Anomalous spin-pumping behavior of half-metallic ferromagnet/-wave superconductor heterostructures
Phys. Rev. Materials 10, 104801 – Published 1 October, 2026
DOI: https://doi.org/10.1103/t7vq-dl3f
Abstract
Spin-pumping experiments in superconductor–ferromagnet heterostructures, which probe spin-sinking by the superconductor, have revealed a variety of complex behaviors. Most experimental studies have focused on conventional -wave superconductors combined with metallic or insulating ferromagnets. Here, we study a -wave superconductor paired with a half-metallic ferromagnet in epitaxial heterostructures with two crystalline orientations: one in which YBCO is -axis oriented and the other in which YBCO grows along the (103) direction. Using ferromagnetic resonance (FMR), we probe the temperature-dependent Gilbert damping coefficient α. For (103) heterostructures, α(T) initially decreases below , but then increases at lower temperatures, eventually exceeding normal-state levels. This behavior can be understood in terms of the opening of the superconducting gap and spin transport via nodal quasiparticles, whose contribution is enhanced when the plane of YBCO is exposed at the interface. In stark contrast, -axis heterostructures exhibit a pronounced enhancement of α(T) below , peaking at before decaying. This anomaly suggests the dominance of interfacial Andreev bound states, arising from a locally suppressed superconducting order parameter because of proximity effects with the half-metallic LSMO.