- Letter
- Open Access
Higher-order topological insulators in two-dimensional Dirac materials
Phys. Rev. Research 3, L042044 – Published 23 December, 2021
DOI: https://doi.org/10.1103/PhysRevResearch.3.L042044
Abstract
As a novel topological state, a higher-order topological insulator has attracted enormous interest, which in spatial dimensions has gapless boundary states at () dimensions (integer is larger than 1). Until now, merely few two-dimensional (2D) materials have been identified as higher-order topological insulators and their experimental confirmations are still absent. Here we propose a universal strategy of antidot engineering to realize second-order topological insulators (SOTIs) in 2D Dirac materials. Based on symmetry analysis, tight-binding model, and first-principles calculations, we demonstrate SOTIs in antidot-decorated Xene (X=C, Si,and Ge) by displaying its finite bulk quadrupole moment, weak topological edge states, and in-gap topological corner states. An inherent connection is established for the existing various mechanisms of the SOTIs, including quadrupole polarization, filling anomaly, and generalized Su-Schrieffer-Heeger model on a Kekulé lattice. The robustness of topological corner states of the SOTIs against edge perturbations and bulk disorders is explicitly demonstrated, rendering our strategy appealing to experimental realization of topological corner states.
Physics Subject Headings (PhySH)
Article Text
Supplemental Material
References (45)
- W. A. Benalcazar, B. A. Bernevig, and T. L. Hughes, Quantized electric multipole insulators, Science 357, 61 (2017).
- W. A. Benalcazar, B. A. Bernevig, and T. L. Hughes, Electric multipole moments, topological multipole moment pumping, and chiral hinge states in crystalline insulators, Phys. Rev. B 96, 245115 (2017).
- Z. Song, Z. Fang, and C. Fang, (d-2)-Dimensional Edge States of Rotation Symmetry Protected Topological States, Phys. Rev. Lett. 119, 246402 (2017).
- F. Schindler, A. M. Cook, M. G. Vergniory, Z. Wang, S. S. Parkin, B. A. Bernevig, and T. Neupert, Higher-order topological insulators, Sci. Adv. 4, eaat0346 (2018).
- T. Mizoguchi, H. Araki, and Y. Hatsugai, Higher-order topological phase in a honeycomb-lattice model with anti-kekulé distortion, J. Phys. Soc. Jpn. 88, 104703 (2019).
- F. Liu, M. Yamamoto, and K. Wakabayashi, Topological edge states of honeycomb lattices with zero berry curvature, J. Phys. Soc. Jpn. 86, 123707 (2017).
- F. Liu, H.-Y. Deng, and K. Wakabayashi, Helical Topological Edge States in a Quadrupole Phase, Phys. Rev. Lett. 122, 086804 (2019).
- J. Langbehn, Y. Peng, L. Trifunovic, F. von Oppen, and P. W. Brouwer, Reflection-Symmetric Second-Order Topological Insulators and Superconductors, Phys. Rev. Lett. 119, 246401 (2017).
- S. K. Radha and W. R. L. Lambrecht, Buckled honeycomb antimony: Higher order topological insulator and its relation to the kekulé lattice, Phys. Rev. B 102, 115104 (2020).
- X.-L. Sheng, C. Chen, H. Liu, Z. Chen, Z.-M. Yu, Y. X. Zhao, and S. A. Yang, Two-Dimensional Second-Order Topological Insulator in Graphdiyne, Phys. Rev. Lett. 123, 256402 (2019).
- B. Liu, G. Zhao, Z. Liu, and Z. Wang, Two-dimensional quadrupole topological insulator in -graphyne, Nano Lett. 19, 6492 (2019).
- M. J. Park, Y. Kim, G. Y. Cho, and S. B. Lee, Higher-Order Topological Insulator in Twisted Bilayer Graphene, Phys. Rev. Lett. 123, 216803 (2019).
- W. A. Benalcazar, T. Li, and T. L. Hughes, Quantization of fractional corner charge in -symmetric higher-order topological crystalline insulators, Phys. Rev. B 99, 245151 (2019).
- F. Schindler, M. Brzezińska, W. A. Benalcazar, M. Iraola, A. Bouhon, S. S. Tsirkin, M. G. Vergniory, and T. Neupert, Fractional corner charges in spin-orbit coupled crystals, Phys. Rev. Research 1, 033074 (2019).
- B. Xie, H.-X. Wang, X. Zhang, P. Zhan, J.-H. Jiang, M. Lu, and Y. Chen, Higher-order band topology, Nat. Rev. Phys. 3, 520 (2021).
- M. Ezawa, Higher-Order Topological Insulators and Semimetals on the Breathing Kagome and Pyrochlore Lattices, Phys. Rev. Lett. 120, 026801 (2018).
- F. K. Kunst, G. van Miert, and E. J. Bergholtz, Lattice models with exactly solvable topological hinge and corner states, Phys. Rev. B 97, 241405(R) (2018).
- Y. Xu, R. Xue, and S. Wan, Topological corner states on kagome lattice based chiral higher-order topological insulator, arXiv:1711.09202.
- A. Molle, J. Goldberger, M. Houssa, Y. Xu, S.-C. Zhang, and D. Akinwande, Buckled two-dimensional xene sheets, Nat. Mater. 16, 163 (2017).
- J. Wang, S. Deng, Z. Liu, and Z. Liu, The rare two-dimen- sional materials with dirac cones, Natl. Sci. Rev. 2, 22 (2015).
