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  • Letter
  • Open Access

Spontaneous fractional Chern insulators in transition metal dichalcogenide moiré superlattices

Heqiu Li1, Umesh Kumar2, Kai Sun1, and Shi-Zeng Lin3

  • 1Department of Physics, University of Michigan, Ann Arbor, Michigan 48109, USA
  • 2Theoretical Division, T-4, Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA
  • 3Theoretical Division, T-4 and CNLS, Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA

Phys. Rev. Research 3, L032070 – Published 22 September, 2021

DOI: https://doi.org/10.1103/PhysRevResearch.3.L032070

Abstract

The Moiré superlattice realized in two-dimensional heterostructures offers an exciting platform to access strongly correlated electronic states. In this work, we study transition metal dichalcogenides (TMD) Moiré superlattices with time-reversal symmetry and nontrivial spin/valley-Chern numbers. Utilizing realistic material parameters and the method of exact diagonalization, we find that at a certain twisting angle and fractional filling, gapped fractional topological states, i.e., fractional Chern insulators, are naturally stabilized by simply introducing the Coulomb repulsion. In contrast to fractional quantum Hall systems, where the time-reversal symmetry has to be broken explicitly, these fractional states break the time-reversal symmetry spontaneously. We show that the Chern number contrasting in the opposite valleys imposes a strong constraint on the nature of fractional Chern insulator and the associated low-energy excitations.

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References (65)

