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  • Open Access

Unifying renormalized and bare viscosity in two-dimensional molecular dynamics simulations

Kazuma Yokota*, Masato Itami, and Shin-ichi Sasa

  • *Contact author: yokota.kazuma.i26@kyoto-u.jp

Phys. Rev. Research 8, 013234 – Published 3 March, 2026

DOI: https://doi.org/10.1103/58g1-c78g

Abstract

Fluctuating hydrodynamics provides a framework connecting mesoscopic fluctuations with macroscopic transport behavior. To bridge mesoscopic and macroscopic transport from microscopic dynamics, we introduce a wave-number-dependent viscosity, defined via the equilibrium correlation of time-averaged Fourier components of the fine-grained shear stress field. Two-dimensional molecular dynamics simulations reveal its small-wave-number divergence characteristic of the renormalized viscosity, while its large-wave-number behavior determines the bare viscosity, thereby establishing a link between mesoscopic and macroscopic transport based on microscopic dynamics.

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References (51)

  1. L. D. Landau and E. M. Lifshitz, Fluid Mechanics, Course of Theoretical Physics (Pergamon Press, London, 1959), Vol. 6.
  2. D. J. Tritton, Physical Fluid Dynamics, 2nd ed. (Clarendon Press, Oxford, 1988).
  3. A. Lucas and K. C. Fong, Hydrodynamics of electrons in graphene, J. Phys.: Condens. Matter 30, 053001 (2018).
  4. L. Fritz and T. Scaffidi, Hydrodynamic electronic transport, Annu. Rev. Condens. Matter Phys. 15, 17 (2024).
  5. W. Busza, K. Rajagopal, and W. van der Schee, Heavy ion collisions: The big picture and the big questions, Annu. Rev. Nucl. Part. Sci. 68, 339 (2018).
  6. I. S. Aranson and L. S. Tsimring, Patterns and collective behavior in granular media: Theoretical concepts, Rev. Mod. Phys. 78, 641 (2006).
  7. J. Toner, The Physics of Flocking: Birth, Death, and Flight in Active Matter (Cambridge University Press, Cambridge, 2024).
  8. A. Gromov, A. Lucas, and R. M. Nandkishore, Fracton hydrodynamics, Phys. Rev. Res. 2, 033124 (2020).
  9. C. W. Chang, D. Okawa, H. Garcia, A. Majumdar, and A. Zettl, Breakdown of Fourier's law in nanotube thermal conductors, Phys. Rev. Lett. 101, 075903 (2008).
  10. X. Xu, L. F. C. Pereira, Y. Wang, J. Wu, K. Zhang, X. Zhao, S. Bae, C. T. Bui, R. Xie, J. T. L. Thong, B. H. Hong, K. P. Loh, D. Donadio, B. Li, and B. Özyilmaz, Length-dependent thermal conductivity in suspended single-layer graphene, Nat. Commun. 5, 3689 (2014).
  11. V. Lee, C.-H. Wu, Z.-X. Lou, W.-L. Lee, and C.-W. Chang, Divergent and ultrahigh thermal conductivity in millimeter-long nanotubes, Phys. Rev. Lett. 118, 135901 (2017).
  12. L. Yang, Y. Tao, Y. Zhu, M. Akter, K. Wang, Z. Pan, Y. Zhao, Q. Zhang, Y.-Q. Xu, R. Chen, T. T. Xu, Y. Chen, Z. Mao, and D. Li, Observation of superdiffusive phonon transport in aligned atomic chains, Nat. Nanotechnol. 16, 764 (2021).
  13. R. Schmitz, Fluctuations in nonequilibrium fluids, Phys. Rep. 171, 1 (1988).
  14. R. Zwanzig, Nonlinear dynamics of collective modes, in Proceedings of the Sixth IUPAP Conference on Statistical Mechanics, edited by S. A. Rice, K. F. Freed, and J. C. Light (The University of Chicago Press, Chicago, IL, 1972), pp. 241–253.
  15. R. Zwanzig, K. S. J. Nordholm, and W. C. Mitchell, Memory effects in irreversible thermodynamics: Corrected derivation of transport equations, Phys. Rev. A 5, 2680 (1972).
  16. H. Mori and H. Fujisaka, On nonlinear dynamics of fluctuations, Prog. Theor. Phys. 49, 764 (1973).
  17. D. Forster, D. R. Nelson, and M. J. Stephen, Large-distance and long-time properties of a randomly stirred fluid, Phys. Rev. A 16, 732 (1977).
  18. O. Narayan and S. Ramaswamy, Anomalous heat conduction in one-dimensional momentum-conserving systems, Phys. Rev. Lett. 89, 200601 (2002).
  19. D. N. Zubarev and V. G. Morozov, Statistical mechanics of nonlinear hydrodynamic fluctuations, Physica A 120, 411 (1983).
  20. R. Zwanzig, Memory effects in irreversible thermodynamics, Phys. Rev. 124, 983 (1961).
  21. K. Saito, M. Hongo, A. Dhar, and S.-i. Sasa, Microscopic theory of fluctuating hydrodynamics in nonlinear lattices, Phys. Rev. Lett. 127, 010601 (2021).
  22. H. Nakano, Y. Minami, and K. Saito, Looking at bare transport coefficients in fluctuating hydrodynamics, arXiv:2502.15241.
  23. M. S. Green, Markoff random processes and the statistical mechanics of time-dependent phenomena. II. Irreversible processes in fluids, J. Chem. Phys. 22, 398 (1954).
  24. A. P. Thompson, H. M. Aktulga, R. Berger, D. S. Bolintineanu, W. M. Brown, P. S. Crozier, P. J. in 't Veld, A. Kohlmeyer, S. G. Moore, T. D. Nguyen, R. Shan, M. J. Stevens, J. Tranchida, C. Trott, and S. J. Plimpton, LAMMPS—A flexible simulation tool for particle-based materials modeling at the atomic, meso, and continuum scales, Comput. Phys. Commun. 271, 108171 (2022).
  25. W. C. Swope, H. C. Andersen, P. H. Berens, and K. R. Wilson, A computer simulation method for the calculation of equilibrium constants for the formation of physical clusters of molecules: Application to small water clusters, J. Chem. Phys. 76, 637 (1982).
  26. J. H. Irving and J. G. Kirkwood, The statistical mechanical theory of transport processes. IV. The equations of hydrodynamics, J. Chem. Phys. 18, 817 (1950).
  27. T. Yamada and K. Kawasaki, Nonlinear effects in the shear viscosity of critical mixtures, Prog. Theor. Phys. 38, 1031 (1967).
  28. B. J. Alder and T. E. Wainwright, Decay of the velocity autocorrelation function, Phys. Rev. A 1, 18 (1970).
  29. T. E. Wainwright, B. J. Alder, and D. M. Gass, Decay of time correlations in two dimensions, Phys. Rev. A 4, 233 (1971).
  30. Y. Pomeau and P. Résibois, Time dependent correlation functions and mode-mode coupling theories, Phys. Rep. 19, 63 (1975).
  31. A. Donev, J. B. Bell, A. de la Fuente, and A. L. Garcia, Diffusive transport by thermal velocity fluctuations, Phys. Rev. Lett. 106, 204501 (2011).
  32. A. Donev, J. B. Bell, A. de la Fuente, and A. L. Garcia, Enhancement of diffusive transport by non-equilibrium thermal fluctuations, J. Stat. Mech. (2011) P06014.
  33. G. Ciccotti, G. Jacucci, and I. R. McDonald, “Thought-experiments” by molecular dynamics, J. Stat. Phys. 21, 1 (1979).
  34. D. J. Evans, Equilibrium fluctuation expressions for the wave-vector- and frequency-dependent shear viscosity, Phys. Rev. A 23, 2622 (1981).
  35. G. Picard, A. Ajdari, F. Lequeux, and L. Bocquet, Elastic consequences of a single plastic event: A step towards the microscopic modeling of the flow of yield stress fluids, Eur. Phys. J. E 15, 371 (2004).
  36. M. Maier, A. Zippelius, and M. Fuchs, Emergence of long-ranged stress correlations at the liquid to glass transition, Phys. Rev. Lett. 119, 265701 (2017).
  37. K. Yokota, M. Itami, and S.-i. Sasa (unpublished).
  38. S. Lepri, R. Livi, and A. Politi, Thermal conduction in classical low-dimensional lattices, Phys. Rep. 377, 1 (2003).
  39. A. Dhar, Heat transport in low-dimensional systems, Adv. Phys. 57, 457 (2008).
  40. S.-i. Sasa, Derivation of hydrodynamics from the Hamiltonian description of particle systems, Phys. Rev. Lett. 112, 100602 (2014).
  41. P. C. Hohenberg and B. I. Halperin, Theory of dynamic critical phenomena, Rev. Mod. Phys. 49, 435 (1977).
  42. W. E. Alley and B. J. Alder, Generalized transport coefficients for hard spheres, Phys. Rev. A 27, 3158 (1983).
  43. B. Hess, Determining the shear viscosity of model liquids from molecular dynamics simulations, J. Chem. Phys. 116, 209 (2002).
  44. J. S. Hansen, P. J. Daivis, K. P. Travis, and B. D. Todd, Parameterization of the nonlocal viscosity kernel for an atomic fluid, Phys. Rev. E 76, 041121 (2007).
  45. A. Furukawa and H. Tanaka, Nonlocal nature of the viscous transport in supercooled liquids: Complex fluid approach to supercooled liquids, Phys. Rev. Lett. 103, 135703 (2009).
  46. N. Grimm, M. von Bischopinck, A. Zumbusch, and M. Fuchs, Long ranged stress correlations in the hard sphere liquid, J. Chem. Phys. 161, 144118 (2024).
  47. N. Grimm, J. Baschnagel, A. N. Semenov, A. Zippelius, and M. Fuchs, Stress correlations and stress memory kernels in viscoelastic fluids, Soft Matter 21, 4256 (2025).
  48. M. A. Rutgers, Forced 2D turbulence: Experimental evidence of simultaneous inverse energy and forward enstrophy cascades, Phys. Rev. Lett. 81, 2244 (1998).
  49. V. Nosenko and J. Goree, Shear flows and shear viscosity in a two-dimensional Yukawa system (dusty plasma), Phys. Rev. Lett. 93, 155004 (2004).
  50. E. Vogt, M. Feld, B. Fröhlich, D. Pertot, M. Koschorreck, and M. Köhl, Scale invariance and viscosity of a two-dimensional Fermi gas, Phys. Rev. Lett. 108, 070404 (2012).
  51. https://github.com/Kazu-Physics/viscosity2D.git.

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