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Signatures of bulk g-wave altermagnetism in optically excited α−MnTe

Luca Felipe Haag1, Marius Weber2,1, Kai Leckron1, Libor Šmejkal3,4,5, Jairo Sinova2,6, and Hans Christian Schneider1

Phys. Rev. Materials 10, 074413 – Published 22 July, 2026

DOI: https://doi.org/10.1103/ypfs-fy39

Abstract

For planar d-wave altermagnets, it has been shown that a spin polarization can be induced in a controlled fashion by ultrashort-pulse excitation, even though the material is magnetically compensated. Here, we theoretically analyze the response of the prototypical bulk g−wave altermagnet α−MnTe to linearly polarized ultrashort pulses. We demonstrate how the electronic spin response in α−MnTe exhibits different symmetry characteristics by calculating the excited electron distributions based on ab initio band structure data. These characteristics depend not only on the nodal planes of the bulk g-wave altermagnet, but also on the excitation pulse. We present a simple procedure to analyze the excited-state characteristics via two-dimensional cuts through the three-dimensional Brillouin zone, which can be used as guidance to present-day magneto-optical techniques.

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Altermagnetic and Related Materials

Editors of Physical Review Materials are pleased to present the Collection on Altermagnetic and Related Materials, highlighting cutting-edge advances in theoretical and experimental identification of novel altermagnetic materials, their properties, and their potential applications. The Collection is being guest-edited by Kirill Belashchenko of the University of Nebraska-Lincoln (USA), Cheng Song of Tsinghua University (China), and Peter Wadley of The University of Nottingham (UK). Every article published in this collection underwent a rigorous peer review process, adhering to the same high standards applied to all papers. The Physical Review Materials editorial team managed the peer review and made all editorial decisions.

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References (38)

  1. L. Šmejkal, J. Sinova, and T. Jungwirth, Beyond conventional ferromagnetism and antiferromagnetism: A phase with nonrelativistic spin and crystal rotation symmetry, Phys. Rev. X 12, 031042 (2022).
  2. L. Šmejkal, J. Sinova, and T. Jungwirth, Emerging research landscape of altermagnetism, Phys. Rev. X 12, 040501 (2022).
  3. C. Song, H. Bai, Z. Zhou, L. Han, H. Reichlova, J. H. Dil, J. Liu, X. Chen, and F. Pan, Altermagnets as a new class of functional materials, Nat. Rev. Mater. 10, 473 (2025).
  4. L. Bai, W. Feng, S. Liu, L. Šmejkal, Y. Mokrousov, and Y. Yao, Altermagnetism: Exploring new frontiers in magnetism and spintronics, Adv. Funct. Mater. 34, 2409327 (2024).
  5. Z. Guo, X. Wang, W. Wang, G. Zhang, X. Zhou, and Z. Cheng, Spin-polarized antiferromagnets for spintronics, Adv. Mater. 37, 2505779 (2025).
  6. J. Krempaský, L. Šmejkal, S. W. D'Souza, M. Hajlaoui, G. Springholz, K. Uhlířová, F. Alarab, P. C. Constantinou, V. Strocov, D. Usanov, W. R. Pudelko, R. González-Hernández, A. Birk Hellenes, Z. Jansa, H. Reichlová, Z. Šobáň, R. D. Gonzalez Betancourt, P. Wadley, J. Sinova, D. Kriegner, et al., Altermagnetic lifting of Kramers spin degeneracy, Nature (London) 626, 517 (2024).
  7. T. Osumi, S. Souma, T. Aoyama, K. Yamauchi, A. Honma, K. Nakayama, T. Takahashi, K. Ohgushi, and T. Sato, Observation of a giant band splitting in altermagnetic MnTe, Phys. Rev. B 109, 115102 (2024).
  8. S. Lee, S. Lee, S. Jung, J. Jung, D. Kim, Y. Lee, B. Seok, J. Kim, B. G. Park, L. Šmejkal, C.-J. Kang, and C. Kim, Broken Kramers degeneracy in altermagnetic MnTe, Phys. Rev. Lett. 132, 036702 (2024).
  9. O. Fedchenko, J. Minár, A. Akashdeep, S. W. D'Souza, D. Vasilyev, O. Tkach, L. Odenbreit, Q. Nguyen, D. Kutnyakhov, N. Wind, L. Wenthaus, M. Scholz, K. Rossnagel, M. Hoesch, M. Aeschlimann, B. Stadtmüller, M. Kläui, G. Schönhense, T. Jungwirth, A. B. Hellenes, et al., Observation of time-reversal symmetry breaking in the band structure of altermagnetic RuO2, Sci. Adv. 10, eadj4883 (2024).
  10. Z. Feng, X. Zhou, L. Šmejkal, L. Wu, Z. Zhu, H. Guo, R. González-Hernández, X. Wang, H. Yan, P. Qin, X. Zhang, H. Wu, H. Chen, Z. Meng, L. Liu, Z. Xia, J. Sinova, T. Jungwirth, and Z. Liu, An anomalous Hall effect in altermagnetic ruthenium dioxide, Nat. Electron. 5, 735 (2022).
  11. P. Keßler, L. Garcia-Gassull, A. Suter, T. Prokscha, Z. Salman, D. Khalyavin, P. Manuel, F. Orlandi, I. I. Mazin, R. Valentí, and S. Moser, Absence of magnetic order in RuO2: Insights from μSR spectroscopy and neutron diffraction, npj Spintron. 2, 50 (2024).
  12. M. Hiraishi, H. Okabe, A. Koda, R. Kadono, T. Muroi, D. Hirai, and Z. Hiroi, Nonmagnetic ground state in RuO2 revealed by muon spin rotation, Phys. Rev. Lett. 132, 166702 (2024).
  13. R. D. Gonzalez Betancourt, J. Zubáč, R. Gonzalez-Hernandez, K. Geishendorf, Z. Šobáň, G. Springholz, K. Olejník, L. Šmejkal, J. Sinova, T. Jungwirth, S. T. B. Goennenwein, A. Thomas, H. Reichlová, J. Železný, and D. Kriegner, Spontaneous anomalous Hall effect arising from an unconventional compensated magnetic phase in a semiconductor, Phys. Rev. Lett. 130, 036702 (2023).
  14. R. D. Gonzalez Betancourt, J. Zubáč, K. Geishendorf, P. Ritzinger, B. Růžičková, T. Kotte, J. Železný, K. Olejník, G. Springholz, B. Büchner, A. Thomas, K. Výborný, T. Jungwirth, H. Reichlová, and D. Kriegner, Anisotropic magnetoresistance in altermagnetic MnTe, npj Spintron. 2, 45 (2024).
  15. A. Hariki, A. Dal Din, O. J. Amin, T. Yamaguchi, A. Badura, D. Kriegner, K. W. Edmonds, R. P. Campion, P. Wadley, D. Backes, L. S. I. Veiga, S. S. Dhesi, G. Springholz, L. Šmejkal, K. Výborný, T. Jungwirth, and J. Kuneš, X-ray magnetic circular dichroism in altermagnetic α−MnTe, Phys. Rev. Lett. 132, 176701 (2024).
  16. D. Y. Kazmin, V. Esin, Y. S. Barash, A. Timonina, N. Kolesnikov, and E. Deviatov, Andreev reflection for MnTe altermagnet candidate, Physica B 696, 416602 (2025).
  17. K. P. Kluczyk, K. Gas, M. J. Grzybowski, P. Skupiński, M. A. Borysiewicz, T. Fąs, J. Suffczyński, J. Z. Domagala, K. Grasza, A. Mycielski, M. Baj, K. H. Ahn, K. Výborný, M. Sawicki, and M. Gryglas-Borysiewicz, Coexistence of anomalous Hall effect and weak magnetization in a nominally collinear antiferromagnet MnTe, Phys. Rev. B 110, 155201 (2024).
  18. O. J. Amin, A. Dal Din, E. Golias, Y. Niu, A. Zakharov, S. C. Fromage, C. J. B. Fields, S. L. Heywood, R. B. Cousins, F. Maccherozzi, J. Krempaský, J. H. Dil, D. Kriegner, B. Kiraly, R. P. Campion, A. W. Rushforth, K. W. Edmonds, S. S. Dhesi, L. Šmejkal, T. Jungwirth, et al., Nanoscale imaging and control of altermagnetism in MnTe, Nature (London) 636, 348 (2024).
  19. M. Weber, S. Wust, L. Haag, A. Akashdeep, K. Leckron, C. Schmitt, R. Ramos, T. Kikkawa, E. Saitoh, M. Kläui, et al., All optical excitation of spin polarization in d-wave altermagnets, arXiv:2408.05187.
  20. M. Weber, K. Leckron, L. F. Haag, R. Jaeschke-Ubiergo, L. Šmejkal, J. Sinova, and H. C. Schneider, Ultrafast electron dynamics in a planar d-wave altermagnet, Newton 1, 100266 (2025).
  21. I. I. Mazin, Altermagnetism in MnTe: Origin, predicted manifestations, and routes to detwinning, Phys. Rev. B 107, L100418 (2023).
  22. M. Vila, V. Sunko, and J. E. Moore, Orbital-spin locking and its optical signatures in altermagnets, Phys. Rev. B 112, L020401 (2025).
  23. Z. Zhou, S. Sharma, J. K. Dewhurst, and J. He, Magnetizing altermagnets through ultrafast asymmetric spin dynamics, Phys. Rev. B 114, 024409 (2026).
  24. A. Eskandari-asl, J. I. Facio, O. Janson, A. Avella, and J. van den Brink, Controlling photoexcited electron spin by light polarization in ultrafast-pumped altermagnets, Phys. Rev. B 112, 024401 (2025).
  25. Z. Zhou, S. Sharma, and J. He, Ultrafast all-optical control of magnetization in the g−wave altermagnet CrSb, Phys. Rev. B 113, 064434 (2026).
  26. S. Li, R. Wang, T. Frauenheim, Z. Zhou, and J. He, Asymmetric spin canting and demagnetization dynamics driven by laser fields in two-dimensional altermagnets, Nano Lett. 26, 1995 (2026).
  27. I. Gray, Q. Deng, Q. Tian, M. Chilcote, J. S. Dodge, M. Brahlek, and L. Wu, Time-resolved magneto-optical effects in the altermagnet candidate MnTe, Appl. Phys. Lett. 125, 212404 (2024).
  28. J. K. Dewhurst et al., The Elk code, http://elk.sourceforge.net/.
  29. J. P. Perdew, K. Burke, and M. Ernzerhof, Generalized gradient approximation made simple, Phys. Rev. Lett. 77, 3865 (1996).
  30. A. I. Liechtenstein, V. I. Anisimov, and J. Zaanen, Density-functional theory and strong interactions: Orbital ordering in Mott-Hubbard insulators, Phys. Rev. B 52, R5467(R) (1995).
  31. D. Kriegner, H. Reichlova, J. Grenzer, W. Schmidt, E. Ressouche, J. Godinho, T. Wagner, S. Y. Martin, A. B. Shick, V. V. Volobuev, G. Springholz, V. Holý, J. Wunderlich, T. Jungwirth, and K. Výborný, Magnetic anisotropy in antiferromagnetic hexagonal MnTe, Phys. Rev. B 96, 214418 (2017).
  32. I. I. Mazin and K. D. Belashchenko, Origin of the gossamer ferromagnetism in MnTe, Phys. Rev. B 110, 214436 (2024).
  33. D. Litvin and W. Opechowski, Spin groups, Physica 76, 538 (1974).
  34. See Supplemental Material at http://link.aps.org/supplemental/10.1103/ypfs-fy39 for details of the optical transitions involved in the excitation processes, additional information about the fit procedure and a discussion of the influence of spin-orbit coupling.
  35. S. Essert and H. C. Schneider, Electron-phonon scattering dynamics in ferromagnetic metals and their influence on ultrafast demagnetization processes, Phys. Rev. B 84, 224405 (2011).
  36. M. Stiehl, M. Weber, C. Seibel, J. Hoefer, S. T. Weber, D. M. Nenno, H. C. Schneider, B. Rethfeld, B. Stadtmüller, and M. Aeschlimann, Role of primary and secondary processes in the ultrafast spin dynamics of nickel, Appl. Phys. Lett. 120, 062410 (2022).
  37. S. Reimers, L. Odenbreit, L. Šmejkal, V. N. Strocov, P. Constantinou, A. B. Hellenes, R. Jaeschke Ubiergo, W. H. Campos, V. K. Bharadwaj, A. Chakraborty, T. Denneulin, W. Shi, R. E. Dunin-Borkowski, S. Das, M. Kläui, J. Sinova, and M. Jourdan, Direct observation of altermagnetic band splitting in CrSb thin films, Nat. Commun. 15, 2116 (2024).
  38. J. Oleszkiewicz, A. Kisiel, and S. Ignatowicz, Optical properties and dielectric function of manganese telluride thin films, Thin Solid Films 157, 1 (1988).

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