  1. J. M. B. Lopes dos Santos, N. M. R. Peres, and A. H. Castro Neto, Graphene Bilayer with a Twist: Electronic Structure, Phys. Rev. Lett. 99, 256802 (2007).
  2. R. Bistritzer and A. H. MacDonald, Moiré bands in twisted double-layer graphene, Proc. Natl. Acad. Sci. USA 108, 12233 (2011).
  3. Y. Cao, V. Fatemi, A. Demir, S. Fang, S. L. Tomarken, J. Y. Luo, J. D. Sanchez-Yamagishi, K. Watanabe, T. Taniguchi, E. Kaxiras, R. C. Ashoori, and P. Jarillo-Herrero, Correlated insulator behaviour at half-filling in magic-angle graphene superlattices, Nature (London) 556, 80 (2018).
  4. Y. Cao, V. Fatemi, S. Fang, K. Watanabe, T. Taniguchi, E. Kaxiras, and P. Jarillo-Herrero, Unconventional superconductivity in magic-angle graphene superlattices, Nature (London) 556, 43 (2018).
  5. X. Lu, P. Stepanov, W. Yang, M. Xie, M. A. Aamir, I. Das, C. Urgell, K. Watanabe, T. Taniguchi, G. Zhang, A. Bachtold, A. H. MacDonald, and D. K. Efetov, Superconductors, orbital magnets and correlated states in magic-angle bilayer graphene, Nature (London) 574, 653 (2019).
  6. M. Yankowitz, S. Chen, H. Polshyn, Y. Zhang, K. Watanabe, T. Taniguchi, D. Graf, A. F. Young, and C. R. Dean, Tuning superconductivity in twisted bilayer graphene, Science 363, 1059 (2019).
  7. A. Kerelsky, L. J. McGilly, D. M. Kennes, L. Xian, M. Yankowitz, S. Chen, K. Watanabe, T. Taniguchi, J. Hone, C. Dean et al., Maximized electron interactions at the magic angle in twisted bilayer graphene, Nature (London) 572, 95 (2019).
  8. Y. Cao, D. Chowdhury, D. Rodan-Legrain, O. Rubies-Bigordà, K. Watanabe, T. Taniguchi, T. Senthil, and P. Jarillo-Herrero, Strange metal in magic-angle graphene with near planckian dissipation, Phys. Rev. Lett. 124, 076801 (2020).
  9. H. Polshyn, M. Yankowitz, S. Chen, Y. Zhang, K. Watanabe, T. Taniguchi, C. R. Dean, and A. F. Young, Large linear-in-temperature resistivity in twisted bilayer graphene, Nat. Phys. 15, 1011 (2019).
  10. Y. Xie, B. Lian, B. Jäck, X. Liu, C.-L. Chiu, K. Watanabe, T. Taniguchi, B. A. Bernevig, and A. Yazdani, Spectroscopic signatures of many-body correlations in magic-angle twisted bilayer graphene, Nature (London) 572, 101 (2019).
  11. Y. Jiang, X. Lai, K. Watanabe, T. Taniguchi, K. Haule, J. Mao, and E. Y. Andrei, Charge order and broken rotational symmetry in magic-angle twisted bilayer graphene, Nature (London) 573, 91 (2019).
  12. Y. Choi, J. Kemmer, Y. Peng, A. Thomson, H. Arora, R. Polski, Y. Zhang, H. Ren, J. Alicea, G. Refael et al., Electronic correlations in twisted bilayer graphene near the magic angle, Nat. Phys. 15, 1174 (2019).
  13. U. Zondiner, A. Rozen, D. Rodan-Legrain, Y. Cao, R. Queiroz, T. Taniguchi, K. Watanabe, Y. Oreg, F. von Oppen, A. Stern, E. Berg, P. Jarillo-Herrero, and S. Ilani, Cascade of phase transitions and Dirac revivals in magic-angle graphene, Nature (London) 582, 203 (2020).
  14. D. Wong, K. P. Nuckolls, M. Oh, B. Lian, Y. Xie, S. Jeon, K. Watanabe, T. Taniguchi, B. A. Bernevig, and A. Yazdani, Cascade of electronic transitions in magic-angle twisted bilayer graphene, Nature (London) 582, 198 (2020).
  15. K. P. Nuckolls, M. Oh, D. Wong, B. Lian, K. Watanabe, T. Taniguchi, B. A. Bernevig, and A. Yazdani, Strongly correlated Chern insulators in magic-angle twisted bilayer graphene, Nature (London) 588, 610 (2020).
  16. M. He, Y. Li, J. Cai, Y. Liu, K. Watanabe, T. Taniguchi, X. Xu, and M. Yankowitz, Symmetry breaking in twisted double bilayer graphene, Nat. Phys. 17, 26 (2020).
  17. X. Liu, Z. Hao, E. Khalaf, J. Y. Lee, Y. Ronen, H. Yoo, D. Haei Najafabadi, K. Watanabe, T. Taniguchi, A. Vishwanath, and P. Kim, Tunable spin-polarized correlated states in twisted double bilayer graphene, Nature (London) 583, 221 (2020).
  18. E. C. Regan, D. Wang, C. Jin, M. I. Bakti Utama, B. Gao, X. Wei, S. Zhao, W. Zhao, Z. Zhang, K. Yumigeta, M. Blei, J. D. Carlström, K. Watanabe, T. Taniguchi, S. Tongay, M. Crommie, A. Zettl, and F. Wang, Mott and generalized Wigner crystal states in WSe 2/WS 2 moiré superlattices, Nature (London) 579, 359 (2020).
