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Quantum non-Gaussian coherences of an oscillating atom

A. Kovalenko1,*, L. Lachman1,*, T. Pham2, K. Singh1, O. Číp2, J. Fiurášek1, L. Slodička1, and R. Filip1

  • *These authors contributed equally to this work.

Phys. Rev. Research 7, 033075 – Published 18 July, 2025

DOI: https://doi.org/10.1103/5nxx-r97j

Abstract

Quantum coherence between energy eigenstates of harmonic oscillators is essential for quantum physics. Even the most elementary binary superpositions of the ground and the higher eigenstate are highly required for quantum sensing, thermodynamics, and computing. We derive upper bounds for quantum coherences achieved by classical and Gaussian states and operations and, subsequently, obtain a hierarchy of the thresholds for the off-diagonal elements necessary to reach genuine quantum non-Gaussian coherences. The presented analysis demonstrates that certification based solely on estimation of coherences can cover the quantum non-Gaussian states, which are undetectable by the criteria based solely on the estimation of the corresponding state populations. We experimentally demonstrate the unambiguous observation of quantum non-Gaussian coherences in mechanical vibrations of a single calcium ion up to the superposition of zero and six phonons. The analysis of the robustness with respect to pure dephasing in a motional Ramsey experiment demonstrates the feasibility of their storage for up to more than 20 ms for superpositions with a large energy difference of participating number states. The presented observations prove that atomic oscillations go deeply into a diverse area of discrete quantum non-Gaussian coherent phenomena critical for their applications.

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References (63)

