- Letter
- Open Access
Spectral compression and frequency shifts of single photons by cascade modulation
Phys. Rev. Research 8, L012035 – Published 10 February, 2026
DOI: https://doi.org/10.1103/9g56-2rh7
Abstract
Spectral manipulation of single photons as an essential quantum technology provides a feasible method for highly efficient quantum interconnects between quantum systems with different transition linewidths via flying photons, which expands the capabilities of quantum networks. In this Letter, we propose a scalable scheme based on side-end cavity and time-dependent phase modulation, which allows the spectral compression of single photons by hundreds of times and even more, with an efficiency higher than active spectrum filtering. In addition, the achievable frequency shifts of single photons can reach hundreds of gigahertz. These techniques allow the implementation of a high-efficiency quantum interface between single photons and atomic quantum memories, as well as high-visibility quantum interference between two independent single photons. Our scheme opens up a way for hybrid quantum networks involving quantum systems with different transition linewidths.
Physics Subject Headings (PhySH)
Article Text
References (37)
- D. Awschalom, et al., Development of quantum interconnects (QuICs) for next-generation information technologies, PRX Quantum 2, 017002 (2021).
- G. Kurizki, P. Bertet, Y. Kubo, K. Mølmer, D. Petrosyan, P. Rabl, and J. Schmiedmayer, Quantum technologies with hybrid systems, Proc. Natl Acad. Sci. USA 112, 3866 (2015).
- C. Chia, D. Huang, V. Leong, J. F. Kong, and K. E. J. Goh, Hybrid quantum systems with artificial atoms in solid state, Adv. Quantum Technol. 7, 2300461 (2024).
- D. Main, P. Drmota, D. P. Nadlinger, E. M. Ainley, A. Agrawal, B. C. Nichol, R. Srinivas, G. Araneda, and D. M. Lucas, Distributed quantum computing across an optical network link, Nature (London) 638, 383 (2025).
- D.-H. Kim, S. Hong, Y.-S. Kim, Y. Kim, S.-W. Lee, R. C. Pooser, K. Oh, S.-Y. Lee, C. Lee, and H.-T. Lim, Distributed quantum sensing of multiple phases with fewer photons, Nat. Commun. 15, 266 (2024).
- M. Saffman, T. G. Walker, and K. Mølmer, Quantum information with Rydberg atoms, Rev. Mod. Phys. 82, 2313 (2010).
- A. Reiserer and G. Rempe, Cavity-based quantum networks with single atoms and optical photons, Rev. Mod. Phys. 87, 1379 (2015).
- L. M. Duan, M. D. Lukin, J. I. Cirac, and P. Zoller, Long-distance quantum communication with atomic ensembles and linear optics, Nature (London) 414, 413 (2011).
- N. Sangouard, C. Simon, H. de Riedmatten, and N. Gisin, Quantum repeaters based on atomic ensembles and linear optics, Rev. Mod. Phys. 83, 33 (2011).
- T. E. Northup and R. Blatt, Quantum information transfer using photons, Nat. Photon. 8, 356 (2014).
- P. Senellart, G. Solomon, and A. White, High-performance semiconductor quantum-dot single-photon sources, Nat. Nanotechnol. 12, 1026 (2018).
- C.-Y. Lu and J.-W. Pan, Quantum-dot single-photon sources for the quantum internet, Nat. Nanotechnol. 16, 1294 (2021).
- N. Tomm, A. Javadi, N. O. Antoniadis, D. Najer, M. C. Löbl, A. R. Korsch, R. Schott, S. R. Valentin, A. D. Wieck, A. Ludwig, and R. J. Warburton, A bright and fast source of coherent single photons, Nat. Nanotechnol. 16, 399 (2021).
- X. Ding, Y.-P. Guo, M.-C. Xu, R.-Z. Liu, G.-Y. Zou, J.-Y. Zhao, Z.-X. Ge, Q.-H. Zhang, H.-L. Liu, L.-J. Wang, M.-C. Chen, H. Wang, Y.-M. He, Y.-H. Huo, C.-Y. Lu, and J.-W. Pan, High-efficiency single-photon source above the loss-tolerant threshold for efficient linear optical quantum computing, Nat. Photon. 19, 387 (2025).
- T. Wilk, S. C. Webster, A. Kuhn, and G. Rempe, Single-atom single-photon quantum interface, Science 317, 488 (2007).
- K. Hammerer, A. S. Sørensen, and E. S. Polzik, Quantum interface between light and atomic ensembles, Rev. Mod. Phys. 82, 1041 (2010).