  19. L. Wang, E.-M. Shih, A. Ghiotto, L. Xian, D. A. Rhodes, C. Tan, M. Claassen, D. M. Kennes, Y. Bai, B. Kim, K. Watanabe, T. Taniguchi, X. Zhu, J. Hone, A. Rubio, A. N. Pasupathy, and C. R. Dean, Correlated electronic phases in twisted bilayer transition metal dichalcogenides, Nat. Mater. 19, 861 (2020).
  20. M. Xie and A. H. MacDonald, Nature of the Correlated Insulator States in Twisted Bilayer Graphene, Phys. Rev. Lett. 124, 097601 (2020).
  21. F. Wu and S. Das Sarma, Collective Excitations of Quantum Anomalous Hall Ferromagnets in Twisted Bilayer Graphene, Phys. Rev. Lett. 124, 046403 (2020).
  22. Y. Su and S.-Z. Lin, Current-Induced Reversal of Anomalous Hall Conductance in Twisted Bilayer Graphene, Phys. Rev. Lett. 125, 226401 (2020).
  23. B. Padhi, C. Setty, and P. W. Phillips, Doped twisted bilayer graphene near magic angles: Proximity to wigner crystallization, not mott insulation, Nano Lett. 18, 6175 (2018).
  24. B. Padhi, R. Chitra, and P. W. Phillips, Generalized wigner crystallization in moiré materials, Phys. Rev. B 103, 125146 (2021).
  25. B. Padhi and P. W. Phillips, Pressure-induced metal-insulator transition in twisted bilayer graphene, Phys. Rev. B 99, 205141 (2019).
  26. N. Stefanidis and I. Sodemann, Excitonic laughlin states in ideal topological insulator flat bands and their possible presence in moiré superlattice materials, Phys. Rev. B 102, 035158 (2020).
  27. N. Bultinck, S. Chatterjee, and M. P. Zaletel, Mechanism for Anomalous Hall Ferromagnetism in Twisted Bilayer Graphene, Phys. Rev. Lett. 124, 166601 (2020).
  28. Y.-H. Zhang, D. Mao, Y. Cao, P. Jarillo-Herrero, and T. Senthil, Nearly flat chern bands in moiré superlattices, Phys. Rev. B 99, 075127 (2019).
  29. C. Repellin, Z. Dong, Y.-H. Zhang, and T. Senthil, Ferromagnetism in Narrow Bands of Moiré Superlattices, Phys. Rev. Lett. 124, 187601 (2020).
  30. A. L. Sharpe, E. J. Fox, A. W. Barnard, J. Finney, K. Watanabe, T. Taniguchi, M. A. Kastner, and D. Goldhaber-Gordon, Emergent ferromagnetism near three-quarters filling in twisted bilayer graphene, Science 365, 605 (2019).
  31. M. Serlin, C. L. Tschirhart, H. Polshyn, Y. Zhang, J. Zhu, K. Watanabe, T. Taniguchi, L. Balents, and A. F. Young, Intrinsic quantized anomalous hall effect in a moiré heterostructure, Science 367, 900 (2019).
  32. G. Chen, A. L. Sharpe, E. J. Fox, Y.-H. Zhang, S. Wang, L. Jiang, B. Lyu, H. Li, K. Watanabe, T. Taniguchi et al., Tunable correlated chern insulator and ferromagnetism in trilayer graphene/boron nitride moiré superlattice, arXiv:1905.06535.
  33. P. J. Ledwith, G. Tarnopolsky, E. Khalaf, and A. Vishwanath, Fractional chern insulator states in twisted bilayer graphene: An analytical approach, Phys. Rev. Research 2, 023237 (2020).
  34. C. Repellin and T. Senthil, Chern bands of twisted bilayer graphene: Fractional chern insulators and spin phase transition, Phys. Rev. Research 2, 023238 (2020).
  35. A. Abouelkomsan, Z. Liu, and E. J. Bergholtz, Particle-Hole Duality, Emergent Fermi Liquids, and Fractional Chern Insulators in Moiré Flatbands, Phys. Rev. Lett. 124, 106803 (2020).
  36. Z. Liu, A. Abouelkomsan, and E. J. Bergholtz, Gate-Tunable Fractional Chern Insulators in Twisted Double Bilayer Graphene, Phys. Rev. Lett. 126, 026801 (2021).
  37. P. Wilhelm, T. C. Lang, and A. M. Läuchli, Interplay of Fractional Chern Insulator and Charge-Density-Wave Phases in Twisted Bilayer Graphene, Phys. Rev. B 103, 125406 (2021).
  38. R. Sohal, L. H. Santos, and E. Fradkin, Chern-simons composite fermion theory of fractional chern insulators, Phys. Rev. B 97, 125131 (2018).
  39. R. Sohal and E. Fradkin, Intertwined order in fractional chern insulators from finite-momentum pairing of composite fermions, Phys. Rev. B 101, 245154 (2020).
  40. Y. Xu, S. Liu, D. A. Rhodes, K. Watanabe, T. Taniguchi, J. Hone, V. Elser, K. F. Mak, and J. Shan, Correlated insulating states at fractional fillings of moiré superlattices, Nature (London) 587, 214 (2020).
  41. C. Jin, Z. Tao, T. Li, Y. Xu, Y. Tang, J. Zhu, S. Liu, K. Watanabe, T. Taniguchi, J. C. Hone, L. Fu, J. Shan, and K. F. Mak, Stripe phases in WSe2/WS2 moiré superlattices, Nat. Mater. 20, 940 (2021).