  1. L. Mandel and E. Wolf, Coherence properties of optical fields, Rev. Mod. Phys. 37, 231 (1965).
  2. A. D. Cronin, J. Schmiedmayer, and D. E. Pritchard, Optics and interferometry with atoms and molecules, Rev. Mod. Phys. 81, 1051 (2009).
  3. A. Streltsov, G. Adesso, and M. B. Plenio, Colloquium: Quantum coherence as a resource, Rev. Mod. Phys. 89, 041003 (2017).
  4. V. Giovannetti, S. Lloyd, and L. Maccone, Quantum-enhanced measurements: Beating the standard quantum limit, Science 306, 1330 (2004).
  5. L. Pezze, A. Smerzi, M. K. Oberthaler, R. Schmied, and P. Treutlein, Quantum metrology with nonclassical states of atomic ensembles, Rev. Mod. Phys. 90, 035005 (2018).
  6. S. Pirandola, U. L. Andersen, L. Banchi, M. Berta, D. Bunandar, R. Colbeck, D. Englund, T. Gehring, C. Lupo, C. Ottaviani et al., Advances in quantum cryptography, Adv. Opt. Photon. 12, 1012 (2020).
  7. J. Eisert, S. Scheel, and M. B. Plenio, Distilling Gaussian states with Gaussian operations is impossible, Phys. Rev. Lett. 89, 137903 (2002).
  8. J. Niset, J. Fiurášek, and N. J. Cerf, No-go theorem for Gaussian quantum error correction, Phys. Rev. Lett. 102, 120501 (2009).
  9. J. Broz, B. You, S. Khan, H. Häffner, D. E. Kaplan, and S. Rajendran, Test of causal nonlinear quantum mechanics by Ramsey interferometry with a trapped ion, Phys. Rev. Lett. 130, 200201 (2023).
  10. S. Lloyd and S. L. Braunstein, Quantum computation over continuous variables, Phys. Rev. Lett. 82, 1784 (1999).
  11. K. C. McCormick, J. Keller, S. C. Burd, D. J. Wineland, A. C. Wilson, and D. Leibfried, Quantum-enhanced sensing of a single-ion mechanical oscillator, Nature (London) 572, 86 (2019).
  12. W. Wang, Y. Wu, Y. Ma, W. Cai, L. Hu, X. Mu, Y. Xu, Z.-J. Chen, H. Wang, Y. Song et al., Heisenberg-limited single-mode quantum metrology in a superconducting circuit, Nat. Commun. 10, 4382 (2019).
  13. L. Hu, Y. Ma, W. Cai, X. Mu, Y. Xu, W. Wang, Y. Wu, H. Wang, Y. Song, C.-L. Zou et al., Quantum error correction and universal gate set operation on a binomial bosonic logical qubit, Nat. Phys. 15, 503 (2019).
  14. L. D. Burkhart, J. D. Teoh, Y. Zhang, C. J. Axline, L. Frunzio, M. H. Devoret, L. Jiang, S. M. Girvin, and R. J. Schoelkopf, Error-detected state transfer and entanglement in a superconducting quantum network, PRX Quantum 2, 030321 (2021).
  15. G. Maslennikov, S. Ding, R. Hablützel, J. Gan, A. Roulet, S. Nimmrichter, J. Dai, V. Scarani, and D. Matsukevich, Quantum absorption refrigerator with trapped ions, Nat. Commun. 10, 202 (2019).
  16. C. S. Wang, J. C. Curtis, B. J. Lester, Y. Zhang, Y. Y. Gao, J. Freeze, V. S. Batista, P. H. Vaccaro, I. L. Chuang, L. Frunzio et al., Efficient multiphoton sampling of molecular vibronic spectra on a superconducting bosonic processor, Phys. Rev. X 10, 021060 (2020).
  17. R. Howl, V. Vedral, D. Naik, M. Christodoulou, C. Rovelli, and A. Iyer, Non-Gaussianity as a signature of a quantum theory of gravity, PRX Quantum 2, 010325 (2021).
  18. N. F. Ramsey, A new molecular beam resonance method, Phys. Rev. 76, 996 (1949).
  19. X. Maître, E. Hagley, G. Nogues, C. Wunderlich, P. Goy, M. Brune, J. Raimond, and S. Haroche, Quantum memory with a single photon in a cavity, Phys. Rev. Lett. 79, 769 (1997).
  20. D. J. Wineland, C. Monroe, W. M. Itano, D. Leibfried, B. E. King, and D. M. Meekhof, Experimental issues in coherent quantum-state manipulation of trapped atomic ions, J. Res. Natl. Inst. Stand. Technol. 103, 259 (1998).
  21. L. Podhora, L. Lachman, T. Pham, A. Lešundák, O. Číp, L. Slodička, and R. Filip, Quantum non-Gaussianity of multiphonon states of a single atom, Phys. Rev. Lett. 129, 013602 (2022).
  22. U. Chabaud, G. Roeland, M. Walschaers, F. Grosshans, V. Parigi, D. Markham, and N. Treps, Certification of non-Gaussian states with operational measurements, PRX Quantum 2, 020333 (2021).
