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  • Letter
  • Open Access

Chiral electron momentum distribution upon strong-field ionization of atoms

A. Geyer1,*, J. Stindl1, I. Dwojak1, M. Hofmann1, N. Anders1, P. Roth1, P. Daum1, J. Kruse1, S. Jacob1 et al.

S. Gurevich1, N. Wong1, M. S. Schöffler1, L. Ph. H. Schmidt1, T. Jahnke2, M. Kunitski1, R. Dörner1, and S. Eckart1,†

  • *Contact author: geyer@atom.uni-frankfurt.de
  • †Contact author: eckart@atom.uni-frankfurt.de

Phys. Rev. Research 7, L032061 – Published 18 September, 2025

DOI: https://doi.org/10.1103/8pnf-fmqt

Abstract

We present a scheme to synthesize a three-dimensional laser field that produces a chiral electron momentum distribution upon strong-field ionization of atoms. Our approach employs two orthogonally propagating two-color laser beams. This results in a time-dependent three-dimensional electric field vector of the combined light field that varies for different positions within the focal volume. For each position, we conduct a simulation of the corresponding electron momentum distribution that includes nonadiabatic dynamics and Coulomb interaction after tunneling. For suitable laser parameters, only a small region of the focal volume contributes to the final momentum distribution. Thus, integrating over all position coordinates, a specific chiral laser field dominates. This leads to a volume-averaged electron momentum distribution, which is chiral, as well. This work will serve as a benchmark for future strong-field experiments aiming at the synthetization of well-defined, three-dimensional laser fields.

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