  42. Y. Zhou, J. Sung, E. Brutschea, I. Esterlis, Y. Wang, G. Scuri, R. J. Gelly, H. Heo, T. Taniguchi, K. Watanabe, G. Zaránd, M. D. Lukin, P. Kim, E. Demler, and H. Park, Signatures of bilayer Wigner crystals in a transition metal dichalcogenide heterostructure, arXiv:2010.03037.
  43. X. Huang, T. Wang, S. Miao, C. Wang, Z. Li, Z. Lian, T. Taniguchi, K. Watanabe, S. Okamoto, D. Xiao, S.-F. Shi, and Y.-T. Cui, Correlated insulating states at fractional fillings of the WS2/WSe2 moiré Lattice, arXiv:2007.11155.
  44. E. Tang, J.-W. Mei, and X.-G. Wen, High-Temperature Fractional Quantum Hall States, Phys. Rev. Lett. 106, 236802 (2011).
  45. K. Sun, Z. Gu, H. Katsura, and S. Das Sarma, Nearly Flatbands with Nontrivial Topology, Phys. Rev. Lett. 106, 236803 (2011).
  46. T. Neupert, L. Santos, C. Chamon, and C. Mudry, Fractional Quantum Hall States at Zero Magnetic Field, Phys. Rev. Lett. 106, 236804 (2011).
  47. N. Regnault and B. A. Bernevig, Fractional chern insulator, Phys. Rev. X 1, 021014 (2011).
  48. D. N. Sheng, Z.-C. Gu, K. Sun, and L. Sheng, Fractional quantum hall effect in the absence of landau levels, Nat. Commun. 2, 389 (2011).
  49. S. A. Parameswaran, R. Roy, and S. L. Sondhi, Fractional quantum Hall physics in topological flat bands, C. R. Phys. 14, 816 (2013).
  50. E. J. Bergholtz and Z. Liu, Topological flat band models and fractional chern insulators, Int. J. Mod. Phys. B 27, 1330017 (2013).
  51. Y.-L. Wu, B. A. Bernevig, and N. Regnault, Zoology of fractional chern insulators, Phys. Rev. B 85, 075116 (2012).
  52. F. Wu, T. Lovorn, E. Tutuc, and A. H. MacDonald, Hubbard Model Physics in Transition Metal Dichalcogenide Moiré Bands, Phys. Rev. Lett. 121, 026402 (2018).
  53. F. Wu, T. Lovorn, E. Tutuc, I. Martin, and A. H. MacDonald, Topological Insulators in Twisted Transition Metal Dichalcogenide Homobilayers, Phys. Rev. Lett. 122, 086402 (2019).
  54. M. Levin and A. Stern, Fractional Topological Insulators, Phys. Rev. Lett. 103, 196803 (2009).
  55. D. Xiao, G.-B. Liu, W. Feng, X. Xu, and W. Yao, Coupled Spin and Valley Physics in Monolayers of mos2 and Other Group-Vi Dichalcogenides, Phys. Rev. Lett. 108, 196802 (2012).
  56. J. Y. Lee, E. Khalaf, S. Liu, X. Liu, Z. Hao, P. Kim, and A. Vishwanath, Theory of correlated insulating behaviour and spin-triplet superconductivity in twisted double bilayer graphene, Nat. Commun. 10, 5333 (2019).
  57. See Supplemental Materials at http://link.aps.org/supplemental/10.1103/PhysRevResearch.3.L032070 for (1) the variational calculations of the energy for the valley polarized and intervalley coherent state, (2) Hartree-Fock calculations, (3) a discussion on the possibility of the Halperin state, and (4) an effective theory for the transition between the valley polarized Fermi liquid and fractional Chern insulator.
  58. A. Stern, Fractional Topological Insulators: A Pedagogical Review, Annu. Rev. Condens. Matter Phys. 7, 349 (2016).
  59. One may think of another possibility, analogous to the Halperin (m1,m2,n1) states. However, this state is not favored because of the opposite Chern number in the opposite valley [57].
  60. B. A. Bernevig and N. Regnault, Emergent many-body translational symmetries of abelian and non-abelian fractionally filled topological insulators, Phys. Rev. B 85, 075128 (2012).
  61. S. L. Sondhi, A. Karlhede, S. A. Kivelson, and E. H. Rezayi, Skyrmions and the crossover from the integer to fractional quantum hall effect at small zeeman energies, Phys. Rev. B 47, 16419 (1993).
  62. S. Chatterjee, M. Ippoliti, and M. P. Zaletel, Skyrmion Superconductivity: DMRG evidence for a topological route to superconductivity, arXiv:2010.01144.
  63. K. Kumar, K. Sun, and E. Fradkin, Chern-simons theory of magnetization plateaus of the spin-12 quantum xxz heisenberg model on the kagome lattice, Phys. Rev. B 90, 174409 (2014).
  64. K. Kumar, K. Sun, and E. Fradkin, Chiral spin liquids on the kagome lattice, Phys. Rev. B 92, 094433 (2015).
  65. W. Zhu, S.-S. Gong, T.-S. Zeng, L. Fu, and D. N. Sheng, Interaction-Driven Spontaneous Quantum Hall Effect on a Kagome Lattice, Phys. Rev. Lett. 117, 096402 (2016).

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