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    Unconventional magnetotransport and antiferromagnetic order in Eu2InTe5

    Matthew S. Cook1,*, Brenden R. Ortiz1, Pyeongjae Park1, Karolina Gornicka1,2, Suchismita Sarker3, Jiaqiang Yan1, and Michael A. McGuire1

    • *Contact author: cookms@ornl.gov

    Phys. Rev. Materials 9, 124410 – Published 16 December, 2025

    DOI: https://doi.org/10.1103/wq1l-wj9k

    Abstract

    We report on the structural characterization and physical properties of Eu2InTe5, a distorted square-net motif antiferromagnetic semiconductor. Single crystal x-ray diffraction measurements reveal a distortion of the Te square-net layers such that an orthorhombic supercell is necessary to accurately describe the structure. Magnetization, resistivity, and specific heat measurements confirm antiferromagnetic ordering at TN=7.3K. Anisotropy in magnetization data suggests the magnetic moments are oriented parallel to the c axis. We observe an unconventional transverse magnetoresistance and Hall resistivity in the paramagnetic state (T≤80K), indicating strong coupling between localized Eu2+ magnetic moments and conduction electrons. Resistivity and Hall measurements indicate the material is a heavily doped semiconductor, with impurity states related to disorder. Our findings highlight a relatively unexplored Eu-based antiferromagnetic semiconductor with unconventional magnetotransport behavior.

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