- J. Borregaard, A. S. Sørensen, and P. Lodahl, Quantum networks with deterministic spin–photon interfaces, Adv. Quantum Technol. 2, 1800091 (2019).
- D. Kielpinski, J. F. Corney, and H. M. Wiseman, Quantum optical waveform conversion, Phys. Rev. Lett. 106, 130501 (2011).
- J. Lavoie, J. M. Donohue, L. G. Wright, A. Fedrizzi, and K. J. Resch, Spectral compression of single photons, Nat. Photon. 7, 363 (2013).
- Y. Li, T. Xiang, Y. Nie, M. Sang, and X. Chen, Spectral compression of single-photon-level laser pulse, Sci. Rep. 7, 43494 (2017).
- M. Allgaier, V. Ansari, L. Sansoni, C. Eigner, V. Quiring, R. Ricken, G. Harder, B. Brecht, and C. Silberhorn, Highly efficient frequency conversion with bandwidth compression of quantum light, Nat. Commun. 8, 14288 (2017).
- D. Zhu, et al., Spectral control of nonclassical light pulses using an integrated thin-film lithium niobate modulator, Light Sci. Appl. 11, 327 (2022).
- M. Karpiński, M. Jachura, L. J. Wright, and B. J. Smith, Bandwidth manipulation of quantum light by an electro-optic time lens, Nat. Photon. 11, 53 (2017).
- F. Sośnicki, M. Mikołajczyk, A. Golestani, and M. Karpiński, Interface between picosecond and nanosecond quantum light pulses, Nat. Photon. 17, 761 (2023).
- M. A. Seidler, X. J. Yeo, A. Cerè, and C. Kurtsiefer, Spectral compression of narrowband single photons with a resonant cavity, Phys. Rev. Lett. 125, 183603 (2020).
- C. Matthiesen, A. N. Vamivakas, and M. Atatüre, Subnatural linewidth single photons from a quantum dot, Phys. Rev. Lett. 108, 093602 (2012).
- Y. He, Y.-M. He, Y.-J. Wei, X. Jiang, M.-C. Chen, F.-L. Xiong, Y. Zhao, C. Schneider, M. Kamp, S. Höfling, C.-Y. Lu, and J.-W. Pan, Indistinguishable tunable single photons emitted by spin-flip raman transitions in InGaAs quantum dots, Phys. Rev. Lett. 111, 237403 (2013).
- A. Sipahigil, R. E. Evans, D. D. Sukachev, M. J. Burek, J. Borregaard, M. K. Bhaskar, C. T. Nguyen, J. L. Pacheco, H. A. Atikian, C. Meuwly, R. M. Camacho, F. Jelezko, E. Bielejec, H. Park, M. Lončar, and M. D. Lukin, An integrated diamond nanophotonics platform for quantum-optical networks, Science 354, 847 (2016).
- M. G. Raymer and C. J. McKinstrie, Quantum input-output theory for optical cavities with arbitrary coupling strength: Application to two-photon wave-packet shaping, Phys. Rev. A 88, 043819 (2013).
- O. Morin, M. Körber, S. Langenfeld, and G. Rempe, Deterministic shaping and reshaping of single-photon temporal wave functions, Phys. Rev. Lett. 123, 133602 (2019).
- L. J. Wright, M. Karpiński, C. Söller, and B. J. Smith, Spectral shearing of quantum light pulses by electro-optic phase modulation, Phys. Rev. Lett. 118, 023601 (2017).
- H. P. Specht, J. Bochmann, M. Mücke, B. Weber, E. Figueroa, D. L. Moehring, and G. Rempe, Phase shaping of single-photon wave packets, Nat. Photon. 3, 469 (2009).
- X. You, et al., Quantum interference with independent single-photon sources over 300 km fiber, Adv. Photon. 4, 066003 (2022).
- L. Zhai, G. N. Nguyen, C. Spinnle, J. Ritzmann, M. C. Löbl, A. D. Wieck, A. Ludwig, A. Javadi, and R. J. Warburton, Quantum interference of identical photons from remote GaAs quantum dots, Nat. Nanotechnol. 17, 829 (2022).
- S. E. Thomas, et al., Deterministic storage and retrieval of telecom light from a quantum dot single-photon source interfaced with an atomic quantum memory, Sci. Adv. 10, eadi7346 (2024).
- J. Liu, et al., A solid-state source of strongly entangled photon pairs with high brightness and indistinguishability, Nat. Nanotechnol. 14, 586 (2019).
- H. Wang, et al., On-demand semiconductor source of entangled photons which simultaneously has high fidelity, efficiency, and indistinguishability, Phys. Rev. Lett. 122, 113602 (2019).