- Open Access
Tuning interactions between static-field-shielded polar molecules with microwaves
Phys. Rev. Research 8, 023087 – Published 29 April, 2026
DOI: https://doi.org/10.1103/2td6-pcvk
Abstract
The ability to tune interparticle interactions is one of the main advantages of using ultracold quantum gases for quantum simulation of many-body physics. Current experiments with ultracold polar molecules employ shielding with microwave or static electric fields to prevent destructive collisional losses. The interaction potential of microwave-shielded molecules can be tuned by using microwaves of two different polarizations, while for static-field-shielded molecules the tunability of interactions is more limited and depends on the particular species. In this work, we propose a general method to tune the interactions between static-field-shielded molecules by applying a microwave field. We carry out coupled-channel scattering calculations in a field-dressed basis set to determine loss rate coefficients and scattering lengths. We find that both the s-wave scattering length and the dipole length can be widely tuned by changing the parameters of the microwave field, while maintaining strong suppression of lossy collisions.
Physics Subject Headings (PhySH)
Article Text
References (32)
- T. Lahaye, C. Menotti, L. Santos, M. Lewenstein, and T. Pfau, The physics of dipolar bosonic quantum gases, Rep. Prog. Phys. 72, 126401 (2009).
- L. Chomaz, I. Ferrier-Barbut, F. Ferlaino, B. Laburthe-Tolra, B. L. Lev, and T. Pfau, Dipolar physics: A review of experiments with magnetic quantum gases, Rep. Prog. Phys. 86, 026401 (2023).
- T. Langen, G. Valtolina, D. Wang, and J. Ye, Quantum state manipulation and cooling of ultracold molecules, Nat. Phys. 20, 702 (2024).
- A. Schindewolf, J. Hertkorn, I. Stevenson, M. Ciardi, P. Gross, D. Wang, T. Karman, G. Quéméner, S. Will, T. Pohl, and T. Langen, From few- to many-body physics: Strongly dipolar molecular Bose-Einstein condensates and quantum fluids, arXiv:2512.14511.
- T. Karman, N. Bigagli, W. Yuan, S. Zhang, I. Stevenson, and S. Will, Double microwave shielding, PRX Quantum 6, 020358 (2025).
- W. Yuan, S. Zhang, N. Bigagli, H. Kwak, C. Warner, T. Karman, I. Stevenson, and S. Will, Extreme loss suppression and wide tunability of dipolar interactions in an ultracold molecular gas, arXiv:2505.08773.
- M. Schmidt, L. Lassablière, G. Quéméner, and T. Langen, Self-bound dipolar droplets and supersolids in molecular Bose-Einstein condensates, Phys. Rev. Res. 4, 013235 (2022).
- G. E. Astrakharchik, J. Boronat, I. L. Kurbakov, and Y. E. Lozovik, Quantum phase transition in a two-dimensional system of dipoles, Phys. Rev. Lett. 98, 060405 (2007).
- H. P. Büchler, E. Demler, M. Lukin, A. Micheli, N. Prokof'ev, G. Pupillo, and P. Zoller, Strongly correlated 2D quantum phases with cold polar molecules: Controlling the shape of the interaction potential, Phys. Rev. Lett. 98, 060404 (2007).
- M. Ciardi, K. R. Pedersen, T. Langen, and T. Pohl, Self-bound superfluid membranes and monolayer crystals of ultracold polar molecules, Phys. Rev. Lett. 135, 153401 (2025).
- R. Bause, A. Christianen, A. Schindewolf, I. Bloch, and X.-Y. Luo, Ultracold sticky collisions: Theoretical and experimental status, J. Phys. Chem. A 127, 729 (2023).
- A. V. Avdeenkov, M. Kajita, and J. L. Bohn, Suppression of inelastic collisions of polar state molecules in an electrostatic field, Phys. Rev. A 73, 022707 (2006).
- G. Wang and G. Quéméner, Tuning ultracold collisions of excited rotational dipolar molecules, New J. Phys. 17, 035015 (2015).
- K. Matsuda, L. De Marco, J.-R. Li, W. G. Tobias, G. Valtolina, G. Quéméner, and J. Ye, Resonant collisional shielding of reactive molecules using electric fields, Science 370, 1324 (2020).
- T. Karman and J. M. Hutson, Microwave shielding of ultracold polar molecules, Phys. Rev. Lett. 121, 163401 (2018).
- L. Lassablière and G. Quéméner, Controlling the scattering length of ultracold dipolar molecules, Phys. Rev. Lett. 121, 163402 (2018).
- L. Anderegg, S. Burchesky, Y. Bao, S. S. Yu, T. Karman, E. Chae, K.-K. Ni, W. Ketterle, and J. M. Doyle, Observation of microwave shielding of ultracold molecules, Science 373, 779 (2021).
- G. Valtolina, K. Matsuda, W. G. Tobias, J.-R. Li, L. De Marco, and J. Ye, Dipolar evaporation of reactive molecules to below the Fermi temperature, Nature (London) 588, 239 (2020).
- A. Schindewolf, R. Bause, X.-Y. Chen, M. Duda, T. Karman, I. Bloch, and X.-Y. Luo, Evaporation of microwave-shielded polar molecules to quantum degeneracy, Nature (London) 607, 677 (2022).
- N. Bigagli, W. Yuan, S. Zhang, B. Bulatovic, T. Karman, I. Stevenson, and S. Will, Observation of Bose-Einstein condensation of dipolar molecules, Nature (London) 631, 289 (2024).
- Z. Shi, Z. Huang, F. Deng, W.-J. Jin, S. Yi, T. Shi, and D. Wang, Bose-Einstein condensation of ultracold sodium-rubidium molecules with tunable dipolar interactions, arXiv:2508.20518.
- B. Mukherjee, M. D. Frye, C. R. Le Sueur, M. R. Tarbutt, and J. M. Hutson, Shielding collisions of ultracold CaF molecules with static electric fields, Phys. Rev. Res. 5, 033097 (2023).
- B. Mukherjee and J. M. Hutson, Controlling collisional loss and scattering lengths of ultracold dipolar molecules with static electric fields, Phys. Rev. Res. 6, 013145 (2024).
- C. Chin, R. Grimm, P. Julienne, and E. Tiesinga, Feshbach resonances in ultracold gases, Rev. Mod. Phys. 82, 1225 (2010).
- H. P. Büchler, A. Micheli, and P. Zoller, Three-body interactions with cold polar molecules, Nat. Phys. 3, 726 (2007).
- A. V. Gorshkov, P. Rabl, G. Pupillo, A. Micheli, P. Zoller, M. D. Lukin, and H. P. Büchler, Suppression of inelastic collisions between polar molecules with a repulsive shield, Phys. Rev. Lett. 101, 073201 (2008).
- T. Karman, Microwave shielding with far-from-circular polarization, Phys. Rev. A 101, 042702 (2020).
- J. M. Hutson and C. R. Le Sueur, molscat: A program for non-reactive quantum scattering calculations on atomic and molecular collisions, Comput. Phys. Commun. 241, 9 (2019).
- J. M. Hutson and C. R. Le Sueur, molscat, bound and field, version 2023.0, GitHub (2023), https://github.com/molscat/molscat.
- J. Dutta, B. Mukherjee, and J. M. Hutson, Universality in the microwave shielding of ultracold polar molecules, Phys. Rev. Res. 7, 023164 (2025).
- B. Mukherjee, J. M. Hutson, and K. R. A. Hazzard, SU() magnetism with ultracold molecules, New J. Phys. 27, 013013 (2025).
- C. J. Ho, J. Dutta, B. Mukherjee, J. M. Hutson, and M. R. Tarbutt, Data for “Tuning interactions between static-field-shielded polar molecules with microwaves”, Zenodo (2026), https://doi.org/10.5281/zenodo.18474678.