- M. Wu, Z. Wang, J. Liu, W. Li, H. Fu, L. Sun, X. Liu, M. Pan, H. Weng, and M. Dincă, Conetronics in 2d metal-organic frameworks: double/half dirac cones and quantum anomalous hall effect, 2D Mater. 4, 015015 (2016).
- K. S. Novoselov, A. K. Geim, S. V. Morozov, D. Jiang, Y. Zhang, S. V. Dubonos, I. V. Grigorieva, and A. A. Firsov, Electric field effect in atomically thin carbon films, Science 306, 666 (2004).
- B. Feng, Z. Ding, S. Meng, Y. Yao, X. He, P. Cheng, L. Chen, and K. Wu, Evidence of silicene in honeycomb structures of silicon on ag (111), Nano Lett. 12, 3507 (2012).
- M. Dávila, L. Xian, S. Cahangirov, A. Rubio, and G. Le Lay, Germanene: A novel two-dimensional germanium allotrope akin to graphene and silicene, New J. Phys. 16, 095002 (2014).
- Z. Ni, Q. Liu, K. Tang, J. Zheng, J. Zhou, R. Qin, Z. Gao, D. Yu, and J. Lu, Tunable bandgap in silicene and germanene, Nano Lett. 12, 113 (2012).
- C. L. Kane and E. J. Mele, Quantum Spin Hall Effect in Graphene, Phys. Rev. Lett. 95, 226801 (2005).
- C.-C. Liu, W. Feng, and Y. Yao, Quantum Spin Hall Effect in Silicene and Two-Dimensional Germanium, Phys. Rev. Lett. 107, 076802 (2011).
- J. Zak, Band representations and symmetry types of bands in solids, Phys. Rev. B 23, 2824 (1981).
- B. Bradlyn, L. Elcoro, J. Cano, M. Vergniory, Z. Wang, C. Felser, M. Aroyo, and B. A. Bernevig, Topological quantum chemistry, Nature (London) 547, 298 (2017).
- J. Cano, B. Bradlyn, Z. Wang, L. Elcoro, M. G. Vergniory, C. Felser, M. I. Aroyo, and B. A. Bernevig, Building blocks of topological quantum chemistry: Elementary band representations, Phys. Rev. B 97, 035139 (2018).
- R.-J. Slager, A. Mesaros, V. Jurić, and J. Zaanen, The space group classification of topological band-insulators, Nat. Phys. 9, 98 (2013).
- J. Kruthoff, J. De Boer, J. Van Wezel, C. L. Kane, and R.-J. Slager, Topological Classification of Crystalline Insulators Through Band Structure Combinatorics, Phys. Rev. X 7, 041069 (2017).
- B. Bradlyn, Z. Wang, J. Cano, and B. A. Bernevig, Disconnected elementary band representations, fragile topology, and wilson loops as topological indices: An example on the triangular lattice, Phys. Rev. B 99, 045140 (2019).
- J.-S. Park and H. J. Choi, Band-gap opening in graphene: A reverse-engineering approach, Phys. Rev. B 92, 045402 (2015).
- See Supplemental Material at http://link.aps.org/supplemental/10.1103/PhysRevResearch.3.L042044 for calculation methods, band representations of GrALs, energy bands, edge and corner states of SiALs and GeALs.
- T. G. Pedersen, C. Flindt, J. Pedersen, N. A. Mortensen, A.-P. Jauho, and K. Pedersen, Graphene Antidot Lattices: Designed Defects and Spin Qubits, Phys. Rev. Lett. 100, 136804 (2008).
- F. Pan, Y. Wang, K. Jiang, Z. Ni, J. Ma, J. Zheng, R. Quhe, J. Shi, C. Chen, and J. Lu, Silicene nanomesh, Sci. Rep. 5, 9075 (2015).
- J. Bai, X. Zhong, S. Jiang, Y. Huang, and X. Duan, Graphene nanomesh, Nat. Nanotechnol. 5, 190 (2010).
- J. Mahmood, E. K. Lee, M. Jung, D. Shin, I.-Y. Jeon, S.-M. Jung, H.-J. Choi, J.-M. Seo, S.-Y. Bae, S.-D. Sohn, N. Park, J. H. Oh, H.-J. Shin, and J.-B. Baek, Nitrogenated holey two-dimensional structures, Nat. Commun. 6, 6486 (2015).
- L. Meng, Y. Wang, L. Zhang, S. Du, R. Wu, L. Li, Y. Zhang, G. Li, H. Zhou, and W. A. Hofer, Buckled silicene formation on ir (111), Nano Lett. 13, 685 (2013).
- M. Kim, N. S. Safron, E. Han, M. S. Arnold, and P. Gopalan, Fabrication and characterization of large-area, semiconducting nanoperforated graphene materials, Nano Lett. 10, 1125 (2010).
- F. Ouyang, S. Peng, Z. Liu, and Z. Liu, Bandgap opening in graphene antidot lattices: the missing half, ACS Nano 5, 4023 (2011).
- P. Delplace, D. Ullmo, and G. Montambaux, Zak phase and the existence of edge states in graphene, Phys. Rev. B 84, 195452 (2011).
- C.-Y. Hou, C. Chamon, and C. Mudry, Electron Fractionalization in Two-Dimensional Graphenelike Structures, Phys. Rev. Lett. 98, 186809 (2007).
- M. I. Aroyo, A. Kirov, C. Capillas, J. Perez-Mato, and H. Wondratschek, Bilbao crystallographic server. ii. Representations of crystallographic point groups and space groups, Acta Crystallogr. Sect. Ay 62, 115 (2006).