banerjee, J. Yan, J. Knolle, C. A. Bridges, M. B. Stone, M. D. Lumsden, D. G. Mandrus, D. A. Tennant, R. Moessner, and S. E. Nagler, Neutron scattering in the proximate quantum spin liquid α−RuCl3, Science 356, 1055 (2017).
  49. A. Revelli, M. Moretti Sala, G. Monaco, C. Hickey, P. Becker, F. Freund, A. Jesche, P. Gegenwart, T. Eschmann, F. L. Buessen, S. Trebst, P. H. M. van Loosdrecht, J. van den Brink, and M. Grüninger, Fingerprints of Kitaev physics in the magnetic excitations of honeycomb iridates, Phys. Rev. Res. 2, 043094 (2020).
  50. D. L. Bergman, C. Wu, and L. Balents, Band touching from real-space topology in frustrated hopping models, Phys. Rev. B 78, 125104 (2008).
  51. T. Bilitewski and R. Moessner, Disordered flat bands on the kagome lattice, Phys. Rev. B 98, 235109 (2018).
  52. The values presented were obtained by a quadratic fit to the sequence of trapezoidal rule approximations. All trapezoidal rule results from values of h>hmin were used for the fit, which was very good, having a variance smaller than the machine precision.
  53. C. L. Henley, Order by Disorder and Gaugelike Degeneracy in a Quantum Pyrochlore Antiferromagnet, Phys. Rev. Lett. 96, 047201 (2006).
  54. T. A. Tóth, A. M. Läuchli, F. Mila, and K. Penc, Three-Sublattice Ordering of the SU(3) Heisenberg Model of Three-Flavor Fermions on the Square and Cubic Lattices, Phys. Rev. Lett. 105, 265301 (2010).
  55. J. von Delft and C. L. Henley, Destructive Quantum Interference in Spin Tunneling Problems, Phys. Rev. Lett. 69, 3236 (1992).
  56. A. Y. Kitaev, Fault-tolerant quantum computation by anyons, Ann. Phys. 303, 2 (2003).
  57. I. Rousochatzakis, Y. Sizyuk, and N. B. Perkins, Quantum spin liquid in the semiclassical regime, Nat. Commun. 9, 1575 (2018).
  58. C. Castelnovo and C. Chamon, Entanglement and topological entropy of the toric code at finite temperature, Phys. Rev. B 76, 184442 (2007).
  59. C. Hickey, L. Cincio, Z. Papić, and A. Paramekanti, Emergence of chiral spin liquids via quantum melting of noncoplanar magnetic orders, Phys. Rev. B 96, 115115 (2017).
  60. A. F. Albuquerque, F. Alet, P. Corboz, P. Dayal, A. Feiguin, S. Fuchs, L. Gamper, E. Gull, S. Gürtler, A. Honecker et al., The ALPS project release 1.3: Open-source software for strongly correlated systems, J. Magn. Magn. Mater. 310, 1187 (2007).
  61. B. Bauer, L. D. Carr, H. G. Evertz, A. Feiguin, J. Freire, S. Fuchs, L. Gamper, J. Gukelberger, E. Gull, S. Guertler et al., The ALPS project release 2.0: Open source software for strongly correlated systems, J. Stat. Mech. (2011) P05001.
  62. ALPS project, http://alps.comp-phys.org.

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation