Reuse & Permissions

It is not necessary to obtain permission to reuse this article or its components as it is available under the terms of the Creative Commons Attribution 4.0 International license. This license permits unrestricted use, distribution, and reproduction in any medium, provided attribution to the author(s) and the published article's title, journal citation, and DOI are maintained. Please note that some figures may have been included with permission from other third parties. It is your responsibility to obtain the proper permission from the rights holder directly for these figures.

Export citation

Export citation

Choose format for download:

Download Citation
  • Open Access

Ion stopping force from Bohmian mechanics

P. L. Grande* and R. C. Fadanelli

F. Vuković, A. Niggas, and R. A. Wilhelm†

  • TU Wien, Institute of Applied Physics, Wiedner Hauptstrasse 8-10, 1040 Vienna, Austria

  • *Contact author: grande@if.ufrgs.br
  • †Contact author: wilhelm@iap.tuwien.ac.at

Phys. Rev. Research 8, 013178 – Published 17 February, 2026

DOI: https://doi.org/10.1103/7plq-xskx

Abstract

We employed Bohmian mechanics to solve the equations of motion for a charged particle traveling in a free electron gas. Quantum effects are accounted for by including the Bohm quantum-mechanical potential Q, which depends on the electronic density, in the typical classical description. Our approach provides a computationally efficient alternative to traditional quantum calculations for determining the electronic stopping force of charged particles in matter. We use this framework to investigate the stopping of fast protons and slow highly charged xenon ions in the free electron gas. For highly charged ions, we predict the stopping force as a function of the projectile charge exchange.

View figure in article

Physics Subject Headings (PhySH)

Article Text

Supplemental Material

References (66)

  1. D. Bohm, A suggested interpretation of the quantum theory in terms of “hidden” variables. I, Phys. Rev. 85, 166 (1952).
  2. D. Bohm, A suggested interpretation of the quantum theory in terms of “hidden” variables. II, Phys. Rev. 85, 180 (1952).
  3. P. R. Holland, The Quantum Theory of Motion (Cambridge University Press, Cambridge, 1993).
  4. D. Bohm and B. J. Hiley, The Undivided Universe: An Ontological Interpretation of Quantum Theory (Routledge, London, 1993).
  5. D. Dürr, S. Goldstein, and N. Zanghì, Quantum equilibrium and the origin of absolute uncertainty, J. Stat. Phys. 67, 843 (1992).
  6. R. E. Wyatt, Quantum Dynamics with Trajectories (Springer, New York, 2005).
  7. A. S. Sanz and S. Miret-Artés, A Trajectory Description of Quantum Processes. I. Fundamentals: A Bohmian Perspective, Lecture Notes in Physics (Springer Berlin, Heidelberg, 2012).
  8. A. S. Sanz and S. Miret-Artés, Quantum phase analysis with quantum trajectories: A step towards the creation of a Bohmian thinking, Am. J. Phys. 80, 525 (2012).
  9. X. Oriols, Quantum trajectory approach to time dependent transport in mesoscopic systems, Phys. Rev. Lett. 98, 066803 (2007).
  10. R. P. Rundle, T. Tilma, J. H. Samson, V. M. Dwyer, R. F. Bishop, and M. J. Everitt, General approach to quantum mechanics as a statistical theory, Phys. Rev. A 99, 012115 (2019).
  11. O. Morandi, On the connection between the Wigner and the Bohm quantum formalism, Phys. Lett. A 443, 128223 (2022).
  12. F. Haas, Quantum Plasmas: An Hydrodynamic Approach, Springer Series on Atomic, Optical, and Plasma Physics (Springer, New York, 2011).
  13. S. Lohmann and D. Primetzhofer, Disparate energy scaling of trajectory-dependent electronic excitations for slow protons and He ions, Phys. Rev. Lett. 124, 096601 (2020).
  14. X. Qi, F. Bruneval, and I. Maliyov, Ab initio prediction of a negative Barkas coefficient for slow protons and antiprotons in LiF, Phys. Rev. Lett. 128, 043401 (2022).
  15. C. Shepard, D. C. Yost, and Y. Kanai, Electronic excitation response of DNA to high-energy proton radiation in water, Phys. Rev. Lett. 130, 118401 (2023).
  16. A. Lim, W. M. C. Foulkes, A. P. Horsfield, D. R. Mason, A. Schleife, E. W. Draeger, and A. A. Correa, Electron elevator: Excitations across the band gap via a dynamical gap state, Phys. Rev. Lett. 116, 043201 (2016).
  17. K. Nordlund, M. Ghaly, R. S. Averback, M. Caturla, T. Diaz de la Rubia, and J. Tarus, Defect production in collision cascades in elemental semiconductors and fcc metals, Phys. Rev. B 57, 7556 (1998).
  18. M. A. Nastasi, J. W. Mayer, and Y. Wang, Ion Beam Analysis: Fundamentals and Applications (CRC Press, Taylor & Francis Group, Boca Raton, 2014).
  19. R. R. Wilson, Radiological use of fast protons, Radiology 47, 487 (1946).
  20. Y. T. Zhao, Y. N. Zhang, R. Cheng, B. He, C. L. Liu, X. M. Zhou, Y. Lei, Y. Y. Wang, J. R. Ren, X. Wang, Y. H. Chen, G. Q. Xiao, S. M. Savin, R. Gavrilin, A. A. Golubev, and D. H. H. Hoffmann, Benchmark experiment to prove the role of projectile excited states upon the ion stopping in plasmas, Phys. Rev. Lett. 126, 115001 (2021).
  21. V. E. Zakharov and S. V. Manakov, On the complete integrability of a nonlinear schrödinger equation, Theor. Math. Phys. 19, 551 (1974).
  22. E. Gruber, R. A. Wilhelm, R. Pétuya, V. Smejkal, R. Kozubek, A. Hierzenberger, B. C. Bayer, I. Aldazabal, A. K. Kazansky, F. Libisch, A. V. Krasheninnikov, M. Schleberger, S. Facsko, A. G. Borisov, A. Arnau, and F. Aumayr, Ultrafast electronic response of graphene to a strong and localized electric field, Nat. Commun. 7, 13948 (2016).
  23. A. Niggas, L. Fischer, S. Kretschmer, M. Werl, H. Biber, C. Speckmann, N. McEvoy, J. Kotakoski, F. Aumayr, A. V. Krasheninnikov, and R. A. Wilhelm, Charge-exchange-dependent energy loss of H and He in freestanding monolayers of graphene and MoS2, Phys. Rev. A 108, 062823 (2023).
  24. H. Hagstrum, Auger ejection of electrons from tungsten by noble gas ions, Phys. Rev. 96, 325 (1954).
  25. L. S. Cederbaum, J. Zobeley, and F. Tarantelli, Giant intermolecular decay and fragmentation of clusters, Phys. Rev. Lett. 79, 4778 (1997).
  26. R. A. Wilhelm, E. Gruber, J. Schwestka, R. Kozubek, T. I. Madeira, J. P. Marques, J. Kobus, A. V. Krasheninnikov, M. Schleberger, and F. Aumayr, Interatomic Coulombic decay: The mechanism for rapid deexcitation of hollow atoms, Phys. Rev. Lett. 119, 103401 (2017).
  27. P. L. Grande, Bohr's stopping-power formula derived for a classical free-electron gas, Phys. Rev. A 104, 012807 (2021).
  28. R. A. Wilhelm, The charge exchange of slow highly charged ions at surfaces unraveled with freestanding 2D materials, Surf. Sci. Rep. 77, 100577 (2022).
  29. P. Sigmund, Particle Penetration and Radiation Effects, 1st ed. (Springer, Berlin, Heidelberg, New York, 2006), Vol. 1, p. 151.
  30. V. Sharoglazova, M. Puplauskis, C. Mattschas, C. Toebes, and J. Klaers, Energy–speed relationship of quantum particles challenges Bohmian mechanics, Nature (London) 643, 67 (2025).
  31. J. Lindhard, On the properties of a gas of charged particles, K. Dan. Vidensk. Selsk. Mat.-Fys. Medd. 28, 1 (1954).
  32. A. Messiah, Quantum Mechanics (North-Holland Publishing Company, Amsterdam, 1967), Vol. 1.
  33. See Supplemental Material at http://link.aps.org/supplemental/10.1103/7plq-xskx for additional details, which includes Refs. [57, 58, 59, 60, 61, 62, 63, 64, 65].
  34. I. Nagy and P. M. Echenique, Stopping power of an electron gas for antiprotons at intermediate velocities, Phys. Rev. A 47, 3050 (1993).
  35. A. F. Lifschitz and N. R. Arista, Velocity-dependent screening in metals, Phys. Rev. A 57, 200 (1998).
  36. J. C. Ashley, Optical-data model for the stopping power of condensed matter for protons and antiprotons, J. Phys.: Condens. Matter 3, 2741 (1991).
  37. P. L. Grande, Alternative treatment for the energy-transfer and transport cross section in dressed electron-ion binary collisions, Phys. Rev. A 94, 042704 (2016).
  38. F. Matias, R. C. Fadanelli, P. L. Grande, N. E. Koval, R. D. Muiño, A. G. Borisov, N. R. Arista, and G. Schiwietz, Ground- and excited-state scattering potentials for the stopping of protons in an electron gas, J. Phys. B: At. Mol. Opt. Phys. 50, 185201 (2017).
  39. I. Nagy and A. Bergara, A model for the velocity-dependent screening, Nucl. Instrum. Methods Phys. Res. Sect. B 115, 58 (1996).
  40. M. Quijada, A. G. Borisov, I. Nagy, R. D. Muiño, and P. M. Echenique, Time-dependent density-functional calculation of the stopping power for protons and antiprotons in metals, Phys. Rev. A 75, 042902 (2007).
  41. R. A. Wilhelm and P. L. Grande, Unraveling energy loss processes of low energy heavy ions in 2D materials, Commun. Phys. 2, 89 (2019).
  42. A. Niggas, M. Werl, F. Aumayr, and R. A. Wilhelm, Charge exchange of slow highly charged ions from an electron beam ion trap with surfaces and 2D materials, J. Phys. B: At. Mol. Opt. Phys. 57, 072001 (2024).
  43. J. P. Briand, L. de Billy, P. Charles, S. Essabaa, P. Briand, R. Geller, J. P. Desclaux, S. Bliman, and C. Ristori, Production of hollow atoms by the excitation of highly charged ions in interaction with a metallic surface, Phys. Rev. Lett. 65, 159 (1990).
  44. M. H. Gass, U. Bangert, A. L. Bleloch, P. Wang, R. R. Nair, and A. K. Geim, Free-standing graphene at atomic resolution, Nat. Nanotechnol. 3, 676 (2008).
  45. Y. Abe, T. Tanaka, H. Sawada, E. Okunishi, Y. Kondo, Y. Tanishiro, and K. Takayanagi, Electron energy loss spectroscopy of graphene identified by aberration, corrected TEM at 300 kV, Microsc. Microanal. 15, 1484 (2009).
  46. R. Garcia-Molina, I. Abril, C. D. Denton, and S. Heredia-Avalos, Allotropic effects on the energy loss of swift H+ and He+ ion beams through thin foils, Nucl. Instrum. Methods Phys. Res. Sect. B 249, 6 (2006).
  47. See Supplemental Material of Ref. [22].
  48. A. Niggas, The role of contaminations in the interaction of highly charged ions with 2D materials, Ph.D. thesis, TU Wien, 2019.
  49. A. Niggas, S. Creutzburg, J. Schwestka, B. Wockinger, T. Gupta, P. L. Grande, D. Eder, J. P. Marques, B. C. Bayer, F. Aumayr, R. Bennett, and R. A. Wilhelm, Peeling graphite layer by layer reveals the charge exchange dynamics of ions inside a solid, Commun. Phys. 4, 180 (2021).
  50. Note that for larger scattering angles (i.e., transmission angles) the charge-state-dependent nuclear losses may become significant [41, 66].
  51. https://doi.org/10.5281/zenodo.18497123
  52. J. D. Jackson, Classical Electrodynamics, 3rd ed. (John Wiley and Sons, Hoboken, NJ, 1998).
  53. W. D. Wilson, L. G. Haggmark, and J. P. Biersack, Calculations of nuclear stopping, ranges, and straggling in the low-energy region, Phys. Rev. B 15, 2458 (1977).
  54. J. Ziegler, J. Biersack, and U. Littmark, The Stopping and Range of Ions in Solids (Pergamon Press, New York, 1985).
  55. R. A. Wilhelm, E. Gruber, V. Smejkal, S. Facsko, and F. Aumayr, Charge-state-dependent energy loss of slow ions. I. Experimental results on the transmission of highly charged ions, Phys. Rev. A 93, 052708 (2016).
  56. J. Burgdörfer, P. Lerner, and F. W. Meyer, Above-surface neutralization of highly charged ions: The classical over-the-barrier model, Phys. Rev. A 44, 5674 (1991).
  57. T. Kato, On the eigenfunctions of many-particle systems in quantum mechanics, Commun. Pure Appl. Math. 10, 151 (1957).
  58. M. Abramowitz and I. A. Stegun, Handbook of Mathematical Functions with Formulas, Graphs, and Mathematical Tables, Applied Mathematics Series (U.S. Government Printing Office, Washington, DC, 1972).
  59. D. R. Penn, Electron mean-free-path calculations using a model dielectric function, Phys. Rev. B 35, 482 (1987).
  60. M. Vos and P. L. Grande, Extension schemes of the dielectric function, and their implications for ion stopping calculations, J. Phys. Chem. Solids 133, 187 (2019).
  61. E. Shiles, T. Sasaki, M. Inokuti, and D. Y. Smith, Self-consistency and sum-rule tests in the Kramers-Kronig analysis of optical data: Applications to aluminum, Phys. Rev. B 22, 1612 (1980).
  62. B. Henke, E. Gullikson, and J. Davis, X-ray interactions: Photoabsorption, scattering, transmission, and reflection at E = 50–30,000 eV, Z = 1–92, At. Data Nucl. Data Tables 54, 181 (1993).
  63. Z. J. Ding, Ding's microsolid research group, research group webpage (2025), https://micro.ustc.edu.cn/ELF/Al.html.
  64. IAEA Nuclear Data Section, version 2024-11, https://nds.iaea.org/stopping/, released 27 November 2024, database maintained by IAEA Nuclear Data Section since 2015, currently compiled by Claudia Montanari.
  65. P. L. Grande and G. Schiwietz, CasP: Convolution approximation for swift particles (2021), http://www.casp-program.org, computer program, freely available.
  66. R. A. Wilhelm and W. Möller, Charge-state-dependent energy loss of slow ions. II. Statistical atom model, Phys. Rev. A 93, 052709 (2016).

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation