- Open Access
Diffuse laser cooling based on the excited state of rubidium atoms via 420 nm blue light
Phys. Rev. Research 8, 033293 – Published 10 September, 2026
DOI: https://doi.org/10.1103/4jtk-471b
Abstract
To date, the laser cooling of rubidium atoms has inevitably relied on 780 nm cooling light corresponding to the first excited state . Here, we demonstrate diffuse laser cooling of atoms using the 420 nm transition without a preceding 780 nm cooling stage. A high-power laser is used as the cooling light to produce cold atoms in a 1-m-long diffuse-cooling cell. Absorption spectroscopy yields a cold-atom density of approximately . We compare the cooling performance of the 420 nm and conventional 780 nm diffuse-cooling schemes and verify the feasibility of using the high-excited-state transition as an independent cooling channel in this large-volume diffuse-cooling system. This approach provides an alternative cooling/pumping pathway for continuous cold-atom active optical clocks, where compatibility with the clock-lasing process and reduced cooling-light-induced perturbations are important. It is also expected to open up research directions and application prospects in frontier fields such as Rydberg atoms, quantum information, and so on.
Physics Subject Headings (PhySH)
Article Text
References (51)
- R. Ciuryło, E. Tiesinga, S. Kotochigova, and P. S. Julienne, Photoassociation spectroscopy of cold alkaline-earth-metal atoms near the intercombination line, Phys. Rev. A 70, 062710 (2004).
- R. A. Hart, X. Xu, R. Legere, and K. Gibble, A quantum scattering interferometer, Nature (London) 446, 892 (2007).
- A. L. Shaw, P. Scholl, R. Finkelstein, R. B.-S. Tsai, J. Choi, and M. Endres, Erasure cooling, control, and hyperentanglement of motion in optical tweezers, Science 388, 845 (2025).
- D. Wineland, C. Monroe, D. Meekhof, B. King, D. Leibfried, W. Itano, J. Bergquist, D. Berkeland, J. Bollinger, and J. Miller, Quantum state manipulation of trapped atomic ions, Proc. R. Soc. London A 454, 411 (1998).
- S. Chu, L. Hollberg, J. E. Bjorkholm, A. Cable, and A. Ashkin, Three-dimensional viscous confinement and cooling of atoms by resonance radiation pressure, Phys. Rev. Lett. 55, 48 (1985).
- E. L. Raab, M. Prentiss, A. Cable, S. Chu, and D. E. Pritchard, Trapping of neutral sodium atoms with radiation pressure, Phys. Rev. Lett. 59, 2631 (1987).
- H. J. Metcalf and P. Van der Straten, Laser Cooling and Trapping (Springer Science & Business Media, New York, 1999).
- J. S. Rosenberg, L. Christakis, E. Guardado-Sanchez, Z. Z. Yan, and W. S. Bakr, Observation of the Hanbury Brown–Twiss effect with ultracold molecules, Nat. Phys. 18, 1062 (2022).
- T. Weber, J. Herbig, M. Mark, H.-C. Nagerl, and R. Grimm, Bose-Einstein condensation of cesium, Science 299, 232 (2003).
- X. Zheng, J. Dolde, V. Lochab, B. N. Merriman, H. Li, and S. Kolkowitz, Differential clock comparisons with a multiplexed optical lattice clock, Nature (London) 602, 425 (2022).
- J. Li, X. Chen, D. Zhang, W. Wang, Y. Zhou, M. He, J. Fang, L. Zhou, C. He, J. Jiang, et al., Realization of a cold atom gyroscope in space, Natl. Sci. Rev. 12, nwaf012 (2025).
- A. Aeppli, K. Kim, W. Warfield, M. S. Safronova, and J. Ye, Clock with systematic uncertainty, Phys. Rev. Lett. 133, 023401 (2024).
- T. Zhang, L. Chen, Y. Shu, W. Xu, Y. Cheng, Q. Luo, Z. Hu, and M. Zhou, Ultrahigh-sensitivity Bragg atom gravimeter and its application in testing Lorentz violation, Phys. Rev. Appl. 20, 014067 (2023).
- J. J. Osborne, I. P. McCulloch, B. Yang, P. Hauke, and J. C. Halimeh, Large-scale 2 + 1D U(1) gauge theory with dynamical matter in a cold-atom quantum simulator, Commun. Phys. 8, 273 (2025).
- J. C. Halimeh, M. Aidelsburger, F. Grusdt, P. Hauke, and B. Yang, Cold-atom quantum simulators of gauge theories, Nat. Phys. 21, 25 (2025).
- O. Heavens, Radiative transition probabilities of the lower excited states of the alkali metals, J. Opt. Soc. Am. 51, 1058 (1961).
- C. Gerz, T. Hodapp, P. Jessen, K. Jones, W. Phillips, C. Westbrook, and K. Molmer, The temperature of optical molasses for two different atomic angular momenta, Europhys. Lett. 21, 661 (1993).
- S. Rosi, A. Burchianti, S. Conclave, D. S. Naik, G. Roati, C. Fort, and F. Minardi, -enhanced grey molasses on the transition of rubidium-87 atoms, Sci. Rep. 8, 1301 (2018).
- C. Liang, S. Gao, J. Liu, G. Wang, S. Yan, J. Yang, L. Zhu, and X. Ma, Multi-parameter optimization of polarization gradient cooling for atoms based on reinforcement learning, Opt. Express 32, 40364 (2024).
- J. Hu, A. Urvoy, Z. Vendeiro, V. Crépel, W. Chen, and V. Vuletić, Creation of a Bose-condensed gas of by laser cooling, Science 358, 1078 (2017).
- A. M. Kaufman, B. J. Lester, and C. A. Regal, Cooling a single atom in an optical tweezer to its quantum ground state, Phys. Rev. X 2, 041014 (2012).
- J. D. Thompson, T. Tiecke, A. S. Zibrov, V. Vuletić, and M. D. Lukin, Coherence and Raman sideband cooling of a single atom in an optical tweezer, Phys. Rev. Lett. 110, 133001 (2013).
- J. Goldwin, S. B. Papp, B. Demarco, and D. S. Jin, Two-species magneto-optical trap with and , Phys. Rev. A 65, 021402(R) (2002).
- K. N. Jarvis, J. Devlin, T. Wall, B. Sauer, and M. Tarbutt, Blue-detuned magneto-optical trap, Phys. Rev. Lett. 120, 083201 (2018).
- J. G. Bohnet, Z. Chen, J. M. Weiner, D. Meiser, M. J. Holland, and J. K. Thompson, A steady-state superradiant laser with less than one intracavity photon, Nature (London) 484, 78 (2012).
- H. Xue, Y. Feng, S. Chen, X. Wang, X. Yan, Z. Jiang, and Z. Zhou, A continuous cold atomic beam interferometer, J. Appl. Phys. 117, 094901 (2015).
- R. Gutterres, C. Amiot, A. Fioretti, C. Gabbanini, M. Mazzoni, and O. Dulieu, Determination of the state dipole matrix element and radiative lifetime from the photoassociation spectroscopy of the ) long-range state, Phys. Rev. A 66, 024502 (2002).
- R. C. Das, D. Shylla, A. Bera, and K. Pandey, Narrow-line cooling of using open transition at 420 nm, J. Phys. B: At. Mol. Opt. Phys. 56, 025301 (2023).
- R. C. Das, T. Ravi, S. Khan, and K. Pandey, Continuous loading of a magneto-optical trap of using a narrow transition, Phys. Rev. A 109, 063107 (2024).
- J. Marek and P. Munster, Radiative lifetimes of excited states of rubidium up to quantum number n = 12, J. Phys. B: At. Mol. Phys. 13, 1731 (1980).
- M. Safronova and U. Safronova, Critically evaluated theoretical energies, lifetimes, hyperfine constants, and multipole polarizabilities in , Phys. Rev. A 83, 052508 (2011).
- W. Ketterle, A. Martin, M. A. Joffe, and D. E. Pritchard, Slowing and cooling atoms in isotropic laser light, Phys. Rev. Lett. 69, 2483 (1992).
- H. Batelaan, S. Padua, D. Yang, C. Xie, R. Gupta, and H. Metcalf, Slowing of atoms with isotropic light, Phys. Rev. A 49, 2780 (1994).
- J. Wan, X. Wang, X. Zhang, Y. Meng, W. Wang, Y. Sun, and L. Liu, Quasi-one-dimensional diffuse laser cooling of atoms, Phys. Rev. A 105, 033110 (2022).
- X. Wang, Y. Sun, and L. Liu, Realizing fast temperature measurement and simulating Maxwell's demon with nearly nondestructive detection in cold atoms, Photonics Res. 10, 1947 (2022).
- P. Chang, S. Zhang, H. Shang, and J. Chen, Stabilizing diode laser to 1 Hz-level Allan deviation with atomic spectroscopy for Rb four-level active optical frequency standard, Appl. Phys. B 125, 196 (2019).
- J. Zhang, T. Shi, J. Miao, D. Yu, and J. Chen, An extremely bad-cavity laser, npj Quantum Inf. 10, 87 (2024).
- I. I. Ryabtsev, I. I. Beterov, D. B. Tretyakov, V. M. Entin, and E. A. Yakshina, Spectroscopy of cold rubidium Rydberg atoms for applications in quantum information, Phys. Usp. 59, 196 (2016).
- S. Zhang, X. Zhang, J. Tu, Z. Jiang, H. Shang, C. Zhu, W. Yang, J. Cui, and J. Chen, A 420 nm blue diode laser for the potential rubidium optical frequency standard, Chin. Phys. Lett. 34, 074211 (2017).
- R. Sun, W. Zhao, Y. Zhang, T. Yuan, H. Liu, S. Gu, and J. Chen, 420 nm Rb optical frequency standard with short-term frequency stability below , Opt. Express 34, 28391 (2026).
- S. Zhang, X. Zhang, J. Cui, Z. Jiang, H. Shang, C. Zhu, P. Chang, L. Zhang, J. Tu, and J. Chen, Compact Rb optical frequency standard with stability, Rev. Sci. Instrum. 88, 103106 (2017).
- L. Salvi, L. Cacciapuoti, G. Tino, and G. Rosi, Atom interferometry with blue transitions, Phys. Rev. Lett. 131, 103401 (2023).
- S. Trémine, E. De Clercq, and P. Verkerk, Isotropic light versus six-beam molasses for Doppler cooling of atoms from background vapor: Theoretical comparison, Phys. Rev. A 96, 023411 (2017).
- X. Guan, J. Zhang, X. Gao, Y. Wang, T. Shi, and J. Chen, A 780 nm optical frequency standard based on diffuse laser cooled atoms, Appl. Phys. Lett. 126, 031104 (2025).
- P. Horak, J.-Y. Courtois, and G. Grynberg, Atom cooling and trapping by disorder, Phys. Rev. A 58, 3953 (1998).
- G. Grynberg, P. Horak, and C. Mennerat-Robilliard, Spatial diffusion of atoms cooled in a speckle field, Europhys. Lett. 49, 424 (2000).
- F.-X. Esnault, D. Holleville, N. Rossetto, S. Guerandel, and N. Dimarcq, High-stability compact atomic clock based on isotropic laser cooling, Phys. Rev. A 82, 033436 (2010).
- X. Wang, Y. Sun, H. Cheng, J. Wan, Y. Meng, L. Xiao, and L. Liu, Nearly nondestructive thermometry of labeled cold atoms and application to isotropic laser cooling, Phys. Rev. Appl. 14, 024030 (2020).
- Y. Hsiao, H. Chen, P. Tsai, and Y. Chen, Cold atomic media with ultrahigh optical depths, Phys. Rev. A 90, 055401 (2014).
- S. Sinha, S. Achar, S. Satheesh, and A. Sharma, Precision measurement of the saturation intensity in rubidium at 420 nm, arXiv:2606.30871.
- X. Wang, Y. Sun, and L. Liu, Characterization of isotropic laser cooling for application in quantum sensing, Opt. Express 29, 43435 (2021).