  23. K. C. McCormick, J. Keller, D. J. Wineland, A. C. Wilson, and D. Leibfried, Coherently displaced oscillator quantum states of a single trapped atom, Quantum Sci. Technol. 4, 024010 (2019).
  24. M. H. Michael, M. Silveri, R. Brierley, V. V. Albert, J. Salmilehto, L. Jiang, and S. M. Girvin, New class of quantum error-correcting codes for a bosonic mode, Phys. Rev. X 6, 031006 (2016).
  25. F. Wolf, C. Shi, J. C. Heip, M. Gessner, L. Pezzè, A. Smerzi, M. Schulte, K. Hammerer, and P. O. Schmidt, Motional Fock states for quantum-enhanced amplitude and phase measurements with trapped ions, Nat. Commun. 10, 2929 (2019).
  26. C. Flühmann, T. L. Nguyen, M. Marinelli, V. Negnevitsky, K. Mehta, and J. Home, Encoding a qubit in a trapped-ion mechanical oscillator, Nature (London) 566, 513 (2019).
  27. D. Leibfried, R. Blatt, C. Monroe, and D. Wineland, Quantum dynamics of single trapped ions, Rev. Mod. Phys. 75, 281 (2003).
  28. N. Akerman, S. Kotler, Y. Glickman, Y. Dallal, A. Keselman, and R. Ozeri, Single-ion nonlinear mechanical oscillator, Phys. Rev. A 82, 061402 (2010).
  29. M. Aspelmeyer, T. J. Kippenberg, and F. Marquardt, Cavity optomechanics, Rev. Mod. Phys. 86, 1391 (2014).
  30. C. Roos, T. Monz, K. Kim, M. Riebe, H. Häffner, D. James, and R. Blatt, Nonlinear coupling of continuous variables at the single quantum level, Phys. Rev. A 77, 040302 (2008).
  31. S. Ding, G. Maslennikov, R. Hablützel, and D. Matsukevich, Quantum simulation with a trilinear Hamiltonian, Phys. Rev. Lett. 121, 130502 (2018).
  32. D. Meekhof, C. Monroe, B. King, W. Itano, and D. Wineland, Generation of nonclassical motional states of a trapped atom, Phys. Rev. Lett. 76, 1796 (1996).
  33. S. Gardiner, J. Cirac, and P. Zoller, Nonclassical states and measurement of general motional observables of a trapped ion, Phys. Rev. A 55, 1683 (1997).
  34. M. Brownnutt, M. Kumph, P. Rabl, and R. Blatt, Ion-trap measurements of electric-field noise near surfaces, Rev. Mod. Phys. 87, 1419 (2015).
  35. V. Jarlaud, P. Hrmo, M. K. Joshi, and R. C. Thompson, Coherence properties of highly-excited motional states of a trapped ion, J. Phys. B: At. Mol. Opt. Phys. 54, 015501 (2021).
  36. A. R. Milne, C. Hempel, L. Li, C. L. Edmunds, H. J. Slatyer, H. Ball, M. R. Hush, and M. J. Biercuk, Quantum oscillator noise spectroscopy via displaced cat states, Phys. Rev. Lett. 126, 250506 (2021).
  37. Q. Turchette, C. Myatt, B. King, C. Sackett, D. Kielpinski, W. Itano, C. Monroe, and D. Wineland, Decoherence and decay of motional quantum states of a trapped atom coupled to engineered reservoirs, Phys. Rev. A 62, 053807 (2000).
  38. See Supplemental Material at http://link.aps.org/supplemental/10.1103/5nxx-r97j for the additional details on the experimental stability of motional coherences, their temporal decay, and derivation of the employed QNG coherence thresholds and dephasing depths.
  39. H. P. Yuen, Two-photon coherent states of the radiation field, Phys. Rev. A 13, 2226 (1976).
  40. L. Innocenti, L. Lachman, and R. Filip, Coherence-based operational nonclassicality criteria, Phys. Rev. Lett. 131, 160201 (2023).
  41. L. Lachman, I. Straka, J. Hloušek, M. Ježek, and R. Filip, Faithful hierarchy of genuine n-photon quantum non-Gaussian light, Phys. Rev. Lett. 123, 043601 (2019).
  42. C. J. Myatt, B. E. King, Q. A. Turchette, C. A. Sackett, D. Kielpinski, W. M. Itano, C. Monroe, and D. J. Wineland, Decoherence of quantum superpositions through coupling to engineered reservoirs, Nature (London) 403, 269 (2000).
  43. A. Ourjoumtsev, H. Jeong, R. Tualle-Brouri, and P. Grangier, Generation of optical ‘Schrödinger cats’ from photon number states, Nature (London) 448, 784 (2007).
  44. B. Vlastakis, G. Kirchmair, Z. Leghtas, S. E. Nigg, L. Frunzio, S. M. Girvin, M. Mirrahimi, M. H. Devoret, and R. J. Schoelkopf, Deterministically encoding quantum information using 100-photon Schrödinger cat states, Science 342, 607 (2013).
  45. U. Delić, D. Grass, M. Reisenbauer, T. Damm, M. Weitz, N. Kiesel, and M. Aspelmeyer, Levitated cavity optomechanics in high vacuum, Quantum Sci. Technol. 5, 025006 (2020).
  46. Y. Tsaturyan, A. Barg, E. S. Polzik, and A. Schliesser, Ultracoherent nanomechanical resonators via soft clamping and dissipation dilution, Nat. Nanotechnol. 12, 776 (2017).
  47. Y. Chu, P. Kharel, T. Yoon, L. Frunzio, P. T. Rakich, and R. J. Schoelkopf, Creation and control of multi-phonon Fock states in a bulk acoustic-wave resonator, Nature (London) 563, 666 (2018).
  48. U. von Lüpke, Y. Yang, M. Bild, L. Michaud, M. Fadel, and Y. Chu, Parity measurement in the strong dispersive regime of circuit quantum acoustodynamics, Nat. Phys. 18, 794 (2022).
  49. W. Wang, L. Hu, Y. Xu, K. Liu, Y. Ma, S.-B. Zheng, R. Vijay, Y. Song, L.-M. Duan, and L. Sun, Converting quasiclassical states into arbitrary Fock state superpositions in a superconducting circuit, Phys. Rev. Lett. 118, 223604 (2017).
  50. M. Reagor, W. Pfaff, C. Axline, R. W. Heeres, N. Ofek, K. Sliwa, E. Holland, C. Wang, J. Blumoff, K. Chou et al., Quantum memory with millisecond coherence in circuit QED, Phys. Rev. B 94, 014506 (2016).
  51. Y. Lu, I. Strandberg, F. Quijandría, G. Johansson, S. Gasparinetti, and P. Delsing, Propagating Wigner-negative states generated from the steady-state emission of a superconducting qubit, Phys. Rev. Lett. 126, 253602 (2021).
  52. M. Kudra, T. Abad, M. Kervinen, A. M. Eriksson, F. Quijandría, P. Delsing, and S. Gasparinetti, Experimental realization of deterministic and selective photon addition in a bosonic mode assisted by an ancillary qubit, arXiv:2212.12079.
  53. M. Kudra, M. Kervinen, I. Strandberg, S. Ahmed, M. Scigliuzzo, A. Osman, D. P. Lozano, M. O. Tholén, R. Borgani, D. B. Haviland et al., Robust preparation of Wigner-negative states with optimized snap-displacement sequences, PRX Quantum 3, 030301 (2022).
  54. M. Yukawa, K. Miyata, T. Mizuta, H. Yonezawa, P. Marek, R. Filip, and A. Furusawa, Generating superposition of up-to three photons for continuous variable quantum information processing, Opt. Express 21, 5529 (2013).
  55. H. Le Jeannic, A. Cavaillès, K. Huang, R. Filip, and J. Laurat, Slowing quantum decoherence by squeezing in phase space, Phys. Rev. Lett. 120, 073603 (2018).
  56. Y. Liu, Q. Liu, H. Sun, M. Chen, S. Wang, and T. Li, Coherent memory for microwave photons based on long-lived mechanical excitations, npj Quantum Inf. 9, 80 (2023).
  57. D. P. Lake, M. Mitchell, D. D. Sukachev, and P. E. Barclay, Processing light with an optically tunable mechanical memory, Nat. Commun. 12, 663 (2021).
  58. V. Fiore, Y. Yang, M. C. Kuzyk, R. Barbour, L. Tian, and H. Wang, Storing optical information as a mechanical excitation in a silica optomechanical resonator, Phys. Rev. Lett. 107, 133601 (2011).
  59. J. Franke, S. R. Muleady, R. Kaubruegger, F. Kranzl, R. Blatt, A. M. Rey, M. K. Joshi, and C. F. Roos, Quantum-enhanced sensing on an optical transition via emergent collective quantum correlations, Nature (London) 621, 740 (2023).
  60. J. Zhang, M. Um, D. Lv, J.-N. Zhang, L.-M. Duan, and K. Kim, Noon states of nine quantized vibrations in two radial modes of a trapped ion, Phys. Rev. Lett. 121, 160502 (2018).
  61. K. S. Chou et al., A superconducting dual-rail cavity qubit with erasure-detected logical measurements, Nat. Phys. 20, 1454 (2024).
  62. J. M. Gertler, B. Baker, J. Li, S. Shirol, J. Koch, and C. Wang, Protecting a bosonic qubit with autonomous quantum error correction, Nature (London) 590, 243 (2021).
  63. A. Kovalenko, M. T. Pham, K. Singh, O. Číp, and L. Slodicka, Experimental Data - Quantum non-Gaussian coherences of an oscillating atom, Zenodo, 2025, https://zenodo.org/records/15797402.

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